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Development of high precision THz-ESR system by using repealing pulsed magnetic fields

Research Project

Project/Area Number 13554011
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section展開研究
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionOKAYAMA UNIVERSITY

Principal Investigator

NOJIRI Hiroyuki  Okayama University, Faculty of Science, Professor, 理学部, 教授 (80189399)

Co-Investigator(Kenkyū-buntansha) MATSUDA Yasuhiro  Okayama University, Faculty of Science, Associate Professor, 理学部, 助教授 (10292757)
MINO Michinobu  Okayama University, Faculty of Science, Associate Professor, 理学部, 助教授 (30222326)
YAMAZAKI Hitoshi  Okayama University, Faculty of Science, Professor, 理学部, 教授 (40013495)
KOYAMA Keiichi  Tohoku University, Institute for Materials Research, Associate Professor, 金属材料研究所, 助教授 (70302205)
SAKON Takuo  Akita University, Faculty of Engineering and Resource Science, Associate Professor, 工学資源学部, 助教授 (80271964)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥14,100,000 (Direct Cost: ¥14,100,000)
Fiscal Year 2003: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2002: ¥4,500,000 (Direct Cost: ¥4,500,000)
Fiscal Year 2001: ¥8,200,000 (Direct Cost: ¥8,200,000)
KeywordsUltra-high magnetic fields / Extreme condition / ESR / Terahertz wave / Pulsed magnetic fields / 繰り返しパルス磁場 / 強磁場 / テラヘルツ / ナノ磁性体 / サブミリ波
Research Abstract

A high precision terahertz ESR system has been developed by using a repeating pulsed magnetic field. The system is capable of generating pulsed magnetic fields up to 30 T every two seconds. The drastic improvement of signal to noise ratio is achieved by the signal averaging technique. The ratio becomes at least 50 times higher than that of the conventional ESR spectrometer by using a single shot type pulse field. The maximum frequency up to 3 THz can be used and it is extremely higher than that of the commercial W-band ESR spectrometer. Moreover, the efficiency defined by the possible number of scans par unit time is much larger than that of ESR spectrometer using superconducting magnets. The typical resolution of the present system is 10 gauss in simple hardware averaging method. The resolution ca be improved to 1 gauss by using a software averaging by suing a peak picking process. Test experiments have been made on a ladder compound and a micro single crystal of nano-magnetic cluster. Even a very weak forbidden transition can be observed by present system. The present result leads to the application of a repeating pulsed magnetic field for various types of spectroscopy such as Raman scattering or X-ray spectroscopy for solid state.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] H.Nojiri: "High Frequency ESR on quantum spin systems by using single shot and repeating pulsed fields"EPR in 21<st> century : basics and applications to material, life and. 751-754 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, H.Tanaka, B.Kuriniawan, M.Motokawa: "The role of ESR in research of low dimensional antiferromagnet"Physica B. 329-333. 701-702 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, H.Nojiri, Y.Inagaki, T.Sakon, J-P Boucher, Y.Ajiro, M.Motokawa: "ESR study of sine-Gordon excitations in S=1/2 antiferromagnet chain : copper benzoate"Physica B. 329-333. 213-214 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, K.Koyama, M.Motokawa, H.Nojiri, T.Asano, Y.Ajiro: "Electron spin resonance measurement at ultralow temperatures"Physica B. 329-333. 1629-1631 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, M.Motokawa, K.Okuda, H.Kageyama, Y.Ueda, H.Tanaka: "THz-ESR system by suing single shot and repeating pulsed magnetic fields"J.Phys.Soc.Jpn.. 72.Suppl.B. 109-116 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Motokawa, H.Ohta, H.Nojiri: "The role of ESR in research of low dimensional antiferromagnet"J.Phys.Soc.Jpn.. 72.Suppl.B. 1-11 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, H.Nojiri, T.Asano, Y.Ajiro, M.Motokawa: "ESR measurement at ultra-low temperature using a dilution refrigerator"J.Phys.Soc.Jpn.. 72.Suppl.B. 140-144 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, T.Taniguchi, Y.Ajiro, A.M.Muller, B.Barbara: "Quantum dynamics of molecular magnets in ultra-fast sweeping magnetic Fields"Physica B. 346-347. 216-220 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Hachisuka, K.Awaga, T.Yokoyama, T.Kubo, T.Goto, H.Nojiri: "Structure and magnetic properties of single-molecule magnet Mn_<11>Cr : Magneization manipulation and internal field in the mixed crystals of Mn_<11>Cr and"Physical Review B. (in print). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri: "High Frequency ESR on quantum spin systems by using single shot and repeating pulsed fields"EPR in the 21_<ST> century : basics and applications to material, life and earth sciences. 751-754. 751-754 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, H.Tanaka, B.Kumiawan, M.Motokawa: "Coexistence of gables and gapped excitations in NH_4CuCl_3"Physica B. 329-333. 701-702 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Asano, H.Nojiri, Y.Inagaki, T.Sakon, J-P.: "ESR study of sine-Gordon excitations in S=1/2 antiferromagnet chain : copper benzoate"Physica B. 329-333. 1213-1214 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, K.Koyama, _M.Motokawa, H.Nojiri, T.Asano, Y.Aijro: "Electron spin resonance measurements at ultralow temperatures"Physica B. 329-333. 1213-1214 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, M.Motokawa, K.Okuda, H.Kageyama, Y.Ueda, H.Tanaka: "THz-ESR System by using Single Shot and Repeating Pulsed Magnetic Fields"J.Phys.Soc.Jpn.Suppl.. B 72. 109-116 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Motokawa, H.Ohta, H.Noiiri, S.Kimura: "The role of ESR in research of low-dimensional antiferromagnets"J.Phys.Soc.Jpn.Suppl.. B 72. 1-11 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Sakon, H.Nojiri, T.Asano, Y.Ajiro, M.Motokawa: "ESR measurement at ultra-low temperature using a dilution refrigerator"J.Phys.Soc.Jpn.Suppl.. B 72. 140-144 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Nojiri, T.Taniguchi, Y.Ajiro, A.M.Muller, B.Barbara: "Quantum dynamics of molecular magnets in ultra-fast sweeping magnetic Fields"Physics B. 346-347. 216-220 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Hachisuka, K.Awaga, T.Yokoyama, T.Kubo, T.Goto, H.Nojiri: "Structure and magnetic properties of single-molecule magnet Mn_<11>Cr : Magnetization manipulation and internal field in the mixed crystals of Mn_<11>Cr and Mn_<12>"Physical Review B. (in print). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Hachisuka, K.Awaga, T.Yokoyama, T.Kubo, T.Goto, H.Nojiri: "Structure and magnetic properties of single-molecule magnet Mn_<11>Cr : Magnetization manipulation and internal field in the mixed crystals of Mn_<11>Cr and Mn_<12>"Physical Review B. (in print). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Nojiri, T.Taniguchi, Y.Ajiro, A.M.Muller, B.Barbara: "Quantum dynamics of molecular magnets in ultra-fast sweeping magnetic Fields"Physica B. (in print). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Nojiri, M.Motokawa, K.Okuda, H.Kageyama, Y.Ueda, H.Tanaka: "THz-ESR system by suing single shot and repeating pulsed magnetic fields"J. Phys. Soc. Jpn.. 72.Suppl.B(in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Motokawa, H.Ohta, H.Nojiri: "The role of ESR in research of low dimensional antiferromagnet"J. Phys. Soc. Jpn.. 72.Suppl.B(in press). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Nojiri: "High frequency ESR on quantum spin systems by using single shot and repeating pulsed fields"Physica B (to be published). (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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