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DEVELOPMENT OF ONE DIMENSIONAL ANGULAR CORRELATION OF POSITRON ANNIHILATION RADIATION MEASU REING WIDE MOMENTUM REGION FOR NON-DESTRUCTIVE INSPECTION OF NUCLEAR REACTOR PRESSURE VESSEL

Research Project

Project/Area Number 12358005
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section展開研究
Research Field Nuclear engineering
Research InstitutionTOHOKU UNIVERSITY

Principal Investigator

HASEGAWA Masayuki  TOHOKU UNIVERSITY, INSTITUTE FOR MATERIALS RESEARCH, PROFESSOR, 金属材料研究所, 教授 (80005975)

Co-Investigator(Kenkyū-buntansha) YUBUTA Kunio  TOHOKU UNIVERSITY, INSTITUTE FOR MATERIALS RESEARCH, RESEARCH ASSOCIATE, 金属材料研究所, 助手 (00302208)
TANG Zeng  TOHOKU UNIVERSITY, INSTITUTE FOR MATERIALS RESEARCH, RESEARCH ASSOCIATE, 金属材料研究所, 助手 (80271972)
NAGAI Yasuyoshi  TOHOKU UNIVERSITY, INSTITUTE FOR MATERIALS RESEARCH, ASSOCIATE PROFESSOR, 金属材料研究所, 助教授 (10302209)
Project Period (FY) 2000 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥36,080,000 (Direct Cost: ¥33,500,000、Indirect Cost: ¥2,580,000)
Fiscal Year 2001: ¥11,180,000 (Direct Cost: ¥8,600,000、Indirect Cost: ¥2,580,000)
Fiscal Year 2000: ¥24,900,000 (Direct Cost: ¥24,900,000)
KeywordsPOSITRON ANNIHILATION / LIFE MANAGEMENT OF NUCLEAR POWER REACTOR / WIDE RANGE MOMENTUM DISTRIBUTION MEASUREMENT / POSITION SENSITIVE GAMMA-RAY DETECTOR / 陽電子消滅 / 原子炉圧力容器鋼 / 非破壊検査 / 角相関 / 照射脆化
Research Abstract

Ensuring safe operation of nuclear power reactors is a recent urgent issue since the reactors of the first generation are going over their initially designed operating lifetimes. One of the most important problem is the embrittlement of the reactor pressure vessel (RPV) steels by neutron irradiation, which is considered to be caused by the ultrafine precipitation of Cu impurities contained in the RPV steels (〜O.3 %) of the first generation induced by neutron irradiation. However, little is known about the irradiation-induced Cu precipitates or aggregations because it is very difficult to observe them even by current high-resolution transmission electron microscopes (HR-TEM). The aim of this work is to develop a new type of one-dimensional angular correlation of positron annihilation radiation (1D-ACAR) apparatus for non-destructive inspection of the RPV steels. Our final goal is to establish the method, using the apparatus, to analyze the formation process and the structure of the ultr … More afine Cu precipitates, difficult to detect by other techniques, utilizing affinity-induced positron confinement in the Cu precipitate which we have recently found.
For the above purpose, we have to develop a new 1D-ACAR apparatus which enables us to measure the momentum distribution of not only conduction electrons but also core electrons with high momentum resolution (〜1x10^<-3>mc). Thus, we developed a pair of position sensitive gamma-ray detectors with high position resolution (〜2 mm), high counting rate (wide effective area : 150 mm x 150 mm) and high time resolution. One detector was mounted on a fixed support, and the other detector was mounted on a support movable vertically. In the next step, the sample chamber for low temperature (〜15K) measurements and the support for the chamber were constructed. Finally, the electric system for the coincidence measurement of a pair of positron annihilation gamma-rays was set up.
We performed a test measurement of the new 1D-ACAR apparatus for the evaluation of the performance. A long tail in the high momentum region was observed, which results in high background and poor position resolution. We found that this was caused by the reflection of the scintillation photons at the light-guide surfaces. To remove this effect, the detectors are now improving the setting of the light-guide geometry and the amplifiers for the timing outputs. Less

Report

(3 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • Research Products

    (26 results)

All Other

All Publications (26 results)

  • [Publications] Y.Nagai et al.: "Fermi Surface of Nano Crystalline Embedded Particles in Material-bcc Cu in Fe-"Physical Review Letters. 87. 176402 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Nagai et al.: "Irradiation-induced Cu aggregations in Fe : An Origin of Embrittlement of Reactor Pressure Vessel Steels"Physical Review B. 63. 134110 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z.Tang et al.: "First-principles calculation of the coincidence Doppler broadening of positron annihilation radiation"Physical Review B. 65. 045108 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Onitsuka et al.: "Deformation-Enhanced Cu precipitation in Fe-Cu Alloy Studied by Positron Annihilation Spectroscopy"Physical Review B. 65. 012204 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z.Tang et al.: "Density Functional Study of Metastable bcc Copper : Electronic structure and momentum density of positron-electron pairs"Physical Review B. (掲載受理). (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Nagai et al.: "Role of Vacancy-Solute Complex in the Initial Rapid Age Hardening in an Al-Cu-Mg Alloy"Acta Materialia. 59. 913-920 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Fermi Surface of Nano Crystalline Embedded Particles in Material - bcc Cu in Fe -"Physical Review Letters. 87. 176402 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Irradiation-induced Cu aggregations in Fe : An Origin of Embrittlement of Reactor Pressure Vessel Steels"Physical Review B. 63. 134110 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z. Tang et al.: "First-principles calculation of the coincidence Doppler broadening of positron annihilation radiation"Physical Review B. 65. 045108 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Onitsuka et al.: "Deformation-Enhanced Cu precipitation in Fe-Cu Alloy Studied by Positron Annihilation"Physical Review B. 65. 012204 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z. Tang et al.: "Density Functional Study of Metastable bcc Copper : Electronic structure and momentum density of positron-electron pairs"Physical Review B, Editorially approved for publication. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Role of Vacancy-Solute Complex in the Initial Rapid Age Hardening in an Al-Cu-Mg Alloy"Acta Materialia. 59. 913-920 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Coincidence Doppler Broadening Study of the Pre-precipitation Stage of an Al-Cu-Mg-Ag alloy"Philosophical Magazine A. (Accepted for publication). (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z. Tang et al.: "Identification of Vacancy-Oxygen Complexes in Si by Coincidence Doppler Broadening of Positron Annihilation Radiation and First-principles Calculations"Material Science Forum. 363-365. 67-96 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Study of Ultrafine Cu Precipitates in Neutron-Irradiated Fe Utilizing Positron Quantum-dot-like States"Material Science Forum. 363-365. 91-93 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Hasegawa et al.: "Magic Number Vacancy Clusters in Graphite and Silicon"Material Science Forum. 363-365. 132-134 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Hasegawa et al.: "Positron and Positronium Studies of Irradiation-induced defects and microvoids in vitreous and metamict silica"Nuclear Instrument Method in Physical Research B. 166-167. 431-439 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Nagai et al.: "Chemical Analysis of Precipitates in Metallic Alloys Using Coincidence Doppler Broadening of Positron Annihilation Radiation"Radiation Physics and Chemistry. 58. 737-742 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Nagai et al.: "Irradiation-induced Cu aggregations in Fe : An Origin of Embrittlement of Reactor Pressure Vessel Steels"Physical Review B. 63. 134110 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Nagai et al.: "Study of Ultrafine Cu Precipitates in Neutron-Irradiated Fe Utilizing Positron Quantum-dot-like States"Material Science Forum. 363-365. 91-93 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 永井康介, 長谷川雅幸: "陽電子消滅法によるFe-Cuモデル合金中の微小Cu析出物の解析"金属. 71・8. 742-748 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Nagai et al.: "Fermi Surface of Nano Crystalline Embedded Particles in Material - bcc Cu in Fe -"Physical Review Letters. 87. 176402 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Z.Tang et al.: "First-principles calculation of the coincidence Doppler broadening of positron annihilation radiation"Physical Review B. 65. 045108 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Onitsuka et al.: "Deformation-Enhanced Cu precipitation in Fe-Cu Alloy Studied by Positron Annihilation Spectroscopy"Physical Review B. 65. 012204 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Nagai et al: "An Origin of Embrittlement of Reactor Pressure Vessel Steels : Ultra-fine Cu Precipitates "Phys.Rev.B. 63(in press). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Nagai et al.: "Study of Ultrafine Cu Precipitates in Neutron-Irradiated Fe Utilizing Positron Quantum-dot-like States"Material Science Forum. (in press).

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2016-04-21  

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