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Pioneering work of the mechanism elucidation of a new type ferromagnet Ca(La)B_6 by ESR.

Research Project

Project/Area Number 13440105
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTohoku University

Principal Investigator

KUNII Satoru  Tohoku University, Graduate School of Science, Professor, 大学院・理学研究科, 教授 (10004368)

Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥16,800,000 (Direct Cost: ¥16,800,000)
Fiscal Year 2003: ¥2,300,000 (Direct Cost: ¥2,300,000)
Fiscal Year 2002: ¥5,500,000 (Direct Cost: ¥5,500,000)
Fiscal Year 2001: ¥9,000,000 (Direct Cost: ¥9,000,000)
Keywordsnew type ferromagnet / Ca(La)B_6 / ESR
Research Abstract

The surprising paper of a new-type of ferromagnet Ca(La)B_6 was reported in "Nature" at February,2000. There were many theoretical papers appeared since then, but an experimental paper was not appeared. The reason was that the sample preparation was very difficult, because the melting point is very high (-2,500℃), and the liquid phase and the gas phase are co-existing. We are overcoming the above problems, we succeeded the single crystals of Ca(La)B_6 by Aluminum-flux method. We found out, first time, the ferromagnetism of Ca(La)B_6 in Japan. Moreover, we elucidate the mechanism of the ferromagnetism by electron spin resonance (ESR). That is, the spins owing to ferromagnetism are strongly forced to stay in the disk plane by an anisotropy field. We conclude that spins in Ca(La)B_6 exist only within the surface layer of approximately 1.5 μm thick, and they feel strong surface magnetic anisotropy of an easy plane type.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report

Research Products

(42 results)

All Other

All Publications (42 results)

  • [Publications] M.Akatsu: "Trigonal Lattice Distortion and Ferro Quadrupole Ordering in Phase IV of Ce_xLa_<1-x>B_6 (x=0.75 and 0.70)"J.Phys.Soc.Jpn.. 72. 205-208 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura: "Transport properties of the dense Kondo system Ce_<0.5>La_<0.5>B_6"Physica B. 329-333. 564-565 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Iwasa: "Newtron-diffraction study of the unusual ordered phases of Ce_<0.75>La_<0.25>B_6"Phisica B. 329-333. 582-583 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Akatsu: "Elastic properties of the Kondo compounds Ce_xLa_<1-x>B_6 (x=0.75 and 0.70)"Phisica B. 329-333. 626-627 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura: "Transport properties of the dense Kondo system Ce_<0.6>La_<0.5>B_6 at low temperature"J.Phys. : Condens.Matter. 15. S2167-S2170 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura: "Field-induced transition from non-Fermi-liquid state to heavy Fermion state in Ce_<0.5>La_<0.5>B_6"Phys.Rev.B. 68. 100402-1-100402-4 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Akatsu et al.: "Trigonal Lattice Distortion and Ferro-Quadrupole Ordering in Phase IV of Ce_xLa_<1-x>B_6(x=0.75 and 0.70)."J.Phys.Soc.Jpn.. 72. 205-208 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura et al.: "Transport properties of the dense Kondo system Ce_<0.5>La_<0.5>B_6."Physica B. 329-333. 564-565 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Iwasa et al.: "Neutron-diffraction study of the unusual ordered phases of Ce_<0.75>La_<0.25>B_6."Physica B. 329-333. 582-583 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Akatsu et al.: "Elastic properties of the Kondo compounds Ce_xLa_<1-x>B_6(x=0.75 and 0.70)."Physica B. 329-333. 626-627 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura et al.: "Transport properties of the dense Kondo system Ce_<0.5>La_<0.5>B_6 at low temperature."J.Phys.: Condens. Matter. 15. S2167-S2170 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Nakamura et al.: "Field-induced transition From non-Fermi-liquid state to heavy Fermion State in Ce_<0.5>La_<0.5>B_6."Phys.Rev. B. 68. 100402-1-100402-4 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Akatsu: "Trigonal Lattice Distortion and Ferro-Quadrupole Ordering in Phase IV of Ce_xLa_<1-x>B_6(x=0.75 and 0.70)"J.Phys.Soc.Jpn. 72. 205-208 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Nakamura: "Transport properties of the dense Kondo system Ce_<0.5>La<0.5>B_6"Physica B. 329-333. 564-565 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Iwasa: "Nerutron-differaction study of the unusual ordered phases of Ce_<0.75>La_<0.25>B_6"Physica B. 329-333. 582-583 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Akatsu: "Elastic properties of the Kondo compounds Ce_x La_<1-x>B_6 (x=0.75 and 0.70)"Physica B. 329-333. 626-627 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Nakamura: "Transport properties of the dense Kondo system Ce_<0.5>La_<0.5>B_6 at low temperature"J.Phys. : Condens.Matter. 15. S2167-S2170 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Nakamura: "Field-induced transition from non-Fermi-liquid state to heavy Fermion state in Ce_<0.5>La_<0.5>B_6"Phys.Rev.B. 68. 100402 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Takagiwa: "Magnetic Properties in Phase IV of Ce_<0.7>La_<0.3>B_6 Studied by Muon Spin Relaxation"J.Phys.Soc.Jpn.. 71・1. 31-34 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in Ce_xLa_<1-x>B_6"J.Phys.Soc.Jpn.. 71・Suppl.. 48-51 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Souma: "Angle-resolved photoemission spectroscopy of Ca_<1-x>La_xB_6"J.Phys.Soc.Jpn.. 71・Suppl.. 317-319 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Nemoto: "Low-temperature behavior of the elastic constant C_<44> in Ce_xLa_<1-x>B_6"Physica B. 312-313. 191-193 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Schenck: "Field-Induced Magnetization Distribution and Antiferroquadrupolar Order in CeB_6"Phys.Rev.Letters. 89・3. 37201-37205 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] N.Sluchanko: "Charge transport anisotropy in SmB_6"Physica B. 312・313. 331-332 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Magishi: "^<11>B NMR study of Ce_<0.75>La_<0.25>B_6"Physica B. 312・313. 189-190 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Udagawa: "Raman scattering investigation of high temperature ferromagnetic crystals"J.Phys.Soc.Jpn.. 71・Suppl.. 314-316 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Akatsu: "Thermal Expansion Measurements on Ce_<0.75>La_<0.25>B_6"J.Phys.Soc.Jpn.. 71・Suppl.. 115-117 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Nakamura: "Anisotropy in the Magnetic Phase Diagrams of Ce_xLa_<1-x>B_6"J.Phys.Soc.Jpn.. 71・Suppl.. 112-114 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kobayashi: "Hall effect of CeB_6 and Ce_xLa_<1-x>B_6"J.Phys.Soc.Jpn.. 71・Suppl.. 109-111 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Saitoh: "Where is the magnetic moment in CeB_6 ?"J.Phys.Soc.Jpn.. 71・Suppl.. 106-108 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Aoki: "Evolution of the Fermi surface of the strongly correlated f electron system under hydrostatic and uniaxial pressures"J.Phys.Condens.Matter. 14. 10705-10708 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Saitoh: "Anomalous Spin Density Distribution in CeB_6"J.Phys.Soc.Jpn.. 71・10. 2369-2372 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Nozawa: "Ultrahigh-resolution and angle-resolved potoemission study of SmB_6"J.Phys.Chem.Solids. 63・6-8. 1223-1226 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara: "Multipole ordering in f electron systems"J.Phys.Chem.Solids. 63. 1147-1153 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Magishi: "^<11>B NMR Study of Ce_xLa_<1-x>B_6"Z.Naturforsch. 57a. 441-446 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Souma: "Direct observation of pseudogap of SmB_6 using ultrahigh-resolution potoemission spectroscopy"Physica B. 312-313. 329-330 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Sera: "Anomalous Temperature Dependence of the Magnetic Field Induced Antiferromagnetic Moment in the Antiferroguadrupolar Orderd State of CeB_6"Phys. Rev. Letters. 86・8. 1578-1581 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Magnuson: "Electronic-structure investigation of CeB_6 By mesas of soft-x-ray scattering"Phys. Rev. B. 63・7. 75101-75105 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kobayashi: "Anisotropic Magnetic Phase Diagram of PrB_6 Dominated By the Oxy Antiferro-Quadrupalar Interaction"J. Phys. Soc. Jpn.. 70・6. 1721-1730 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] H.Nakao: "Antiferro-Quadrupole Ordering of CeB_6 Studied by Resonant X-Ray Scattering"J. Pluys. Soc. Jpn.. 70・7. 1857-1860 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.A.Granovsky: "Magnetic and magneto-elastic properties of a single crystal of TbB_6"J. Phys. Condens. Matten. 13・29. 6307-6321 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] N.E.Sluchauko: "Low-ternperature transport anisotropy and many-Body ettects in SmB_6"Phys. Rev. B. 64・15. 153103-153106 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2001-03-31   Modified: 2020-05-15  

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