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Development of wave-packet interference control with an attosecond accuracy and is application to quantum computing

Research Project

Project/Area Number 13440120
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 物理学一般
Research InstitutionTohoku University

Principal Investigator

OHMORI Kenji  Tohoku University, Institute of Multidisciplinary Research for Advanced Materials, Associate Professor., 多元物質科学研究所, 助教授 (10241580)

Co-Investigator(Kenkyū-buntansha) OKUNISHI Misaki  Tohoku University, Institute of Multidisciplinary Research for Advanced Materials, Research Assistant., 多元物質科学研究所, 助手 (80224161)
Project Period (FY) 2001 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥14,900,000 (Direct Cost: ¥14,900,000)
Fiscal Year 2002: ¥4,600,000 (Direct Cost: ¥4,600,000)
Fiscal Year 2001: ¥10,300,000 (Direct Cost: ¥10,300,000)
Keywordswave packet / attoseconds / quantum interference / coherent control / quantum information / quantum phase / molecule / quantum computer / 純粋状態
Research Abstract

Quantum phase manipulation of wave functions opens a novel technology through "coherent control" such as quantum computing and bond selective chemistry. One promising approach is to use coherent light to modulate a wave function with its optical phase. For example, irradiating a diatomic molecule with a femtosecond (fs) optical pulse, with bandwidth broad enough to cover several vibrational eigenstates, coherently superpose those eigenstates to yield a spatially localized wave function called a nuclear "wave packet (WP)" traveling back and forth along the bond axis. In the generalon of this WP, the phase of an optical field is imprinted on the WP as its quantum phase. Hence engineering the optical phase with an accuracy better than the optical cycle allows us to engineer the phase of the WP with the same accuracy.
We have developed the "attosecond phase modulator", by which we can manipulate the relative phase of two fs laser pulses with an accuracy of 7 attoseconds. This phased pair of fs laser pulses has been used to realize unprecedented high-resolution interference of two nuclear WP's moving in a single Hg-Ar molecule where its fringe contrast is almost 100 %, demonstrating a pure wave nature of heavy particles.
This high-resolution WP interference has been utilized to encode 9 typical trinary codes into a 3 tritquantum reglster assembled within a single molecule as nodal patterns of a WP. In principle it can be used for fhe storage of the phase information contained in an optical field. Moreover, by using this WP interference control, we have developed a high-precision phase shiffer operated on a qubitorqutrit composed of coherent superposition of two or three vibrational eigenstates within a single molecule. The present studies indicate a possibility of large-sale quantum computing using many vibrational eigenstates within a single molecule.

Report

(3 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • Research Products

    (20 results)

All Other

All Publications (20 results)

  • [Publications] E.I.Dashevskaya: "Energy dependence of the intramultiplet mixing cross section in Hg-N_2 collisions: conical intersection mechanism, indication at tunneling and interference"Phys. Chem. Chem. Phys.. 5. 1198-1204 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 大森賢治: "アト秒精度の量子波束エンジニアリング"応用物理. 71・2. 195-199 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Ohmori: "Development of attosecond optical-phase manipulation for the wave-packet engineering"J. Photochemistry & Photobiology A: Chemistry. 145. 17-21 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. 11. 284-286 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Ohmori: "Using optical collision to control the transition-region dynamics"Multiphoton Processes and Spectroscopy. 14. 80-96 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] E.Bichoutskaia: "Spectroscopy of quasimolicular optical transitions: Ca(4s^2 ^1S_0 【tautomer】 4s4p ^1P,4s3d ^1D_2)-He. The influence of radiation width"J. Phys. B: At. Mol. Opt. Phys.. 34. 2301-2312 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] E. I. Dashevskaya: "Energy of the intramultiplet mixing cross section in Hg-N_2 collisions: concial intersection mechanism, indication at tunneling and interference"Phys. Chem. Chem. Phys.. 5. 1198-1204 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Kenji Ohmori: "Attosecond Wave packet engineering"Oyobuturi. 71. 195-199 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K. Ohmori: "Development of attosecond optical-phase manipulation for the wave-packet engineering"J.Photochem. Photobiol. A: Chemistry. 145. 17-21 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K. Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. 11. 284-286 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Kenji Ohmori: "Using Optical Collision to Control the Transition-region Dynamics"Multiphoton processes and Spectroscopy. 14. 80-96 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] E. Bichoutskaia: "Spectroscopy of quasimolecular optical transitions:(4s^<21>So⇔4s4p^1P,4s3d^1D_2)-He. The influence of radiation width"J.Phys.B:At.M0L.Opt.Phys.. 34. 2301-2312 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] E.L.Dashevskaya, K.Ohmori: "Enegry dependence of the intramultiplet mixing cross seccion in Hg-N2 collisions ; Conical intersection mechanism, indication at tunneling and interference"Phys.Chem.Chem.Phys.. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] 大森賢治: "アト秒精度の量子波束エンジニアリング"応用物理. 71・2. 195-199 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 大森賢治: "アト秒精度の量子波束エンジニアリング"応用物理. 71・2. 195-199 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Ohmori: "Development of attosecond optical-phase manipulation for the wave-packet engineering"J. Photochemistry & Photobiology A : Chemistry. 145. 17-21 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. 11. 284-286 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Ohmori: "Using optical collision to control the transition-region dynamics'"Multiphoton Processes and Spectroscopy. 14. 80-96 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Sato: "Double-pulse manipulation of vibrational wave packets in HgAr van der Waals complex"Laser Control and Manipulation of Molecules. (印刷中).

    • Related Report
      2001 Annual Research Report
  • [Publications] E.Bichoutskaia: "Spectroscopy of quasimolecular optical transitions : Ca(4s^2^1S_0【tautomer】4s4p^1P,4s3d^1D_2)-He. The influence of radiation width"J. Phys. B : At. Mol. Opt. Phys. 34. 2301-2312 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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