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Development of high energy-resolution inverse photoemission spectroscopy

Research Project

Project/Area Number 12440080
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionThe University of Tokyo

Principal Investigator

MIZOKAWA Takashi  Graduate School of Frontier Sciences, Associate Professor, 大学院・新領域創成科学研究科, 助教授 (90251397)

Project Period (FY) 2000 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥15,500,000 (Direct Cost: ¥15,500,000)
Fiscal Year 2002: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2001: ¥2,800,000 (Direct Cost: ¥2,800,000)
Fiscal Year 2000: ¥11,800,000 (Direct Cost: ¥11,800,000)
Keywordsinverse photoemission spectroscopy / off-plane Eagle mounting / dispersion matching / ultraviolet light / parallel plate analyzer / unoccupied state / Cu oxides / Ru oxides / 真空紫外線分光 / 電子線エネルギー分析器 / off-plane eagle 型配置 / 低次元遷移金属酸化物
Research Abstract

It is highly important to study occupied and unoccupied states of electrons in order to understand electronic properties of solids. Photoemission spectroscopy (PES) and inverse photoemission spectroscopy (IPES) are complementary to each other and very powerful experimental methods to study the electronic structure of solids. While PES directly observes the occupied states below the Fermi level, IPES observes the unoccupied states above the Fermi level. Energy resolution of 2 meV has been achieved for PES and, consequently detailed information of occupied states of solids has been obtained. On the other hands, since the energy resolution of IPES is about 200 meV, information of unoccupied states is considerably limited by the poor energy resolution. Understanding of high-Tc cuprates is one of the most challenging problems in the field of solid state physics. The lacking of information about unoccupied states prevents us from the full understanding of their electronic properties. We have developed high energy-resolution IPES technique in order to study unoccupied states of high-Tc cuprates. We made a new IPES machine based on two ideas to improve the energy resolution : off-plane Eagle mounting of the optical system and dispersion matching between incoming electron and outgoing photon. The off-plane Eagle mounting of the optical system has been completed by setting the diffraction grating, the detector, and the test sample. In order to achieve the dispersion matching between the incoming electron beam and outgoing photon, we have made the parallel plate electron source and have investigated whether the electron beam is obtained as expected. Since the parallel plate electron source cannot supply enough current on the sample to measure inverse photoemission spectra, the IPES system is still not completed yet. We will continue the effort to construct the IPES machine.

Report

(4 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • Research Products

    (11 results)

All Other

All Publications (11 results)

  • [Publications] T.Mizokawa, C.Kim, Z.-X.Shen, A.Ino, T.Yoshida, A.Fujimori, M.Goto, H.Eisaki, S.Uchida, M.Tagami, K.Yoshida, A.I.Rykov, Y.Siohara, K.Tomimoto, S.Tajima, Yuh Yamada, S.Horii, N.Yamada, Yasuji Yamada, I.Hirabayashi: "Angle-resolved photoemission study of insulating and metallic Cu-O chains in PrBa_2Cu_3O_7 and PrBa_2Cu_4O_8"Physical Review Letters. 85. 4779-4783 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Mizokawa, L.H.Tjeng, G.A.Sawatzky, G.Ghiringhelli, O.Tjengberg, N.B.Brookes, H.Fukazawa, S.Nakatsuji, Y.Maeno: "Spin-orbit coupling in the Mott insulator Ca_2RuO_4"Physical Review Letters. 87. 077202-1-077202-4 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Mizokawa, L.H.Tjeng, P.G.Steeneken, L.Tsukada, T.Yamamoto, K.Uchinoura: "Photoemission and x-ray absorption study of misfit-layered (Bi,Pb)-Sr-Co-O compounds : Electronic structure of a hole-doped Co-O triangular lattice"Physical Review B. 64. 115104-1-115104-7 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Mizokawa, C.Kim, Z.-X.Shen, T.Yoshida, A.Fujimori, S.Horii, Yuh Yamada, K.Nakada, H.Ikuta, U.Mizutani: "Observation of Single Particle Spectral Function of a Tomonaga-Luttinger Liquid : Angle-Resolved Photoemission Study of Zn-Doped PrBa_2Cu_4O_8"Physical Review B. 65. 193101-1-193101-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Mizokawa, C. Kim, Z. -X. Shen, A. Ino, T. Yoshida, A. Fujimori, M. Goto, H. Eisaki, S. Uchida, M. Tagami, K. Yoshida, A. I. Rykoy, Y. Siohara, K. Tomimoto, S. Tajima, Yuh Yamada, S. Horii, N. Yamada, Yasuji Yamada, and I. Hirabayashi: "Angle-resolved photoemission study of insulating and metallic Cu-O chains in PrBa_2Cu_3O_7 and PrBa_2CU_4O_8"Physical Review Letters. 85. 4779 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Mizokawa, L. H. Tjeng, G. A. Sawatzky, G. Ghiringhelli, O. Tjengberg, N. B. Brookes, H. Fukazawa, S. Nakatsuji, and Y. Maeno: "Spin-orbit coupling in the Mott insulator Ca_2RuO_4"Physical Review Letters. 87. 077202 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Mizokawa, L. H. Tjeng, P. G. Steeneken, I Tsukada, T. Yamamoto, and K. Uchinoura: "Photoemission and x-ray absorption study of misfit-layered (Bi,Pb)-Sr-Co-O compounds : Electronic structure of a hole-doped Co-O triangular lattice"Physical Review B. 64. 115104 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Mizokawa, C. Kim, Z. -X. Shen, T. Yosbida, A. Fujimori, S. Horii, Yuh Yamada, K. Nakada, H. Ikuta and U. Mizutani: "Observation of Single Particle Spectral Function of a Tomonaga-Luttinger Liquid : Angle-Resolved Photoemission Study of Zn-Doped PrBa_2Cu_4O_8"Physical Review B. 65. 193101 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Mizokawa, K.Nakada, C.Kim, Z.-X.Shen, T.Yoshida, A.Fujimori, S.Horii, Yuh Yamada, H.Ikuta, U.Mizutani: "Angle-resolved photoemission study of Zn-doped PrBa_2Cu_4O_8 : Possible observation of single-particle spectral function for a Tomonaga-Luttinger liquid"Physical Review B. 65巻. 19310 1-1-19310 1-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Mizokawa, et al.: "Spin-orbit coupling in the Mott insulator Ca_2RuO_4"Physical Review Letters. 87巻・077202. 1-4 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Mizokawa et al.: "Angle-Resolved Photoemission Study of Insulating and Metallic Cu-O Chains in PrBa_2Cu_3O_7 and PrBa_2Cu_4O2_8"Physical Review Letters. 85. 4779-4782 (2000)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2020-05-15  

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