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Study on strongly correlated electron systems by means of angle-resolved magnetization measurements at low temperatures

Research Project

Project/Area Number 13440106
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionThe University of Tokyo

Principal Investigator

SAKAKIBARA Toshiro  The University of Tokyo, Institute For Solid State Physics, Professor, 物性研究所, 教授 (70162287)

Co-Investigator(Kenkyū-buntansha) TAYAMA Takashi  The University of Tokyo, Institute For Solid State Physics, Research Associate, 物性研究所, 助手 (20334344)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥14,800,000 (Direct Cost: ¥14,800,000)
Fiscal Year 2003: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2002: ¥4,300,000 (Direct Cost: ¥4,300,000)
Fiscal Year 2001: ¥9,100,000 (Direct Cost: ¥9,100,000)
Keywordsquadrupole ordering / anisotropic quadrupole interaction / anisotropic superconductivity / gap symmetry / spin ice / skutterudite / magnetization measurement / specific heat measurement / 角度分解磁化測定 / 角度分解比熱測定 / 磁気熱量効果 / 反強四重極相図 / d波超伝導ギャップ構造 / スピンアイス化合物 / 気相液相型相転移 / エントロピー変化 / 気相液相転移 / 磁場誘起秩序状態 / 上部臨界磁場 / 不純物効果 / 非フェルミ液体的振舞い / 結晶場基底状態 / 残留状態密度 / 連続角度変化 / 常磁性効果 / メタ磁性転移
Research Abstract

1.We developed a new magnetometer that can rotate the field direction continuously at low temperatures below 0.5 K. Using this magnetometer, we examined the phase diagram of an antiferro-quadrupole ordering system PrPb3 and obtained the field-angle variation of the transition temperature. From the results, we could identify the order parameter, which requires the quadrupole interaction to be anisotropic.
2.We developed a new calorimeter that can rotate magnetic field direction continuously at low temperatures below 0.5 K. Using this calorimeter, we investigated the low temperature specific heat of the anisotropic superconductor CeCoIn5 in the superconducting mixed state. We observed a clear fourfold angular oscillation of the electronic specific heat, indicating d wave superconductivity. From the angular position of the minima in the specific heat, the d_xy type gap symmetry is concluded.
3.Magnetization process of a spin-ice compound Dy2Ti2O7 has been examined in a (111] magnetic field. We observed a clear magnetization plateau in the kagome ice state, followed by a first-order transition to a saturated sate. The transition is found to be of a liquid-gs type, which is new for the localized spin systems.
4.Field-temperature phase diagrams of the skutterudite compound PrOs4Sb12 has been examined at low temperatures and a field-induced ordering is observed for all the principal field directions. The results indicate the ground state of this system to be a Gamma_1 singlet.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (54 results)

All Other

All Publications (54 results)

  • [Publications] T.Tayama et al.: "Antiferro-quadrupolar ordering and multipole interactions in PrPb_3"J.Phys.Soc.Jpn.. 70. 248-258 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Unconventional Heavy-Fermion Superconductor CeCoIn_5 : Dc Magnetization Study at Very Low Temperature down to 50 mK"Phys.Rev.B. 65. 180504(R)-1-180504(R)-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Anomalous uniaxial pressure effect on the phase IV ordering in Ce_xLa_<1-x>B_6"J.Phys.Soc.Jpn.Suppl.. 71. 48-51 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Magnetic susceptibility of Ce0.75La0.25B6 under uniaxial pressure"Physica B. 312-313. 194-196 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Multipole ordering in f electron systems"J.Phys.Chem.Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Magnetization study of the heavy fermion superconductor CeCoIn_5"J.Phys.Chem.Solids. 63. 1155-1158 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "First-order superconducting transition at the upper critical field in CeCoIn_5 studied by DC magnetization measurement"Acta Physica Polonica B. 34. 467-470 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Harita et al.: "Measuring nuclear magnetization in strong magnetic fields"Physica B. 329-333. 1582-1585 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Quadrupole Ordering and Multipole Interactions in Pr-based Compounds"J.Phys : Condensed Matter. 15. S2055-S2061 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Magnetic phase diagram of the heavy fermion superconductor PrOs4Sb12"J.Phys.Soc.Jpn.. 72. 1516-1522 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Observation of a liquid-gas type transition in the pyrochlore spin ice compound Dy_2Ti_2O_7 in a magnetic field"Phys.Rev.Lett.. 90. 207205-1-207205-4 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Aoki et al.: "Field-angle dependence of the zero-energy density of states in the unconventional heavy-fermion superconductor Ce CoIn_5"J.Phys : Condensed Matter. 16. L13-L19 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Liquid-gas transition in the spin-ice dysprosium titanate"J.Mag.Mag.Matter.. (in press). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Antiferro-quadrupolar ordering and multipole interactions in PrPb_3"J.Phys.Soc.Jpn.. 70. 248-258 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Unconventional Heavy-Fermion Super-conductor CeCoIn_5: Dc Magnetization Study at Very Low Temperature down to 50 mK"Phys.Rev.B. 65. 180504(R)-1-180504(R)-4 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Anomalous uniaxial pressure effect on the phase IV ordering in Ce_xLa_<1 -x>B_6"J.Phys.Soc.Jpn.Suppl.. 71. 48-51 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Magnetic susceptibility of Ce0.75La0.25B6 under uniaxial pressure"Physica B. 312-313. 194-196 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Multipole ordering in f electron systems"J.Phys.Chem.Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Magnetization study of the heavy fermion superconductor CeCoIn_5"J.Phys.Chem.Solids. 63. 1155-1158 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "First-order superconducting transition at the upper critical field in CeCoIn_5 studied by DC magnetization measurement"Acta Physica Polonica B. 34. 467-470 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Harita et al.: "Measuring nuclear magnetization in strong magnetic fields"Physica B. 329-333. 1582-1585 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Quadrupole Ordering and Multipole Interactions in Pr-based Compounds"J.Phys : Condensed Matter. 15. S2055-S2061 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Tayama et al.: "Magnetic phase diagram of the heavy fermion superconductor PrOs4Sb12"J.Phys.Soc.Jpn.. 72. 1516-1522 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Observation of a liquid-gas type transition in the pyrochlore spin ice compound Dy_2Ti_2O_7 in a magnetic field"Phys.Rev.Lett.. 90. 207205-1-207205-4 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Aoki et al.: "Field-angle dependence of the zero-energy density of states in the unconventional heavy-fermion super-conductor CeCoIn_5"J.Phys : Condensed Matter. 16. L13-L19 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Liquid-gas transition in the spin-ice dysprosium titanate"J.Mag.Mag.Matter.. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakakibara et al.: "Quadrupole Ordering and Multipole Interactions in Pr-based Compounds"J.Phys.: Condens.Matter. 15. S2055-S2061 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Umeo et al.: "Field-induced magnetic transition in the heavy-fermion antiferromagnet Ce_7Ni_3"Phys.Rev.B. 67. 144408-1-144408-6 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Sakakibara et al.: "Observation of a liquid-gas type transition in the pyrochlore spin ice compound Dy_2Ti_2O_7 in a magnetic field"Phys.Rev.Lett.. 90. 207205-1-207205-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Y.Taguchi et al.: "Magnetic-field induced sign reversal of anomalous Hall effect in a pyrochlore ferromagnet Nd_2Mo_2O_7: evidence for spin chirality mechanism"Phys.Rev.Lett.. 90. 257202-1-257202-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.S.Kim et al.: "Anisotropic transport and magnetic properties of frustrated CeRhSn"Physica B. 329-333. 524-525 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.S.Kim et al.: "Low temperature anomalies in magnetic, transport, and thermal properties of single-crystal CeRhSn with valence fluctuations"Phys.Rev.B. 68. 054416-1-054416-7 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Umeo et al.: "The field-induced magnetic phase in a heavy-fermion antiferromagnet Ce_7Ni_3"J.Phys.: Condens.Matter. 15. S2159-S2162 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 榊原 俊郎: "PrOs_4Sb_<12>におけるエキゾチックな超伝導状態"日本物理学会誌. 58巻・12号. 887 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Aoki et al.: "Field-angle dependence of the zero-energy density of states in the unconventional heavy-fermion superconductor CeCoIn_5"J.Phys.: Condens.Matter. 16. L13-L19 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Tayama et al.: "Unconventional Heavy-Fermion Superconductor CeCoIn_5 : Dc Magnetization Study at Very Low Temperature down to 50 mK"Phys.Rev.B. 65. 180504(R)-1-180504(R)-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara et al.: "Anomalous uniaxial pressure effect on the phase IV ordering in Ce_xLa_<1-x>B_6"J.Phys.Soc.Jpn,. 71. Suppl.124-126 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara et al.: "Magnetic susceptibility of Ce_<0.75>La_<0.25>B_6 under uniaxial pressure"Physica B. 312-313. 194-196 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Amitsuka et al.: "Hidden order and weak antiferromagnetism in URu_2Si_2"Physica B. 312-313. 390-396 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara et al.: "Multipole ordering in felectron systems"J.Phys.Chem.Solids. 63. 1147-1153 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Amitsuka et al.: "Low temperature magnetization study on the non-Kramers cubic system Pr_3Pd_<20>Ge_6"J.Phys.Soc.Jpn.. 71. Suppl.124-126 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Tayama et al.: "Magnetization study of the heavy fermion superconductor CeCoIn_5"J.Phys.Chem.Solids. 63. 1155-1158 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Matsuhira et al.: "Low-temperature magnetic properties of pyrochlore stannates"J.Phys.Soc.Jpn.. 71. 1576-1582 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Matsuhira et al.: "A new macroscopically degenerate ground state in the spin ice compound Dy_2Ti_2O_7 under magnetic field"J.Phys.Condens.Matter. 14. L559-L565 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Yokoyama et al.: "Anomalous Fermi liquid behavior of the dilute uranium alloys La_<1-x>U_xRu_2Si_2,(x<0.07)"J.Phys.Soc.Jpn.. (印刷中).

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara et al.: "First-order superconducting transition at the upper critical field in CeCoIn_5 studied by DC magnetization measurement"Acta Physica Polonica B. (印刷中).

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Harita et al.: "Measuring nuclear magnetization in strong magnetic fields"Physica B. (印刷中).

    • Related Report
      2002 Annual Research Report
  • [Publications] Z.Hiroi et al.: "Specific Heat of Kagome's Ice in the Pyrochlore Oxide Dy_2Ti_<207>"J.Phys.Soc.Jpn.. 72. 411-418 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara: "Multipole Ordering In f electron systems"J. Phys. Chem. Solids. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sakakibara: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in Ce_xLa_<1-x>B_6"J. Phys. Soc. Jpn.. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sakakibara: "Magnetic susceptibility of Ce_<0.75>La_<0.25>B_6 under uniaxial pressure"Physica B. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Tayama: "Magnetization study of the heavy fermion superconductor CeCoIn_5"J. Phys. Chem. Solids. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Matsuhira: "Low temperature magnetic properties of frustrated pyrochlore ferromagnet Ho_2Sn_2O_7 and Ho_2Ti_2O_7"J. Phys. Condens. Matter. 12. L649-L656 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Matsuhira: "Novel dynamical magnetic properties in the spin ice compound Dy_2Ti_2O_7"J. Phys. Condens. Matter. 13. L737-L746 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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