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Diffraction of electrons Auger-excited by metastable-atoms or ions at the topmost surface layers and its application to surface structural analysis

Research Project

Project/Area Number 13440098
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionKyushu Institute of Technology

Principal Investigator

NISHIGAKI Satoshi  Kyushu Institute of Technology, Dpt.of Engineering, Professor, 工学部, 教授 (60126943)

Co-Investigator(Kenkyū-buntansha) WATANABE Akihiko  Kyushu Institute of Technology, Dpt.of Engineering, Education Ass., 工学部, 教務職員 (80363406)
NAZAROV Vladimir  Kyushu Institute of Technology, Dpt.of Engineering, Ass.Professor, 工学部, 助教授 (70315167)
NAITOH Masamichi  Kyushu Institute of Technology, Dpt.of Engineering, Ass.Professor, 工学部, 助教授 (60264131)
YAMADA Kenji  Ishikawa National College of Technology, Lecturer, 講師 (50249778)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥10,200,000 (Direct Cost: ¥10,200,000)
Fiscal Year 2003: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 2002: ¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2001: ¥6,100,000 (Direct Cost: ¥6,100,000)
KeywordsMetastable do-excitation / Ion neutralization / Inter-atomic Auger transition / Surface electron spectroscopy / Surface atomic structure / Density response function / Surface plasmon / イオン中性子
Research Abstract

This research aims at developing a technique of surface structural analysis by utilizing the effect of diffraction of Auger electrons emitted by the impact of excited atoms or ions with the surface. Although our research is still short of this target, we have obtained many important results which contributes solving fundamental and practical problems in the electron transition processes between surfaces and excited atoms or ions.
(1) We investigated the secondary electron emission upon impact of excited atoms at low-work function surfaces and proposed a mechanism of electron excitation above E_F through decay of hot holes in the cascade of electron-hole pair creation.
(2) Metastable-induced electron spectroscopy has been applied to many surface systems, e.g., oxygen/Ni(110)=changes in the electronic states in the process of oxygen-induced structural change ; alkali/Si(100) promotion or poisoning effects by alkali metals on surface oxidation or nitridation.
(3) A new spectroscopy system has been constructed which measures projectile-velocity resolved electron spectra induced by metastable atoms or ions. Fast He*atoms reach positions rather close to the, surface, which perturbs effectively the surface electronic structure. With slow He* atoms, the spectra contains higher contribution of electrons due to Auger de-excitation channel.
(4) We proposed a variant of the quadratic response theory that remains valid near or at plasma frequency and demonstrated that the nonlinearity serves itself to restrict the amplitude of plasma oscillations, thus providing a mechanism of "nonlinear damping." We also related the cross section for the inelastic scattering of charges in solids in the 2nd Born approximation to the quadratic retarded density-response function, deriving by this a formula applicable to describe the electron and positron energy-loss spectroscopy.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (28 results)

All Other

All Publications (28 results)

  • [Publications] T.Ikari: "A metastable-induced electron spectroscopy study on the process of oxygen adsorption at a Ni(110) surface"Applied Surface Science. 212-213. 579-582 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov: "Nonlinear mechanism of plasmon damping in electron gas"Physical Review B. 66. 092301,1-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov: "Z^3 theory of quantum inelastic scattering of charges by solids"Physical Review B. 65. 094303,1-11 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nishigaki: "A metastable-induced electron spectroscopy study on the promotion of nitridatioh by oxygen/alkali pre-adsorbates at Si(100) surfaces"Nuclear Instruments and Methods in Physics Research B. 193. 460-465 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov: "Non-linear aspects of particle-solids interactions in 3 and 2 dimensions : New developments"Proc.5th Russia-Japan Seminar on Semiconductor Surfaces. 5. 37-47 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Yamada: "Sodium-assisted nitrogen adsorption on Si(001) surfaces at room temperature studied by metastable de-excitation spectroscopy"Surface Science. 507-510. 207-212 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov: "Inelastic low-energy electron diffraction at metal surfaces"Surface Science. 482-485. 640-647 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov: "Inelastic electron scattering at metal surfaces : the role of elastic scattering"Vacuum. 63. 151-155 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ikari, T.Kojima, K.Yamada, M.Naitoh, S.Nishigaki: "A metastable-induced electron spectroscopy study on the process of oxygen adsorption at a Ni(110) surface"Applied Surface Science. Vol.212-213. 579-582 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov, S.Nishigaki, T.Nagao: "Nonlinear mechanism of plasmon damping in electron gas"Physical Review B. Vol.66. 092301,1-092301,4 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov, S.Nishigaki: "Z^3 theory of quantum inelastic scattering of charges by solids"Physical Review B. Vol.65. 094303,1-094303,11 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nishigaki, T.Sugiman, T.Ikari, I.Yokoh, K.Yamada, M.Naitoh: "A metastable-induced electron spectroscopy study on the promotion of nitridation by oxygen/alkali pre-adsorbates at Si(100) surfaces"Nuclear Instruments and Methods in Physics Research B. Vol.193. 460-465 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov, S.Nishigaki, T.Nagao: "Non-linear aspects of particle-solids interactions in 3 and 2 dimensions : New developments"Proc.5th Russia-Japan Seminar on Semiconductor Surfaces. Vol.5. 37-47 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Yamada, T.Sugiman, T.Ikari, I.Yokoh, M.Naitoh, S.Nishigaki: "Sodium-assisted nitrogen adsorption on Si(001) surfaces at room temperature studied by metastable de-excitation spectroscopy"Surface Science. Vol.507-510. 207-212 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov, S.Nishigaki: "Inelastic low-energy electron diffraction at metal surfaces"Surface Science. Vol.482-485. 640-647 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] V.U.Nazarov, S.Nishigaki: "Inelastic electron scattering at metal surfaces : the role of elastic scattering"Vacuum. Vol.63. 151-155 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ikari: "A metastable-induced electron spectroscopy study on the process of oxygen adsorption at a Ni(110) surface"Applied Surface Science. 212-213. 579-582 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] V.U.Nazarov: "Z^3 theory of quantum inelastic scattering of charges by solids"Physical Review B. 65. 094303,1-094303,11 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Nishigaki: "A metastable-induced electron spectroscopy study on the promotion of nitridation by oxygen/alkali pre-adsorbates at Si(100) surfaces"Nuclear Instruments and Methods in Physics Research B. 193. 460-465 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Yamada: "Sodium-assisted nitrogen adsorption on Si(001) surfaces at room temperature studied by metastable de-excitation spectroscopy"Surface Science. 507-510. 207-212 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] V.U.Nazarov: "Inelastic low-energy electron diffraction at metal surfaces"Surface Science. 482-485. 640-647 (2001)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Ikari: "A metastable-induced electron spectroscopy study on the process of oxygen adsorption at a Ni(110) surface"Applied Surface Science. (in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] V.U.Nazarov: "Z^3 theory of quantum inelastic scattering of charges by solids"Physical Review B. 65. 094303-1-094303-11 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Nishigaki: "A metastable-induced electron spectroscopy study on the promotion of nitridation by oxygen/alkali pre-adsorbates at Si(100) surfaces"Nuclear Instruments and Methods in Physics Research B. 193. 460-465 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Yamada: "Sodium-assisted nitrogen adsorption on Si(001) surfaces at room temperature studied by metastable de-excitation spectroscopy"Surface Science. 507-510. 207-212 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] V.U.Nazarov: "Inelastic low-energy electron diffraction at metal surfaces"Surface Science. 482-485. 640-647 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] V.U.Nazarov: "Z^3-order theory of quantum inelastic scattering of charges by solids"Physical Review B. 65. 094303 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Nishigaki: "A metastable-induced electron spectroscopy study on the promotion of nitridation by oxygen/alkali pre-adsorbates at Si(100)surfaces"Nuclear Instruments and Methods in Physics Research B. (in press). (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2021-04-07  

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