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Dynamics of structural phase transition studied by picosecond time-resolved X-ray diffraction

Research Project

Project/Area Number 13450265
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionTokyo Institute of Technology

Principal Investigator

KONDO Ken-ichi  Tokyo Institute of Technology, Materials and Structures Laboratory, Professor, 応用セラミックス研究所, 教授 (50111670)

Co-Investigator(Kenkyū-buntansha) HIRONAKA Yoichiro  Materials and Structures Laboratory, Research Associate, 応用セラミックス研究所, 助手 (20293061)
G.NAKAMURA Kazutaka  Materials and Structures Laboratory, Associate Professor, 応用セラミックス研究所, 助教授 (20302979)
Project Period (FY) 2001 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥14,400,000 (Direct Cost: ¥14,400,000)
Fiscal Year 2002: ¥6,100,000 (Direct Cost: ¥6,100,000)
Fiscal Year 2001: ¥8,300,000 (Direct Cost: ¥8,300,000)
Keywordstime-resolved X-ray diffraction / femtosecond laser / pulsed X-rays / pump and probe / dynamics / phase transition / レーザー吸収 / X線回折 / 時間分解測定 / シリコン / オージェ再結合 / プラズマ臨界密度 / 衝撃波
Research Abstract

We investigated dynamics of a phase transition, which is induced by impulsive excitation, using a picosecond time-resolved X-ray diffraction technique. The pulsed X-rays were generated by focusing femtosecond laser beams onto metal targets at 10^17 W/cm^2 in a vacuum chamber, and extracted from a Be window. The X-rays were directed to a sample and the diffracted X-rays were detected by the L-N_2 cooled X-ray charge-coupled device. Time-resolved measurements were performed using a pump and probe technique. A 300-ps laser beam was irradiated on the sample at power density of 3.3 GW/cm^2 for excitation. The sample used was a silicon crystal (Si(111)). The time-resolved X-ray diffraction was obtained every 50 ps of time interval with a time-resolution of 10 ps. Lattice deformation corresponds to laser heating and acoustic-phonon propagation, which followed by the energy transfer from an electronic system to a lattice system, was directly observed. In order to increase the X-ray intensity at the sample position, an X-ray focusing system was constructed using a Johansson curved crystal. The X-rays were focused at a spot size with a diameter of 100・m and 400-times higher intensity. The newly constructed X-ray diffraction system can observe approximately 4 degrees at the spot.

Report

(3 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • Research Products

    (15 results)

All Other

All Publications (15 results)

  • [Publications] H.Kishimura, A.Yazaki, Y.Hironaka, K.G.Nakamura, K.Kondo: "Lattice deformation of laser-irradiated silicon crystal studied by picosecond X-ray diffraction"Appl.Surf.Sci.. 207. 314-317 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Kishimura, A.Yazaki, H.Kawano, Y.Hironaka, K.G.Nakamura, K.Kondo: "Picosecond structural dynamics in photoexcited Si probed by time-resolved x-ray diffraction"J.Chem.Phys.. 117. 10239-10243 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.G.Nakamura, K.Wakabayashi, Y.Hironaka, K.Kondo: "Pump and probe measurements of shock compressed states"J.Phys. : Condens.Matter. 14. 10817-10820 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Hironaka, A.Yazaki, K.G.Nakamura, K.Kondo: "Picosecond X-ray diffraction from laser-irradiated crystals"Appl.Suf.Sci. 197-198. 189-293 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A.Yazaki, H.Kishimura, H.Kawano, Y.Hironaka, K.G.Nakamura, K.Kondo: "Picosecond time-resolved X-ray diffraction of a photo-excited silicon crystal"Jpn.J.Appl.Phys.. 41・3A. 1614-1615 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H. Kishimura, A. Yazaki, Y. Hironaka, K.G. Nakamura, and K. Kondo: "Lattice deformation of laser-irradiated silicon crystal studied by picosecond X-ray diffraction"Appl. Surf. Sci. 207. 314-317 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Kishimura, A.Yazaki. H.Kawano, Y.Hironaka K.G.Nakamura, K.Kondo: "Picosecond structural dynamics in photoexcited Si probed by time-resolved x-ray diffraction"J. Chem. Phys.. 117. 0239-10243 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.G. Nakamura, K.Wakabayashi, Y.Hironaka, K. Kondo: "Pump and probe measurements of shock compressed states"J. Phys. : Condens. Matter. 14. 10817-10820 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Hironaka, A.Yazaki, K.G.Nakamura, K. Kohdo: "Picosecond X-ray diffraction from laser-irradiated crystals"Appl. Surf. Sci. 197-198. 189-293 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A.Yazaki, H.Kishimura, H.Kawano, H. Hironaka, K.G. Nakamura, K.Kondo: "Picosecond time-resolved X-ray diffraction of a photo-excited silicon crystal"Jpn. J. Appl. Phys.. 41.3A.. 1614-1615 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Kishinrura, A.Yazaki, Y.Hironaka, K.G.Nakamura, K.Kondo: "Lattice deformation of laser-irradiated silicon crystal studied by picosecond X-ray diffraction"Appl.Surf.Sci.. 207. 314-317 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Kishimura, A.Yazaki, H.Kawano, Y.Hironaka, K.G.Nakamura, K.Kondo: "Picosecond structural dynamics in photoexcited Si probed by time-resolved x-ray diffraction"J.Chem.Phys.. 117. 10239-10243 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.G.Nakamura, K.Wakabayashi, Y.Hironaka, K.Kondo: "Pump and probe measurements of shock compressed states"J.Phys. : Condens Matter. 14. 10817-10820 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Hironaka, A.Yazaki, K.G.Nakamura, K.Kondo: "Picosecond X-ray diffraction from laser-irradiated crystals"Appl.Suf.Sci. 197-198. 189-293 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Yazaki, H.Kishimura, H.Kawano, Y.Hironaka, K.G.Nakamura, K.Kondo: "Picosecond time-resolved X-ray diffraction of a photo-excited silicon crystal"Jpn.J.Appl.Phys.. 41・3A. 1614-1615 (2002)

    • Related Report
      2002 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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