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Development of Radio-Active Waste Decontamination Process by Using Atmospheric Pressure Plasma and Its Safety Analysis.

Research Project

Project/Area Number 13558060
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section展開研究
Research Field Nuclear engineering
Research InstitutionTokyo Institute of Technology

Principal Investigator

SUZUKI Masaaki  Tokyo Institute of Technology, Graduate School of Science and Engineering, Professor, 大学院・理工学研究科, 教授 (70114874)

Co-Investigator(Kenkyū-buntansha) GOTO Takanobu  Tokyo Institute of Technology, Graduate School of Science and Engineering, Research Associate (~March,2002) (at the time), 大学院・理工学研究科, 助手 (60313342)
AKATSUKA Hiroshi  Tokyo Institute of Technology, Research Lab. For Nuclear Reactors, Associate Professor, 原子炉工学研究所, 助教授 (50231808)
SEKIGUCHI Hidetoshi  Tokyo Institute of Technology, Graduate School of Science and Engineering, Associate Professor, 大学院・理工学研究科, 助教授 (50226643)
TADENUMA Katsuyoshi  KAKEN Corporation, President, 代表取締役(研究職)
MORI Shinsuke  Tokyo Institute of Technology, Graduate School of Science and Engineering, Research Associate (May2002-), 大学院・理工学研究科, 助手 (80345389)
坂岸 公二  (株)アトックス, 主任技師・研究職
菱沼 克嘉  (株)化研, 代表取締役・研究職
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥13,500,000 (Direct Cost: ¥13,500,000)
Fiscal Year 2003: ¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2002: ¥4,000,000 (Direct Cost: ¥4,000,000)
Fiscal Year 2001: ¥6,500,000 (Direct Cost: ¥6,500,000)
Keywordsdecontamination / plasma decontamination / atmosphenic pressure plasma discharge / fluorination reaction / decontamination process safety / 大気圧パルス放電 / フッ素過反応 / 除線の安全性
Research Abstract

In this project, we have studied the following two subjects, which is required to make the plasma decontamination process, which we have suggested, practicable. (1)To demonstrate the plasma decontamination process by using practical atmospheric pressure plasma. (2)To develop the process safety assessment method and to assess its process safety.
In the former subject, we generated the atmospheric-pressure non-equilibrium plasma by using rare gases and CF_4/O_2 mixture and we carried out some experiments of removal of cobalt oxide film stained on the stainless steel plate surface. The atmospheric -pressure non-equilibrium plasma generated here had two operation modes, atmospheric pressure glow discharge and dielectric burner discharge, depending on its discharge conditions. The decontamination characteristics under each mode and various conditions were made clear. In the case of Mel CF_4/O_2 gas mixture plasma the fluorination reaction proceeds sufficiently at 180-200 degree C and almost of cobalt oxide was converted into its fluoride within 5 minutes. The fluoride could be flush out easily by water and it could indicate the possibility of practical use of this process.
In the latter subject, we made modeling of processes of fine particle generation and its growth, adding to the evaporation of metal, which takes place in the plasma process. And also we developed the numerical calculation code to simulate a series of process which appears in the plasma process. By using this code we calculated the characteristics of fine particles generated in the plasma process. By adding to its code a collecting process by various air filter, furthermore, we completed a series of the process for the estimation process estimate the amount of fine particles which were released into the environment without collecting. Consequently, we could develop a method to obtain information fo safety assessment of the plasma decontamination technique.

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (16 results)

All Other

All Publications (16 results)

  • [Publications] M.Suzuki et al.: "Microwave Plasma Decontamination of Radioactive Material Operated at Atmospheric Pressure"Proc.of 15th Intl.Symp.Plasma Chemistry (Orlean). 2. 623-628 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Yamamoto et al.: "Chracteristics of the Fine Particles Generated in Plasma Process"Proc.of 15th Intl.Symp.Plasma Chemistry (Orlean). 2. 405-410 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 鈴木正昭: "大気圧反応性プラズマの原子力分野への応用-除染技術を中心として-"高温学会誌. 28[3]. 107-112 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Yamamoto et al.: "Simulation of the Evaporation Phenomenon of Metals by the Lattice Boltzmann Method"J.Chem.Eng.Japan. 35[10]. 944-951 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] 鈴木正昭: "反応性マイクロ波プラズマによる廃棄物処理の研究"応用物理. 72[4]. 462-465 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Suzuki et al.: "Microwave Plasma Decontamination of Radioactive Material Operated at Atmospheric Pressure"Proc. of 15th Intl. Symp. Plasma Chemistiy (Orlean). vol.2. 405-410 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Yamamoto, M.Suzuki: "Chracteristics of the Fine Particles Generated in Plasma Process"Proc. of 15th Intl. Symp. Plasma Chemistiy (Orlean). vol.2. 405-410 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Suzuki: "Application of Atmospheric Pressure Reactive Plasma To Nuclear Engineering Field. (in Japanese)"Kouon-Gakkai-Shi. 28[3]. 107-112 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Yamamoto, M.Suzuki: "Simulation of the Evaporation Phenomenon of Metals by the Lattice Boltzmann Method."J. Chem. Eng. Japan. 35[10]. 944-951 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Suzuki: "Waste Treatment Process by Reactive Microwave Plasma"Ouyoubutsuri. 72[4]. 462-465 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Yamamoto, M.Suzuki: "Aerosol Particles Generated in a Plasma Process and Penetrations through an Airfilter"Proc. of 15th Intl. Symp. Plasma Chemistry Taormina. (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Suzuki, S.Mori: "Plasma Processes of Nuclear Waste Materials under Atmospheric Pressure"30th IEEE International Conference on Plasma Science. 7CA. 01-02 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Yamamoto, K.Matsubayashi, M.Suzuki: "Aerosol Particles Generated in a Plasma Process and Penetrations through an Airfilter"Proc.16th Intl.Symp.Plasma Chemistry (ISPC16), Taormina. 3. 562-567 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Yamamoto, M.Suzuki: "Simulation of the Evapolation Phenomenon of Metals by the Lattice Boltzmann"Journal of Chemical Engineering of Japan. 35[10]. 944-951 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Suzuki et al.: "Microwave plasma decontamination of radioactive material operated at atmospheric pressure"Proc. 15^<th> Intl. Symp. On Plasma Chemistry. 647-652 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Yamamoto, M.Suzuki: "Characteristics of the fine particles generated in plasma process"Proc. 15^<th> Intl. Symp. On Plasma Chemistry. 405-412 (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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