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Precise life-time measurements of unstable nuclides in capsulated in fullerene cage

Research Project

Project/Area Number 12640532
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic chemistry
Research InstitutionTohoku University

Principal Investigator

OHTSUKI Tsutomu  Graduate School of Science, Tohoku University, Associate Professor, 大学院・理学研究科, 助教授 (50233193)

Project Period (FY) 2000 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2001: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2000: ¥2,600,000 (Direct Cost: ¥2,600,000)
KeywordsFULLERENE / DECAY CONSTANT / Be-7 / 半減期 / 原子核反跳
Research Abstract

A precise measurement of decay constant for ^7Be encapsulated in fullerene cage were performed with extreme conditions, such as 6K temperature. The results measured in 6K were compared with data for the normal temperature and that presented so far in the different chemical forms.
^7Be atom can penetrate into the C_<60> to produce ^7Be@C_<60> by a recoil process of the nuclear reactions, ^<12>C(γ , α n)^7Be or ^7Li(p,n)^7Be. Radioactive endohedral fullerenes produced by the nuclear recoil, namely ^7B@C_<60>, were detected using radiochemical and radiochromatographic techniques in the final solution. To measure the decay constant of ^7Be encapsulated in the cage, ^7B@C_<60>, the same apparatus in a system (Ge-detector, MCA, Computer, etc.) was used. Furthermore, an automated sample-exchange system were installed in this term for the reduction of systematical errors. Data were collected at 8 hours intervals in the MCA system. Analysis was performed using by a least-squares fitting with the CERN program, PAW. Finally we obtained the life-time of 52.98±0.05 day for 6K and 51.97±0.05 for normal temperature, respectively. It seems that a relatively large change was obtained compared to the value resented so far.

Report

(3 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • Research Products

    (36 results)

All Other

All Publications (36 results)

  • [Publications] T.Ohtsuki et al.: "Systematic study of foreign-atom-doped fullerenes by using nuclear recoil method and their MD simulation"Journal of Chemical Physics. 112. 2834-2842 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Akiyama et al.: "Isolation and characterization of light actinide metallofullerene"Journal of American Chemical Society. 123. 181-182 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Formation of new materials in fullerenes by using nuclear recoil : Sb case"Scripta Materialia. 44. 1575-1578 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Formation of Sb-and Te-doped fullerenes by using a nuclear recoil and MD simulation"Physical Review B. 64. 1254021-1254025 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Shiga et al.: "Formation of N-doped C_<60> studied by ab initio molecular dynamics simulation"Material Transitions. 42. 2189-2193 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Se-atom incorporation in fullerene by using nuclear recoil and ab initio MD simulations"Physical Review B. 65. 0734021-0734024 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M.Ebihara et al.: "How effectively is the photon activation analysis applied to meteorite samples?"J. Radioanalitical and Nuclear Chemistry. 244. 491-496 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] J.Kasagi et al.: "Bremostrahlung in alpha-decay of ^<210>Po : Do alpha particles emit photons in tunneling?"Physical Review Letters. 85. 3062 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Ilievski et al.: "Multi-photon giant resonances and coulomb Assion of ^<238>V"Nuclear Physics. A687. 178-183 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "In corporation of Sb atom and fullerene by using nuclear recoil and their MD simulation"Transactions of Materials Research of Japan. 26. 1159-1162 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Clusters and Nanomaterials"Springer and Verlage. 340 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Nuclear and Radiochemical Approaches to fulleren Sieuces"Kluwer Academic Publisher. 136-157 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki et al.: "Systematic study of foreign-atom-doped fullerenes by using nuclear recoil method and their MD simulation"J. Chemical Physics. 112. 2834-2842 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Ebihara et al.: "How effectively is the photon activation analysis applied to meteorite samples?"J. Radioanal. Nucl. Chem.. 244. 491-496 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] J. Kasagi et al.: "Bremsstrahlung in alpha-decay of 210Po: Do alpha particles emit photons in tunneling?"Phys. Rev. Lett.. 85. 3062 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Akiyama et al.: "Isolation and characterization of light actinide metallofullerene"J. Am. Chem. Soc.. 123. 181-182 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Ilievski, et al.: "Multi-phonon giant resonances and coulomb fission of 238U"Nucl. Phys. A. 687. 178-183c (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki et al.: "Formation of new materials in fullerenes by using nuclear recoil: Sb case"Scripta Materialia. 44. 1575-1578 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki, et al.: "Formation of Sb- and Te-doped fullerenes by using a nuclear recoil and MD simulation"Phys. Rev. B. 64. 125402-(1-5) (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Shiga et al.: "Formation of N-doped C60 studied by ab initio molecular dynamics simulations"Materials Transitions. 42. 2189-2193 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki, et al.: "Incorporation of Sb atom and fullerene by using nuclear recoil and their MD simulation"Trans. Mater. Res. Soc. of Japan. 26. 1159-1162 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki, et al.: "Se-atom incorporation in fullerene by using nuclear recoil and ab initio MD simulations"Phys. Rev. B. 65. 073402-(1-4) (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki, et al.: "The study of endohedral fullerenes and heterofullerenes by nuclear recoil and MD simulation"Nuclear and Radiochemical Approaches to Fullerene Sciences, Edited by T. Braun (Kluwer Academic Publisher). 136-157 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Ohtsuki, et al.: "Formation of foreign atom doped fullerenes"Clusters and Nanomaterials: Theory and Experiment, Eds. Y. Kawazoe, K. Ohno and T. Kondo (Springer and Verlag). 170-185 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Ohtsuki et al.: "Systematic study of foreign-atom-doped fullerenes by using nuclear recoil method and their MD simulation"Journal of Chemical Physics. 112. 2834-2842 (2000)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Akiyama et al.: "Isolation and characterization of light actinide metallofullerene"Journal of American Chemical Society. 123. 181-182 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Ohtsuki et al.: "Formation of new materials in fullerenes by using nuclear recoil : Ab case"Scripta Materialia. 44. 1575-1578 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Ohtsuki et al.: "Formation of Sb-and Te-doped fullerenes by using a nuclear recoil and MD simulation"Physical Review B. 64. 125402-(1-5) (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Shiga et al.: "Formation of N-doped C_<60> studied by ab initio molecular dynamics simulations"Materials Transitions. 42. 2189-2193 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Ohtsuki et al.: "Se-atom incorporation in fullerene by using nuclear recoil and Ab initio MD simulations"Physical Review B. 65. 073402-(1-4) (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Ohtsuki (共著): "Clusters and Nanomaterials"Springer. 340 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Ohtsuki et al.: "Systematic study of foreign-atom-doped fullerenes by using nuclear recoil method and their M.D simulation"Journal of Chemical Physics. 112. 2834-2842 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Akiyama et al.: "Isolation and characterization of light actinide metallo-fullerene"Journal of American Chemical Society. 123. 181-182 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Ohtsuki et al.: "Formation of new materials in fullerenes by using nuclear recoil : Sb case."Scripta Materialia. (in press).

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Ohtsuki,K.Ohno: "Nuclear and Radiochemical Approaches to Fullerene Sciences"T.Braun,Kluwer Academic Publisher. 22 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Ohtsuki,K.Ohno: "Physics and Chemistry of Clusters"Y.Kawazoe,Springer and Verlage(in press). (2001)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2016-04-21  

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