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PHASE TRANSITION ASSOCIATED WITH CHIRAL SYMMETRY BREAKING

Research Project

Project/Area Number 13440115
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionKyushu University

Principal Investigator

AJIRO Yoshitami  KYUSHU UNIVERSITY, Faculty of Sciences, Prof., 大学院・理学研究院, 教授 (00025438)

Co-Investigator(Kenkyū-buntansha) KAWAMURA Hikaru  KYUSHU UNIVERSITY, Faculty of Sciences, Prof., 大学院・理学研究科, 教授 (30153018)
ASANO Takayuki  KYUSHU UNIVERSITY, Faculty of Sciences, Res.Assoc., 大学院・理学研究院, 助手 (00301333)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥15,300,000 (Direct Cost: ¥15,300,000)
Fiscal Year 2003: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2002: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2001: ¥12,100,000 (Direct Cost: ¥12,100,000)
Keywordschiral symmetry / phase transition / spin symmetry / frustration / chiral glass / Josenhson junction / triangular lattice / universality
Research Abstract

Phase transitions and critical phenomena have been a central subject of condensed matter physics for many years. We performed a variety of experimental studies to verify new types of phase transitions associated with chiral symmetry breaking.
1.Chiral glass ordering in the YBCO ceramic superconductors
A new type of the ordered phase, a chiral glass(CG) phase, is predicted to appear in the high-T_c ceramic, which contains frustrated inter-grain Josephson junction networks. Aiming to detect the weak but finite internal fields produced by the freezed spontaneous chiral loop supercurrent in the CG phase, ZF-jμSR technique was applied. We succeeded in detecting an anomalous magnetic field in the superconducting state. At the present stage of analysis, however, the appearance of the weak field is not correlated with the occurrence of the predicted CG transition. The origin of this anomalous magnetic field is interesting but not clear at present.
2.Chiral spin order in the frustrated magnets
We synthesized a variety of frustrated magnetic systems such as 2D triangular lattice, 3D stacked triangular lattice, 1D chain with the competing interactions, and explored possible chiral spin order, in collaboration with many groups. We examined new technique to provide direct information on the chiral variable, including a possible application of the synchrotron X-ray diffraction to this problem.
3.Quantum spin dynamics in nanoscale molecular magnets
In nanoscale magnetic systems, quantum mechanical dynamics due to the discrete energy levels plays an important role. We studied molecular magnets, Fe12 and V15 with focusing on the determination of low-lying energy levels which have permanent importance in understanding their unique quantum magnetism.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (63 results)

All Other

All Publications (63 results)

  • [Publications] Y.Ajiro et al.: "Magnetism of 1D Quantum Ferrimagnets, A3Cu3(PO4)4 with A=Ca, Sr"J.Phys.Soc.Jpn.. 70. 186-188 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Koike et al.: "Neutron Scattering Study of the Field Induced Antiferromagnets Order and Magnetic Excitation in Linear Chain Haldane Compound"J.Phys.Soc.Jpn.. 70. 189-191 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon et al.: "Electron Spin Resonance Study of Cu Benzoate Using a 3He-4He Dilution Refrigerator"J.Phys.Soc.Jpn.. 70. 2259-2262 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Fukita et al.: "Trinuclear Cu(II)M(II)Cu(II) complexes of anoxamide/dioxime ligand and extension to a bimetallic magnetic compound"J.Chem.Soc., Dalton Trans.. 64-70 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Mekata et al.: "Quantum spin chain systems with singlet ground state, ACu2(PO4)2 (A=Sr and Ba)"J.Magn.Magn.Mater.. 226-230. 410-411 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Kimura et al.: "High-field ESR measurements on CsCoCl3"Physica B. 294-295. 60-63 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano et al.: "mSR Study of Cu Benzoate at Very Low Temperature"J.Phys.Soc.Jpn.. 71. 594-598 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano et al.: "Elementary Excitations in Quantum Antiferromagnetic Chains : Dyons, Spinon, and Breather"Mol.Cryst.Liq.Cryst.. 121-130. 379-386 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri et al.: "Non-linear excitations on a field induced gap of Cu benzoate - an ESR investigation"Solid State Physics (in Japanese). 37. 27-34 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.V.Sologubenko et al.: "Diffusive energy transport in the S=1 Haldane chain compound AgVP2S6"Phys.Rev.. B68. 0944321-0944326 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Ito et al.: "Pressure-induced stabilization of an intermediate phase in the triangular lattice antiferromagnet CsNiCl3"J.Phys.: Condens.Matter. 15. L681-L686 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Inagaki et al.: "High Field Magnetization Process in a Dodecanuclear Fe(III) Ring Cluster"J.Phys.Soc.Jpn.. 72. 1178-1183 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro: "ESR Experiments on Quantum Spin System"J.Phys.Soc.Jpn.. 72. 12-25 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Kimura et al.: "High field / high frequency ESR in Osaka University"J.Phys.Soc.Jpn.. 72. 99-108 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon et al.: "ESR measurements at ultra-low temperatures using a dilution refrigerator"J.Phys.Soc.Jpn.. 72. 140-144 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro et al.: "Random quantum chain system ; mixture of S=1/2 antiferromagnetic chains with uniform and alternating couplings"Physica B. 329-333. 1004-1005 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano et al.: "Effect of staggered field in S=1/2 antiferromagnet chain : copper pyrimidine"Physica B. 329-333. 1006-1007 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro et al.: "Magnetic properties of bond-alternating quantum spin chain system : (CH3)2NH2CuX3 (X=Cl,Br)"Physica B. 329-333. 1008-1009 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro et al.: "Quantum level structure of molecular magnets, Fe12 and V15"Physica B. 329-333. 1038-1039 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano et al.: "ESR study of sine-Gordon Excitation in S=1/2 antiferromagnetic chain : copper benzoate"Physica B. 329-333. 1213-1214 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Karaki et al.: "Magnetic ordering of quasi-1D S=1/2 Heisenberg antiferromagnetic Cu benzoate at sub-mk temperature"Physica B. 329-333. 1002-1003 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon et al.: "Electron spin resonance measurements at ultralow temperatures"Physica B. 329-333. 1629-1631 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro, T.Asano, K.Nakaya, M.Mekata, H.Ohoyama, Y.Yamaguchi, Y.Koike, Y.Mori, K.Kamishima, H.Aruga Katori, T.Goto: "Magnetism of 1D Quantum Ferrimagnets, A_3Cu_3(PO_4)_4 with A=Ca,Sr"J.Phys.Soc.Jpn.. 70. 186-188 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Koike, N.Metoki, Y.Mori, T.Asano, Y.Ajiro: "Neutron Scattering Study of the Field Induced Antiferromagnets Order and Magnetic Excitation in Linear Chain Haldane Compound"J.Phys.Soc.Jpn.. 70. 189-191 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, H.Nojiri, K.Koyama, T.Asano, Y.Ajiro, M.Motokawa: "Electron Spin Resonance Study of Cu Benzoate Using a ^3He-^4He Dilution Regrigerator"J.Phys.Soc.Jpn.. 70. 2259-2262 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Fukita, M.Ohba, T.Shiga, H.Okawa, Y.Ajiro: "Trinuclear Cu(II)M(II)Cu(II) complexes of anoxamide/dioxime ligand and extension to a bimetallic magnetic compound"J.Chem.Soc.(Dalton Trans). 64-70 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Mekata, T.Hanabata, K.Nakaya, Y.Ajiro: "Quantum spin chain systems with singlet ground state, ACu_2(PO_4)_2 (A=Sr and Ba)"J.Magn.Magn.Mater. 226-230. 410-411 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Kimura, S.Hirai, K.Kindo, H.Kikuchi, Y.Ajiro: "High-field ESR measurements on CsCoCl_3"Physiea B. 294-295. 60-63 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, H.Nojiri, W.Higemoto, A.Koda, R.Kadono, Y.Ajiro: "μSR Study of Cu Benzoate at Very Low Temperature-Existence or Nonexistence of Long Range Order in Coupled Chains-"J.Phys.Soc.Jpn.. 71. 594-598 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, H.Nojiri, Y.Inagaki, Y.Ajiro, L.P.Regnault, J.P.Boucher: "Elementary Excitations in Quantum Antiferromagnetic Chains : Dyons, Spinon, and Breathers"Mol.Cryst.Liq.Cryst.. 121-130. 379-386 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, T.Asano, Y.Ajiro, M.Motokawa: "Non-linear excitations on a field induced gap of Cu benaoate-an ESR investigation"Solid State Physics(in Japanese). 37. 27-34 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.V.Sologubenko, S.M.Kazakov, H.R.Ott, T.Asano, Y.Ajiro: "Diffusive energy transport in the S=1 Haldane chain compound AgVP_2S_6"Phys.Rev.. B68. 0944321-0944326 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Ito, T.Asaho, T.Kawae, Y.Ajiro, K.Takeda: "Pressure-induced stabilization of an intermediate phase in the triangular lattice antiferromagnet CsNiCl_3"J.Phys. : Condens.Matter. 15. L681-L686 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Inagaki, T.Asano, Y.Ajiro, Y.Narumi, K.Kindo, A.Cornia, D.Gatteschi: "High Field Magnetization Process in a Dodecanuclear Fe(III)Ring Cruste"J.Phys.Soc.Jpn.. 72. 1178-1183 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro: "ESR Experiments on Quantum Spin Systems"J.Phys.Soc.Jpn.. 72. 12-25 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Kimura, K.Kindo, Y.Narumi, M.Hagiwara, H.Kikuchi, Y.Ajiro: "High field/high frequency ESR in Osaka University"J.Phys.Soc.Jpn.. 72. 99-108 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, H.Nojiri, K.Koyama, T.Asano, Y.Ajiro, M.Motokawa: "ESR measurements at ultra-low temperatures using a dilution refrigerator"J.Phys.Soc.Jpn.. 72. 140-144 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro, T.Wakisaka, H.Itbh, K.Watanabe, H.Satoh, Y.Inagaki, T.Asano, M.Mito, K.Takeda, H.Mitamura, T.Goto: "Random quantum chain system ; mixture of S=1/2 antiferromagnetic chains with uniform and alternating couplings"Physiea B. 329-333. 1004-1005 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, D.Nomura, Y.Inagaki, Y.Ajiro, H.Nojiri, Y.Narumi, K.Kindo, T.Ishida, T.Nogami: "Effect of staggered field in S=1/2 antiferromagnet chain: cooper pyrimidine"Physiea B. 329-333. 1006-1007 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro, K.Takeo, Y.Inagaki, T.Asano, A.Shimogai, M.Miti, T.Kawae, K.Takeda, T.Sakon, H.Nojiri, M.Motokawa: "Magnetic properties of bond-alternating quantum spin chain system : (CH_3)_2NH_2CuX_3(X=Cl,Br)"Physiea B. 329-333. 1008-1009 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro, Y.Inagaki, H.Itdh, T.Asano, Y Narumi, K.Kindo, T.Sakjon, H.Nojiri, M.Motokawa, A.Cornia, D.Gatteschi, A.Muller, B.Barbara: "Quantum level structure of molecular magnets, Fel2 and V15"Physiea B. 329-333. 1038-1039 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, H.Nojiri, Y.Inagaki, T.Sakon, J.P.Boucher, Y.Ajiro, M.Motokawa: "ESR study of sine-Gordon excitation in S=1/2 antiferromagnetic chain : copper benzoate"Physiea B. 329-333. 1213-1214 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Karaki, R.Masutomi, M.Kubota, H.Ishimoto, T.Asano, Y.Ajiro: "Magnetic ordering of quasi-1D S=1/2 Heisenberg antiferromagnetic Cu benzoate at sub-mK temperature"Physiea B. 329-333. 1002-1003 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, K.Koyama, M.Motokawa, H.Nojiri, T.Asano, Y.Ajiro: "Electron spin resonance measurements at ultralow temperatures"Physiea B. 329-333. 1629-1631 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Ajiro: "ESR Experiments on Quantum Spin Systems"J. Phys. Soc. Jpn.. 72. 12-25 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Random quantum chain system : mixture of S=1/2 antiferromagnetic chains with uniform and alternating coupling"Physica B. 329-333. 1004-1005 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Asano et al.: "Effect of staggered field in S=1/2 antiferromagnet chain : copper pyrimidine"Physica B. 329-333. 1006-1007 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Magnetic properties of bond-alternating quantum spin chain system (CH_3)_2NH_2CuX_3 (X=C1, Br)"Physica B. 329-333. 1008-1009 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Magnetic level structure of molecular magnets, Fe12 and V15"Physica B. 329-333. 1038-1039 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Asano et al.: "ESR study of sine-Gordon excitation in S=1/2 antiferrormagnetic chain : copper benzoate"Physica B. 329-333. 1213-1214 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Asano et al.: "μSR Study of Cu Benzoate at Very Low Temperature--Existence or Nonexistence of Long Range Order in Coupled Chains--"J. Phys. Soc. Jpn.. 71. 594-598 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] J.P.Boucher et al.: "Elementary Excitations in Quantum Antiferromagnetic Chains : Dyons, Spinons and Breathers"Mol. Cryst. Liq. Cryst.. 379. 121-130 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 野尻裕之, 浅野貴行, 網代芳民, 本河光博: "1次元鎖の束Cu benzoateの磁気励起"固体物理. 37. 537-544 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Magnetic Properties of V15 Molecular Magnet"Physica B. (in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Randam Quantum Chain System : Mixture of S=1/2 Amtiferromagnetic Chains with Uniform and Alternating Couplings"Physica B. (in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Magnetic Properties of Bond-Alternating Quantum Spin Chain System : (CH3)2NH2CuX3(X=Cl,Br)"Physica B. (in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Ajiro, J.P.Boucher: "Quantum Properties of Low-Dimensional Antiferromagnets"Kyushu University Press. 204 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Ajiro et al.: "Magnetism of 1D Quantum Ferrimagnets, A3Cu3(PO4)4 with A=Ca, Sr"J. Phys. Soc. Jpn.. 70. 186-188 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Koike et al.: "Neutron Scattering Study of the Field Induced Antiferromagnets Order and Magnetic Excitation in Linear Chain Haldane Compound"J. Phys. Soc. Jpn.. 70. 189-191 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sakon et al.: "Electron Spin Resonance Study of Cu Benzoate Using a 3He-4He Dilution Regrigerator"J. Phys. Soc. Jpn.. 70. 2259-2262 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Fukita et al.: "Trinuclear Cu(II)M(II)Cu(II) complexes of an oxamide/dioxime ligand and extension to a bimetallic magnetic compound"J. Chem. Soc., Dalton Trans. 64-70 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Mekata et al.: "Quantum spin chain systems with singlet ground state, ACu2(PO4)2 (A=Sr and Ba)"J. Magn. Magn. Mater. 226-230. 410-411 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Asano et al.: "μSR Study of Cu Benzoate at Very Low Temperature --Existence or Nonexis tence of Long Range Order in Coupled Chains--"J. Phys. Soc. Jpn. 71. 594-598 (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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