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Manipulation of population transfer by stimulated emission process

Research Project

Project/Area Number 12640503
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionTokyo University of Science

Principal Investigator

KOICHI Tsukiyama  Department, of Chemistry. Tokyo University of Science Professor, 理学部・第一部, 教授 (20188519)

Project Period (FY) 2000 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2001: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2000: ¥2,100,000 (Direct Cost: ¥2,100,000)
KeywordsNO / CO / Amplified spontaneous emission / seed / Rydberg state
Research Abstract

Two techniques have been developed for control of cascade-type amplified spontaneous emission pathways in the NO Rydberg states. The first method, referred to as switching, is based on destruction of the population inversion required for amplification. The second method, called seeding, utilizes the injection of external field. The weak ASE radiation generated in a seeder cell travels collinearly with pump beams, acting as seeder light for the inverted medium in a main cell. By extracting desired seeder wavelengths with optical filtering, amplification of the selected electronic transition is realized. In addition, selective enhancement between the rotational transitions belonging to the same inter-Rydberg system is achieved by taking advantage of their different polarization properties. Finally, we demonstrated that the combined use of switching and seeding provided with rotational selectivity.
The effect of externally injected radiation on the two-photon laser induced amplified spontaneous emission (LI-ASE) has been investigated. The wave generated via the same LI-ASE process in a seeder cell acts as a seeder field for the inverted medium created in a main cell. A nearly tenfold gain is achieved in the B1Z+→A1II(0, 3) transition of the CO molecule. We demonstrate that the single rotational transition in the B1Z+→A1II(0, 4) band is selectively amplified by injection of laser radiation. This pump and seed arrangement facilitates detection of molecular spectra by simply tuning the seed laser frequency.

Report

(3 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • Research Products

    (21 results)

All Other

All Publications (21 results)

  • [Publications] Y.Ogi., et al.: "Laser induced amplified spontaneous emission from the 3d and of Rydberg states of NO"Chem. Phys.. 255. 379-395 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Ogi, K.Tsukiyama: "Seeded amplification of amplified spontaneus emission"J. Chem. Phys. 113. 1426-1433 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Tsukiyama, et al.: "The E^2S^+C^2π transtion of No"J. Mol. Spectrose.. 203. 65-74 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Sakoda, K.Tsukiyama: "Effect of externally ingected reiation on amplitied spontaneous emission in Co"Appl. Phys. B. 72. 411-415 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Ogi., et al.: "Polarization properties of laser induced amplified spontaneous emission from NO Rydberg states"Chem. Phys. 271. 215-225 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Kajimoto., et al.: "The infrared N^2Δ→K^2Π emission of No"J. Mol. Spectrosc. (in press). (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] ベムラパリ: "物理化学III"丸善. 71 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Ogi, M. Takahashi, K. Tsukiyama and R. Bersohn: "Laser induced amplified spontaneous emission from the3d and nf Rydberg states of NO"Chem.Phys. 255. 379-395 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Ogi, A. Sakoda and K. Tsukiyama: "Seeded amplification of amplified spontaneous emission in NO"J.Chem.Phys. 113. 1426-1433 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] V. B. Braun, K. P. Huber, M. Vervloet, C. Amiot, J. Verges and K. Tsukiyama: "The E 2」+->C 2n transition of NO, and term values for the A, D, E, and C lowest Rydberg levels"J.Mol.Spectrosc. 203. 65-74 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A. Sakoda, H. Mutoh and K. Tsukiyama: "Effect of externally injected radiation on amplified spontaneous emission in CO"Appl.Phys.B. 72. 411-415 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Ogi, A. Sakoda, H. Mutoh, H. Taki and K. Tsukiyama: "Polarization properties of laser induced amplified spontaneous emission from NO Rydberg states"Chem.Phys.. 271. 215-225 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Sato, D. Omiya, K. Tsukiyama, Y. Ogi and K. Soai: "Evidence of asymmetric autocatalysis in the enantioselective addition of diisopropylzinc to pyrimidine-5-carbaldehyde using chiral pyrimidyl alkanol"Tetrahedron : Asymm.. 12. 1965-1969 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Kajimoto, Y. Ogi and K. Tsukiyama: "The infrared N2A->K2n emission of NO"J.Mol.Spectrosc. (in press). (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Sakoda, H.Mutoh, K.Tsukiyama: "Effect of externally injected radiation on amplified spontaneous emission in CO"Appl.Phys.B. 72. 411-415 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Ogi, A.Sakoda, et al: "Polarization properties of laser induced amplitiod emission from NO Rydberg states"Chem.Phys.. 271. 215-225 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] I.Sato, D.Omiya, et al: "Evidence of asymmetric autocatalycis in the…"Tetrahedion:Asymm.. 12. 1965-1969 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] ベムラパリ: "物理化学III"丸善. 71 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Ogi et.al: "Laser induced amplified spontaneous-"Chem.Phys.. 255. 379-395 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Ogi et.al: "Seeded amplification of amplified-"J.Chem.Phys.. 113. 1426-1433 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] V.B,Braun et.al: "The E^2ε^+→C^2πtransition of No.-"J.Mol.Spectrosc.. 203. 65-74 (2000)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2016-04-21  

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