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Convection and Diffusion of Supercritical Carbon Dioxide in High-Pressure Porous Media Filled with Water

Research Project

Project/Area Number 13450081
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thermal engineering
Research InstitutionTokyo Institute of Technology

Principal Investigator

HIRAI Shuichiro  Tokyo Institute of Technology, Recearch Center for Carbon Recycling and Energy, Professor, 炭素循環エネルギー研究センター, 教授 (10173204)

Co-Investigator(Kenkyū-buntansha) TSUSHIMA Shoji  Tokyo Institute of Technology, the Faculty of Engineering, Research Associate, 工学部, 助手 (30323794)
SUEKANE Tetsuya  Tokyo Institute of Technology, Recearch Center for Carbon Recycling and Energy, Professor, 炭素循環エネルギー研究センター, 助教授 (30262314)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥14,000,000 (Direct Cost: ¥14,000,000)
Fiscal Year 2003: ¥1,800,000 (Direct Cost: ¥1,800,000)
Fiscal Year 2002: ¥4,500,000 (Direct Cost: ¥4,500,000)
Fiscal Year 2001: ¥7,700,000 (Direct Cost: ¥7,700,000)
Keywordsgeological sequestration / carbon dioxide / porous media / MRI / LBM / 北中隔離
Research Abstract

This paper describes experimental and numerical research on two-phase flow of supercritical CO_2 and water in porous media under sequestration conditions. We used a magnetic resonance imaging technique to directly visualize the distribution of supereritical CO_2 injected into porous media containing water. in situ water saturation distributions in a Berea sandstone core and a packed bed of glass beads were successfully visualized under conditions that simulate those at 700 -1000-m depths in an aquifers at the depth in the range from 700m to 1000m. By applying the coreflood interpretation method to our saturation data, we could describe the local Darcy phase velocities as a function of saturation. Finally, the effect of buoyancy on displacement process and gravity dominated pure counter-current flow is discussed by comparing the data obtained at two conditions that model the aquifers at depths of 1000 m and 700 m. We found that buoyancy largely controls the pure counter-current flow in … More well permeable porous media for conditions at 700 and 1000-m depths. We had developed a numerical code, which simulates two-phase flow of supercritical C0_2 and water in porous media including the effect of interfacial tension, wettability, buoyancy, and viscosity ratio, by a lattice Boltzmann method. A present study shows that the wettability and interfacial tension affect the relative permeability to deviate from Darcy law at low body forces such as buoyancy. Therefore, the effect of wettability and interfacial tension on the relative permeability should be taken into account to estimate the long-term fate of sequestered C0_2 by large-scalp reservoir simulations. The relative permeability of C0_2 decreases with an increase of the capillary pressure of water, As a result, the capillary pressure could make the flow of C0_2 slower than that has estimated in former simulations. Since the effect of the capillary pressure is significant in cap-rocks, the deviation from Darcy law is vital to the leakage of C0_2 through the cap-rocks. Less

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (20 results)

All Other

All Publications (20 results)

  • [Publications] T.Suekane, et al.: "Behavior of supercritical CO_2 injected into porous media containing water"Energy. (印刷中). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane, et al.: "Experimental and Numerical Studies on an Immiscible Flow of Supercritical CO_2 and Water in Porous Media"Addendum to the Proceedings of GHGT6. Addendum. 5-10 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane, et al.: "CO_2 Sequestration in Aquifers - Experimental and Numerical Studies on Flow of Supercritical CO_2 in Porous Media"the 6th ASME-JSME Thermal Engineering Joint Conference. (CD-ROM). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 石井稔宏, 末包哲也, 津島将司, 平井秀一郎: "地中隔離における多孔質内の超臨界CO_2-水二相流動計測"第40回日本伝熱シンポジウム講演論文集. III. 785-786 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 塚本佳久, 末包哲也, 平井秀一郎: "格子ボルツマン法による超臨界CO_2-水の二相流数値解析"第40回日本伝熱シンポジウム講演論文集. II. 371-372 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 末包哲也, 石井稔宏, 津島将司, 平井秀一郎: "CO_2地中隔離における多孔質内二相流のMRI計測"2003年度熱工学コンファレンス講演論文集. 517-518 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekaiie, et al.: "Behavior of supercritical CO2 injected into porous media containing water"Energy,2004. (in print). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane, et al.: "Experimental and Numerical Studies on an Immiscible Flow of Supercritical CO2 and Water in Porous Media"Addendum to the Proceedings of GHGT6, Addendum. 5-10 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane, et al.: "CO2 Sequestration in Aquifers -Experimental and Numerical Studies on Flow of Supercritical CO2 in Porous Media"the 6th ASME-JSME Thermal Engineering Joint Conference, 2003. (CD-ROM). (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ishii et al.: "Underground sequestration -measurement of two-phase flow of supercritical C02 and water in Porous Media"40^<th> National Heat Transfer Symposium of Japan. Vol.3. 785-786 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Y.Tsukamoto et al.: "Numerical simulation on two-phase flow of supercritical C02 and water by lattice Boltzmann method"40^<th> National Heat Transfer Symposium of Japan. Vol.2. 371-372 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane et al.: "MRI measurement of two-phase flow in porous media for underground sequestration of C02"Proceedings of Thermal Engineering Conference'03. 517-518 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Suekane, et al.: "Behavior of supercritical CO_2 injected into porous media containing water"Energy. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Suekane, et al.: "Experimental and Numerical Studies on an Immiscible Flow of Supercritical CO_2 and Water in Porous Media"Addendum to the Proceedings of GHGT6. Addendum. 5-10 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Suekane, et al.: "CO_2 Sequestration in Aquifers - Experimental and Numerical Studies on Flow of Supercritical CO_2 in Porous Media"the 6th ASME-JSME Thermal Engineering Joint Conference. (CD-ROM). (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 石井稔宏, 末包哲也, 津島将司, 平井秀一郎: "地中隔離における多孔質内の超臨界CO_2-水二相流動計測"第40回日本伝熱シンポジウム講演論文集. III. 785-786 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 塚本佳久, 末包哲也, 平井秀一郎: "格子ボルツマン法による超臨界CO_2-水の二相流数値解析"第40回日本伝熱シンポジウム講演論文集. II. 371-372 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 末包哲也, 石井稔宏, 津島将司, 平井秀一郎: "CO_2地中隔離における多孔質内相流のMRI計測"2003年度熱工学コンファレンス講演論文集. 517-518 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 末包哲也, 岩谷聴, 平井秀一郎, 惣川真吾, 津島将司: "地下貯留における超臨界CO_2の多孔質内流動"第39回日本伝熱シンポジウム. Vol.I. 305-306 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Suekane, S.Soukawa, S.Iwatani, S.Tsushima, S.Hirai: "Behavior of Supercritical CO2 Injected into Porous Media Containing water"The 5th International Symposium on CO2 Fixation and Efficient Utilization of Energy (C&E 2002). 417-422 (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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