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PREPARATION AND DISTRIBUTION OF ENVIRONMENTAL STANDARD SAMPLES FOR URANIUM AND PLUTONIUM

Research Project

Project/Area Number 13558067
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section展開研究
Research Field 環境影響評価(含放射線生物学)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

SASAKI Takayuki  KYOTO UNIVERSITY, ASSOCIATE PROFESSOR, 工学研究科, 助教授 (60314291)

Co-Investigator(Kenkyū-buntansha) FUJII Toshiyuki  KYOTO UNIVERSITY, RESEARCH REACTOR INSTITUTE, ASSISTANT RESEARCHER, 原子炉実験所, 助手 (10314296)
KUBOTA Takumi  KYOTO UNIVERSITY, RESEARCH REACTOR INSTITUTE, ASSISTANT RESEARCHER, 原子炉実験所, 助手 (90335240)
吉田 善行  日本原子力研究所, 東海研究所物質科学研究部付, 研究主幹
工藤 章  京都大学, 原子炉実験所, 教授 (00281113)
松井 三郎  京都大学, 工学研究科, 教授 (90092808)
菅原 正孝  大阪産業大学, 工学部, 教授 (60026119)
Project Period (FY) 2001 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥6,900,000 (Direct Cost: ¥6,900,000)
Fiscal Year 2004: ¥1,200,000 (Direct Cost: ¥1,200,000)
Fiscal Year 2003: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2002: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2001: ¥2,600,000 (Direct Cost: ¥2,600,000)
KeywordsURANIUM / ENVIRONMENTAL SAMPLES / ISOTOPIC RATIO / PRE-CONCENTRATION / LICHEN / CROSS-CHECKING / 苔
Research Abstract

FOR THE PREPARATION OF ENVIRONMENTAL STANDARD SAMPLES OF URANIUM AND PLUTONIUM, THE SOIL AND THE LICHEN WERE COLLECTED AT THE SEVERAL POINTS IN JAPAN. IN ORDER TO KEEP SAMPLES STABLE FOR LONG TERM, THESE WERE DRIED AND GAMMA-RAY IRRADIATED APPROPRIATELY. THE ISOTOPIC RATIO OF URANIUM IN THE SAMPLE WAS MEASURED BY ICP-MS (INDUCTIVELY COUPLED PLASMA MASS SPECTROMETRY), TIMS(THERMAL IONIZATION MASS SPECTROMETRY) AND ALPHA-RAY SPECTROMETRY. BEFORE THE MEASUREMENT, THE URANIUM WAS CONCENTRATED BY LIQUID-LIQUID MICROEXTRACTION SYSTEM. THE EQUIPMENT IS COMPOSED OF THREE SIMPLE EXTRACTION CELLS FOR PHASE MIXING, PHASE SEPARATION, AND COLLECTION OF A SOLVENT. METAL SEPARATION CAN BE COMPLETED IN A SINGLE OPERATION LASTING ONLY A MINUTE, FROM SOLVENT EXTRACTION TO PREPARATION. THE EXTRACTABILITY IN THE LMES WAS COMPARABLE TO THAT OF TRADITIONAL METHODS, AND THE DEVELOPED METHOD WAS FEASIBLE FOR RAPID SEPARATION. IN ORDER TO CHECK THE PRECISION OF OUR ISOTOPIC DATA, SOME SAMPLES WERE SENT TO THE OTHER RESEARCH PARTIES, AND WERE CROSS-CHECKED. THE ISOTOPE RATIOS WERE GOOD AGREEMENT WITH OUR VALUES. THESE SAMPLES CAN BE APPLIED TO THE STANDARD SAMPLES AS THE BACKGROUND OF URANIUM ISOTOPE RATIO IN JAPAN.

Report

(5 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (23 results)

All 2005 2004 2003 2002 Other

All Journal Article (14 results) Publications (9 results)

  • [Journal Article] SEPARATION OF RADIONUCLIDES IN A MULTITRACER PREPARED BY THERMAL NEUTRON FISSION OF 235U2005

    • Author(s)
      S.SHIBATA, K.TAKAMIYA, T.ICHIHARA, T.SASAKI
    • Journal Title

      APPL.RADIAT.ISOTOPES 60

      Pages: 625-628

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Separation of Radionuclides in a Multitracer Prepared by Thermal Neutron Fission of 235U2004

    • Author(s)
      S.Shibata, K.Takamiya, T.Ichihara, T.Sasaki
    • Journal Title

      Appl.Radiat.Isotopes 60

      Pages: 625-628

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Liquid-Liquid Micro Batch Extraction System for Rapid Separation2003

    • Author(s)
      T.Sasaki, K.Takamiya
    • Journal Title

      Chemistry Letters 32

      Pages: 184-185

    • NAID

      10012814144

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Liquid-Liquid micro batch extraction system (LMES) for rapid mutual separation of fission products2003

    • Author(s)
      T.Sasaki, K.Takamiya, T.Ichihara, S.Shibata
    • Journal Title

      Analytica Chimica Acta 484

      Pages: 139-144

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Concentrations of 222Rn, its Short-lived Daughters and 212Pb and their Ratios under Complex Atmospheric Conditions and Topography2003

    • Author(s)
      T.Kataoka, T.Sasaki et al.
    • Journal Title

      Boundary-Layer Meteorology 107

      Pages: 219-249

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] LIQUID-LIQUID MICRO BATCH EXTRACTION SYSTEM FOR RAPID SEPARATION2003

    • Author(s)
      T.SASAKI, K.TAKAMIYA
    • Journal Title

      CHEMISTRY LETTERS 32

      Pages: 184-185

    • NAID

      10012814144

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] LIQUID-LIQUID MICRO BATCH EXTRACTION SYSTEM (LMES) FOR RAPID MUTUAL SEPARATION OF FISSION PRODUCTS2003

    • Author(s)
      T.SASAKI, K.TAKAMIYA, T.ICHIHARA, S.SHIBATA
    • Journal Title

      ANALYTICA CHIMICA ACTA 484

      Pages: 139-144

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] CONCENTRATIONS OF 222RN, ITS SHORT-LIVED DAUGHTERS AND 212PB AND THEIR RATIOS UNDER COMPLEX ATMOSPHERIC CONDITIONS AND TOPOGRAPHY2003

    • Author(s)
      T.KATAOKA, T.SASAKI et al.
    • Journal Title

      BOUNDARY-LAYER METEOROLOGY 107

      Pages: 219-249

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Interaction of neptunium with humic acid and anaerobic bacteria2002

    • Author(s)
      T.Kubota, T.Sasaki, O.Tochiyama, A.Kudo
    • Journal Title

      Journal of Nuclear Science and Technology S3

      Pages: 946-949

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Radionuclides Sorption to a Mixture of Anaerobic Bacteria in the Repository Environment2002

    • Author(s)
      T.Sasaki, T.Kubota, S.Mito, T.Kauri, A.Kubo
    • Journal Title

      Journal of Nuclear Science and Technology S3

      Pages: 954-957

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Measurement of Nagasaki Pu Global Transport Rates, Comparing with SO_2 from Historic Volcanic Eruptions2002

    • Author(s)
      A.Kubo, T.Kubota, J.Zheng, T.Sasaki, et al.
    • Journal Title

      Journal of Nuclear Science and Technology S3

      Pages: 537-543

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] INTERACTION OF NEPTUNIUM WITH HUMIC ACID AND ANAEROBIC BACTERIA2002

    • Author(s)
      T.KUBOTA, T.SASAKI, O.TOCHIYAMA, A.KUDO
    • Journal Title

      J.NUCLEAR SCIENCE AND TECHNOLOGY S3

      Pages: 946-949

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] RADIONUCLIDES SORPTION TO A MIXTURE OF ANAEROBIC BACTERIA IN THE REPOSITORY ENVIRONMENT2002

    • Author(s)
      T.SASAKI, T.KUBOTA, S.MITO, T.KAURI, A.KUDO
    • Journal Title

      J.NUCLEAR SCIENCE AND TECHNOLOGY S3

      Pages: 954-957

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] MEASUREMENT OF NAGASAKI PU GLOBAL TRANSPORT RATES, COMPARING WITH SO2 FROM HISTORIC VOLCANIC ERUPTIONS2002

    • Author(s)
      A.KUDO, T.KUBOTA, J.ZHENG, T.SASAKI, et al.
    • Journal Title

      J.NUCLEAR SCIENCE AND TECHNOLOGY S3

      Pages: 537-543

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] T.Sasaki, K.Takamiya, T.Ichihara, S.Shibata: "Liquid-liquid micro batch extraction system (LMES) for rapid mutual separation of fission products"Analytica Chimica Acta. 484. 139-144 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Kataoka, T.Sasaki, et al.: "Concentrations of 222Rn, its Short-lived Daughters and 212Pb and their Ratios under Complex Atmospheric Conditions and Topography"Boundary-Layer Meteorology. 107. 219-249 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Sasaki, I.Kubota, S.Mito, T.Kauri, A.Kudo: "Radionuclides Sorption to a Mixture of Anaerobic Bacteria in the Repository Environment"Journal of Nuclear Science and Technology. 3. 954-957 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Kubota, T.Sasaki, O.Tochiyama, A.Kudo: "Interaction of neptunium with humic acid and anaerobic bacteria"Journal of Nuclear Science and Technology. 3. 946-949 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Kudo, T.Kubota, J.Zheng, T.Sasaki et al.: "Measurement of Nagasaki Pu Global Transport Rates, Comparing with SO_2 from Historic Volcanic Eruption"Journal of Nuclear Science and Technology. 3. 537-543 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sasaki, K.Takamiya: "Liquid-Liquid Micro Batch Extraction System for Rapid Separation"Chemistry Letters. 32. 184-185 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.KUBOTA, T.Sasaki, O.Tochiyama, A.Kudo: "Interaction of neptunium with humic acid and anaerobic bacteria"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sasaki, T.Kubota, S.Mito, T.Kauri, A.Kudo: "Radionuclides Sorption to a Mixture of Anaerobic Bacteria in the Repository Environment"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Kudo, T.Kubota, J.Zheng, T.Sasaki, et al.: "Measurement of Nagasaki Pu Global Transport Rates, Comparing with SO_2 from Historic Volcanic Eruptions"Journal of Nuclear Science and Technology. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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