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Study on basic characteristics of hollow filament polyimide membrane in tritium separation and its application to tritium monitors

Research Project

Project/Area Number 12680513
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionHigh Energy Accelerator Researcgh Organization(KEK)

Principal Investigator

SASAKI Shinichi  KEK, Radiatoin Science Center, Associate Professor, 放射線科学センター, 助教授 (80178649)

Co-Investigator(Kenkyū-buntansha) SUZUKI Takenori  KEK, Radiatoin Science Center, Professor, 放射線科学センター, 教授 (40162961)
OKUNO Kenji  Shizuoka Univ., Fac.of Science, Professor, 理学部, 教授 (80293596)
KONDO Knjiro  KEK, Applied Research Laboratory, professor, 共通研究施設, 教授 (20004434)
OKI Yuichi  Kyoto University Research reactor Institute, Assistant Professor, 原子炉実験所, 助教授 (40204094)
NUMAJIRI Masaharu  KEK, Radiation Science Center, Instructor, 放射線科学センター, 助手 (20189385)
Project Period (FY) 2000 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥3,600,000 (Direct Cost: ¥3,600,000)
Fiscal Year 2001: ¥1,700,000 (Direct Cost: ¥1,700,000)
Fiscal Year 2000: ¥1,900,000 (Direct Cost: ¥1,900,000)
Keywordshollow-filament type membrane / tritium / polyimide / accelerator / environmental radioactivity / slack(gas) monitor / separation and enrichment / radiation monitoring system / 電離箱
Research Abstract

In order to establish monitoring method of tritium in air released from accelerator beam-line tunnels through the stacks, a new real-time continuous gas monitoring system using a follow-filament polyimide membrane as a gas-separation device, has been proposed and basic gas-separation characteristics of membranes have been investigated experimentally in this study. Especially, the separation characteristics of hydrogen isotopes in nitrogen and water in dry-air were measured extensively, and a computer simulation using the simplified cross-flow model for the gas separation was also performed. The result showed that the polyimide membrane module could enrich significantly hydrogen isotopes and water vapor from nitrogen and dry air, and there were not observed remarkable isotope effects in separation characteristics between hydrogen isotopes (H2 and D2). It can be concluded from these results that the membrane is useful for the real time tritium monitoring. A conceptual design of a tritium monitoring system in also proposed. The results obtained in this study were presented at the several international conferences/meetings and were published in the journals.

Report

(3 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • Research Products

    (17 results)

All Other

All Publications (17 results)

  • [Publications] 赤堀 誠至: "中空糸高分子膜を用いたトリチウムの濃縮について(2)"Proceedings of the Second Workshop on Environmental Radioactivity. KEK Proceedings 2001-14. 67-71 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Shinichi Sasaki: "Basic characteristics of hollow-filament polyimide membrane in gas separation and application to tritium monitors"Journal of Radioanalytical and Nuclear Chemistry. (To be published).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Eriko Tega: "STUDY ON SELECTIVE SEPARATION OF TRITIUM USING A HOLLOW-FILAMENT TYPE POLYIMlDE MEMBRANE MODULE-ITS APPLICATION TO TRITIUM MONTORING IN HIGH-ENERGY ACCELERATOR FACILITIES"Fusion Science and Technology. (To be published in Vol.41 No.3).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Shimada: "Development of Tritium Monitor Using Hollow Filament Polyimide Membrane"Proceedings of the 10th International Congress of the International Radiation Protection Association (IRPA-10). 4a248 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 佐々木慎一: "加速器環境のモニタリング"放射線. Vol.26,No.3. 11-22 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Sasaki, E. Tega, A. Shimada, S. Akabori, T. Suzuki, K. Okuno and K. Kondo: "Basic Characteristics of Hollow-filament Polyimide Membrane in Gas Separation and Application to Tritium Monitors"Journal of Radioanalytical and Nuclear Chemistr. to be published. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] E. Tega, S. Akabori, K. Okuon, S. Sasaki, T. Suzuki and K. Kondo: "Study on Selective Separation of Tritium Using a Hollowfilament Type Polyimide Membrane Module Its Applicaton ot Tritiumi Monitoring un Highenergy Accelerator Facilities"Fusioni Science Technology. to be published. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A. Shimada, Y. morimoto, K.Igucih, K.Okuno, S.Sasaki, T.Suzuki and K.Kondo: "Development of Tritium Monitor Using Hollow Filament Polyimide Membrane"Proceedings of the 10th International Cougress of the International radiation Protetction Association (IRPA-10). P-4a248. (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Shinichi Sasaki: "Radiation Monitoring around Accerator Facilities (in Japanese)"Ionizing Radinatoin. Vol.26, No.3. 11-22 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] A.Shimada, S.Akahori, t.Sugiyama, Y.Morimoto, K.Okuno, S.Sasaki, T.Suzuki and K.Kondo: "Tritium Enrichment Using Hollow Filament membrane (in Japanese)"KEK=Procceedings 2000, 13. 37-41 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Akahori, E.Tega, H.Kodama, K.Okuno, S.Sasaki, T.Suzuki and K.Kondo: "Tritum Enrichment Using Hollow Filament Membrane(in Japanese)"KEK-Proceedings 2001, 14. 67-71 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 赤堀誠至: "中空糸高分子膜を用いたトリチウムの濃縮について(2)"Proceedings of the Second Workshop on Environmental Radioactivity. KEK Proceedings 2001-14. 67-71 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] Shinichi Sasaki: "Basic characteristics of hollow-filament polyimide membrane in gas separation and application to tritium monitors"Jornal of Radioanalytical and Nuclear Chemistry. (To be published).

    • Related Report
      2001 Annual Research Report
  • [Publications] Eriko Tega: "STUDY ON SELECTIVE SEPARATION OF TRITIUM USING A HOLLOW-FILAMENT TYPE POLYIMIDE MEMBRANE MODULE ITS APPLICATION TO TRITIUM MONITORING IN HIGH-ENERGY ACCELERATOR FACILITIES"Fusion Science and Technology. (To be published)Vol.41No.3.

    • Related Report
      2001 Annual Research Report
  • [Publications] 島田亜佐子: "中空糸高分子膜を用いたトリチウムの濃縮について"KEK Proceedings. 2000-13. 37-41 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] 佐々木慎一: "加速器環境のモニタリング"放射線. Vol 26 No.3. 11-22 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Shimada: "Development of Tritium Monitor Using Hollow Filament Polyimide Membrane"Proceedings of 10th International Congress of The International Radiation Protection Association. P-4a248-1-5 (2000)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2025-11-20  

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