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Study on magnetic excitons in uranium-based heavy fermion superconductors

Research Project

Project/Area Number 12440091
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionNagoya University

Principal Investigator

SATO Noriaki  Nagoya University, Graduate School of Science, Associate Professor, 大学院・理学研究科, 助教授 (30170773)

Co-Investigator(Kenkyū-buntansha) ASO Naofumi  University of Tokyo, Institute for Solid State Physics, Assistant Professor, 物性研究所, 助手 (40313118)
Project Period (FY) 2000 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥11,400,000 (Direct Cost: ¥11,400,000)
Fiscal Year 2002: ¥2,000,000 (Direct Cost: ¥2,000,000)
Fiscal Year 2001: ¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 2000: ¥7,200,000 (Direct Cost: ¥7,200,000)
Keywordsuranium compounds / heavy fermions / superconductivity / magnetic exciton / UPd_2Al_3 / UNi_2Al_3 / UGe_2 / URu_2Si_2 / UNi_2Ai_3
Research Abstract

(1) Magnetic exciton mediated superconductivity in UPd_2Al_3
We succeeded in preparing single crystals of high quality, and measured physical properties of those crystals to obtain information of the magnetism and superconductivity. We discovered the existence of two components in inelastic neutron scattering spectra, and we safely ascribed the lower energy component to quasiparticle excitations and the higher energy one to magnetic excitons. We proposed a new model, that is called "dual nature of 5f electrons", to analyze the data. We finally found the strong coupling between the two components. We also found that the spectra are consistent with spectra obtained from tunneling experiments within the Eliashberg equation framework. From these results, we pointed out that the superconducting attractive interaction is mediated by exchange of bosonic magnetic excitons. This result was reported in Nature, 410(2001)340-343.
(2) Magnetism and superconductivity in UNi_2Al_3
In UNi_2Al_3 that has … More the same crystal structure as UPd_2Al_3, the antiferromagnetic ordered state also coexists with superconductivity. We carried out NMR experiments, and found that the Knight shift shows no reduction below the superconducting transition temperature, in remarkably contrast with the isotropic reduction in UPd_2Al_3. From this result together with the absence of the Pauli limiting effect in the temperature dependence of the superconducting upper critical field, we concluded that the spin-triplet (odd parity) paring is formed.
(3) Magnetism and superconductivity in UGe_2 and URu_2Si_2
We prepared single crystals to investigate the correlation of ferromagnetism and superconductivity in UGe_2. We measured the dc magnetization and ac magnetic susceptibility under high pressures, and we found that the superconducting volume fraction grows with increasing pressure. From this, we suggested that the superconductivity coexists in a competitive way with the ferromagnetism.
We also carried out the dilatation measurements under high pressure for single crystals of URu_2Si_2. We found an anomaly in the thermal expansion coefficient that corresponds to the phase transition between hidden and antiferromagnetic order. Less

Report

(4 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • Research Products

    (39 results)

All Other

All Publications (39 results)

  • [Publications] T.Nishioka, G.Motoyama, S.Nakamura, H.Kadoya, N.K.Sato: "Unusual nature of ferromagnetism coexisting with superconductivity in UGe_2"Phys. Rev. Lett.. 88. 237203-1-237203-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakon, N.K.Sato, Y.Nakanishi, T.Komatsubara, M.Motokawa: "Magnetic phase diagram of UPd_2Al_3 in high magnetic fields"Jpn. J. Appl. Phys.. 41. 3673-3677 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Ishida, N.K.Sato, N.Aso, C.Geibel, F.Steglich 他: "Spin-triplet superconductivity in UNi_2Al_3 revealed by the ^<27>Al Knight shift measurement"Phys. Rev. Lett.. 89. 037002-1-037002-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyama, T.Nishioka, N.K.Sato: "Crystal field effect on specific heat and magnetization of PrPd_2Al_3"J. Phys. Soc. Jpn.. 71. 1609-1610 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N.K.Sato: "Magnetism and superconductivity in UT_2Al_3 (T=Pd, Ni) and UGe_2"Physica C (Proceedings of LT23, Hiroshima, 2002). (印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyaina, T.Nishioka, N.K.Sato: "Observation of phase transition between hidden and antiferromagnetic order in URu_2Si_2"Phys. Rev. Lett.. (印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Miyake and N.K.Sato: "Unconventional Cooper pairing in the superconducting state of UPd_2Al_3"Phys.Rev.B. 63. 052508 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N.K.Sato: "Strong coupling between local moments and superconducting 'heavy' electrons in UPd_2Al_3"Nature. 410. 340-343 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A.Hiess, N.K.Sato: "Spherical neutron polarimetry of the magnetic structure in UNi_2Al_3"Phys.Rev.B. 64. 134413-1-4 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] J.S.Kim, N.K.Sato and G.R.Stewart: "Specific heat near H_<metamag>=18 T in UPd_2Al_3"J.Low Temp.Phys.. 124. 527-535 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyama, N.K.Sato: "Possible competitive coexistence of ferromagnetism and superconductivity in UGe_2"Phys.Rev.B. 65. 020510(R) (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakon, N.K.Sato: "Magnetization of UPd_2Al_3 in the ultra-low temperature and high magnetic fields"J.Magn.Magn.Mater.. 226-230. 75-76 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A.Hiess, N.K.Sato: "Neutron scattering study of the static and dynamic magnetic properties of UNi_2Al_3"J.Magn.Magn.Mater.. 226-230. 54-56 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyama, T.Nishioka and N.K.Sato: "Crystal field effect on specific heat and magnetization of PrPd_2Al_3"J.Phys.Soc.Jpn.. 71. 1609-1610 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Nishioka, N.K.Sato: "Unusual nature of ferromagnetism coexisting with superconductivity in UGe_2"Phys.Rev.Lett.. 88. 237203-1-4 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakon, N.K.Sato: "Magnetic phase diagram of UPd_2Al_3 in high magnetic fields"Jpn.J.Appl.Phys.. 41. 3673-3677 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Ishida, N.K.Sato: "Spin-triplet superconductivity in UNi_2Al_3 revealed by the <27>^Al Knight shift measurement"Phys.Rev.Lett. 89. 037002-1-4 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N.K.Sato: "Magnetism and superconductivity in UT_2Al_3(T=Pd, Ni) and UGe_2"to appear in LT23 Proceedings, Hiroshima. in press. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Nakane, N.K.Sato: "AC magnetic susceptibility measurements on UGe_2"to appear in LT23 Proceedings, Hiroshima. in press. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Ushida, N.K.Sato: "Thermal expansion measurement under pressure of UGe_2"to appear in LT23 Proceedings, Hiroshima. in press. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyama, N.K.Sato: "Magnetic and superconducting properties under high pressure in URu_2Si_2"to appear in LT23 Proceedings, Hiroshima. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N.K.Sato: "Correlation between superconductivity and magnetism in uranium heavy fermion compounds"to appear in Proceedings of ASR-2002, Tokai. in press. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] G.Motoyama, T.Nishioka, N.K.Sato: "Observation of phase transition between hidden and antiferromagnetic order in URu_2Si_2"to appear in Phys.Rev.Lett.. in press.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Nishioka, G.Motoyama, S.Nakamura H.Kadoya, N.K.Sato: "Unusual nature of ferromagnetism coexisting with superconductivity in UGe_2"Phys. Rev. Lett.. 88. 237203-1-237203-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakon, N.K.Sato, Y.Nakanishi, T.Komatsubara, M.Motokawa: "Magnetic phase diagram of UPd_2Al_3 in high magnetic fields"Jpn. J. Appi. Phys.. 41. 3673-3677 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Ishida, N.K.Sato, N.Aso, C.Geibel, F.Steglich 他: "Spin-triplet superconductivity in UNi_2Al_3 revealed by the ^<27>Al Knight shift measurement"Phys. Rev. Lett.. 89. 037002-1-037002-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] G.Motoyama, T.Nishioka, N.K.Sato: "Crystal field effect on specific heat and magnetization of PrPd_2Al_3"J. Phys. Soc. Jpn.. 71. 1609-1610 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] N.K.Sato: "Magnetism and superconductivity in UT_2Al_3(T=Pd, Ni) and UGe_2"Physica C (Proceedings of LT23, Hiroshima, 2002). 534-553 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] G.Motoyatna, Y.Ushida, T.Nishioka, N.K.Sato: "Magnetic and superconducting properties under high pressure in URu_2Si_2"Physica B (Proceedings of LT23, Hiroshima, 2002). (印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] N.K.Sato, N.Aso, K.Miyake, R.Shiina, P.Thalmeier et al.: "Strong coupling between local moments and superconducting'heavy'electrons in UPd_2Al_3"Nature. 410. 340-343 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Miyake, N.K.Sato: "Unconventional Cooper pairing in the superconducting state of UPd_2Al_3"Phys. Rev. B. 63. 052508-1-2 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Hiess, P.J.Brown, E.Lelievre-Berna, N.Aso, N.K.Sato et al.: "Spherical neutron polarimetry of the magnetic structure in UNi_2Al_3"Phys. Rev. B. 64. 134413-1-4 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] J.S.Kim, N.K.Sato, G.R.Stewart: "Specific heat near H_<metamag>=18T in UPd_2Al_3"J.Low Temp. Phys.. 124. 527-535 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] G.Motoyama, S.Nakamura, H.Kadoya, T.Nishioka, N.K.Sato: "Possible competitive coexistence of ferromagnetism and superconductivity in UGe_2"Phys. Rev. B. 65. 020510(R) (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sakon, T.Namiki, N.K.Sato, T.Komatsubara, M.Motokawa: "Magnetization of UPd_2Al_3 in the ultra-low temperature and high magnetic fields"J. Magn. Magn. Mater.. 226-230. 75-76 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Nishioka et al.: "High pressure magnetization measurements on URu_2Si_2"J.Phys.Soc.Jpn.. 69. 2415-2418 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] F.Steglich et al.: "Unconventional normal-state properties and superconductivity in heavy-fermion metals"Physica C. 341-348. 691-694 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Miyake et al.: "Unconventional Cooper pairing in the superconducting state of UPd_2Al_3"Phys.Rev.B. 63(印刷中). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] N.K.Sato et al.: "Strong coupling between local moments and superconducting 'heavy' electrons in UPd_2Al_3"Nature. 3月15日号(印刷中). (2001)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2020-05-15  

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