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Low-Dimensional Electronic Excitations in a Metallic Monolayer of Finite Area Adsorbed on a Semiconductor Surface

Research Project

Project/Area Number 13640315
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionIwate University

Principal Investigator

INAOKA Takeshi  Iwate University, Faculty of Engineering, Associate Professor, 工学部, 助教授 (40184709)

Co-Investigator(Kenkyū-buntansha) NAGAO Tadaaki  Tohoku University, Institute for Materials Research, Associate Professor, 金属材料研究所, 助教授 (40267456)
Project Period (FY) 2001 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2003: ¥1,000,000 (Direct Cost: ¥1,000,000)
Fiscal Year 2002: ¥1,000,000 (Direct Cost: ¥1,000,000)
Fiscal Year 2001: ¥1,000,000 (Direct Cost: ¥1,000,000)
KeywordsSemiconductor Surface / Metallic Monolayer / Low-Dimensional Electronic Excitation / Edge Plasmon / Area Plasmon / Energy Dispersion / Induced Electron-Density Distribution / Energy-Loss Intensity / 誘起電荷密度分布 / 2次元電子励起 / 2次元プラズモン / 交換・相関効果 / 固体表面電子分光
Research Abstract

The Si(111)-√<3>×√<3> -Ag surface can be formed by depositing one monolayer of Ag atoms on a Si(111)-7×7 surface, and the surface-state band at this surface provides an ideal two-dimensional conduction-electron system (2DES). This electron system is confined in each √<3> ×√<3>-Ag domain surrounded by atomic steps or out-of-phase boundaries. Electronic excitations in this 2DES involves some interesting characteristics, such as low dimensionality, quantum-size effects, and presence of both edge and area excitations.
First, we have investigated two-dimensional plasmons (PL's) in the metallic monolayer of infinite area. This investigation has shown that, owing to low dimensionality, the exchange-correlation effects begin to appear remarkably with an increase in PL wave number q, though the 2DES has a high effective density. Our calculation has given a virtually quantitative description of the experimental results of high-resolution electron energy-loss spectroscopy (HREELS).
Next, by means o … More f the local-density approximation, we have examined low-dimensional PL's in a 2DES restricted to a strip region with constant width D and infinite length. We have found a series of PL dispersion branches where the node number increases one by one with ascending energy. Here, the node number is specified from the distribution of the induced electron density δn across the strip. The 0-node and 1-node modes are edge PL's with different parity in the δn distribution. With a decrease in D, the 0-node modes evolve into one-dimensional PL's. Each higher-order mode with more than one node has a standing-wave pattern in its δn distribution in a smaller q region, which evolves into area PL's with an increase in q. In a mode with more nodes, the standing-wave pattern persists up to a larger q range. As the width D becomes larger, the energy separation between neighboring PL dispersion branches becomes smaller, and the evolution into the area PL's occurs at smaller q values. Our analysis in relation to HREELS has shown that loss peaks due to a series of PL dispersion branches should appear clearly in the energy-loss spectrum, and that the loss peaks should have observable intensity, if a probe electron follows a trajectory in the vicinity of the strip region. Less

Report

(4 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (34 results)

All 2004 2003 2002 2001 Other

All Journal Article (12 results) Book (2 results) Publications (20 results)

  • [Journal Article] Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface2004

    • Author(s)
      Takeshi INAOKA
    • Journal Title

      Journal of the Physical Society of Japan 73・8(印刷中)

    • NAID

      110001954957

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface2004

    • Author(s)
      Takeshi INAOKA
    • Journal Title

      Journal of the Physical Society of Japan 73-8(in press)

    • NAID

      110001954957

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Characteristics of Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface2003

    • Author(s)
      Takeshi INAOKA
    • Journal Title

      Physical Review B 68・4

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Characteristics of Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface2003

    • Author(s)
      Takeshi INAOKA
    • Journal Title

      Physical Review B 68-4

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Two-Dimensional Plasmon in a Metallic Monolayer on a Semiconductor Surface : Exchange-Correlation Effects2002

    • Author(s)
      T.INAOKA, T.NAGAO, S.HASEGAWA, T.HILDEBRANDT, M.HENZLER
    • Journal Title

      Physical Review B 66・24

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Evolution of Electron States at a Narrow-Gap Semiconductor Surface in an Accumulation-Layer Formation Process2002

    • Author(s)
      S.ABE, T.INAOKA, M.HASEGAWA
    • Journal Title

      Physical Review B 66・20

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Electronic Excitations in a Nonparabolic Conduction Band of an n-Type Narrow-Gap Semiconductor2002

    • Author(s)
      M.YAMAGUCHI, T.INAOKA, M.HASEGAWA
    • Journal Title

      Physical Review B 65・8

    • NAID

      110009719119

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Two-Dimensional Plasmon in a Metallic Monolayer on a Semiconductor Surface : Exchange-Correlation Effects2002

    • Author(s)
      Takeshi INAOKA, Tadaaki NAGAO, Shuji HASEGAWA, Torsten HILDEBRANDT, Martin HENZLER
    • Journal Title

      Physical Review B 66-24

      Pages: 245320-245320

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Evolution of Electron States at a Narrow-Gap Semiconductor Surface in an Accumulation-Layer Formation Process2002

    • Author(s)
      Shuma ABE, Takeshi INAOKA, Masayuki HASEGAWA
    • Journal Title

      Physical Review B 66-20

      Pages: 205309-205309

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Electronic Excitations in a Nonparabolic Conduction Band of an n-Type Narrow-Gap Semiconductor2002

    • Author(s)
      Mitsutaka YAMAGUCHI, Takeshi INAOKA, Masayuki HASEGAWA
    • Journal Title

      Physical Review B 65-8

      Pages: 85207-85207

    • NAID

      110009719119

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Dispersion and Damping of a Two-Dimensional Plasmon in a Metallic Surface-State Band2001

    • Author(s)
      T.NAGAO, T.HILDEBRANDT, M.HENZLER, S.HASEGAWA
    • Journal Title

      Physical Review Letters 86・25

      Pages: 5747-5750

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Journal Article] Dispersion and Damping of a Two-Dimensional Plasmon in a Metallic Surface-State Band2001

    • Author(s)
      Tadaaki NAGAO, Torsten HILDEBRANDT, Martin HENZLER, Shuji HASEGAWA
    • Journal Title

      Physical Review Letters 86-25

      Pages: 5747-5750

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Book] Size-Dependent Evolution of Conduction-Electron Excitations in Small Spherical Particles : in "Clusters and Nanomaterials"(eds, Y.KAWAZOE et al.)2002

    • Author(s)
      Takeshi INAOKA
    • Publisher
      Springer-Verlag
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Book] Size-Dependent Evolution of Conduction-Electron Excitations in Small Spherical Particles in "Clusters and Nanomaterials", (eds.Y.KAWAZOE et al.)2002

    • Author(s)
      Takeshi INAOKA
    • Publisher
      Springer-Verlag
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.INAOKA, T.NAGAO, S.HASEGAWA, T.HILDEBRANDT, M.HENZLER: "Two-Dimensional Plasmon in a Metallic Monolayer on a Semiconductor Surface : Exchange-Correlation Effects"Physical Review B. 66・24. 245320 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takeshi INAOKA: "Characteristics of Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface"Physical Review B. 68・4. 41301(R) (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takeshi INAOKA: "Low-Dimensional Plasmons in a Metallic Strip Monolayer on a Semiconductor Surface"Journal of the Physical Society of Japan. (発表予定). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.NAGAO, T.HILDEBRANDT, M.HENZLER, S.HASEGAWA: "Dispersion and Damping of a Two-Dimensional Plasmon in a Metallic Surface-State Band"Physical Review Letters. 86・25. 5747-5750 (2001)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.ABE, T.INAOKA, M.HASEGAWA: "Evolution of Electron States at a Narrow-Gap Semiconductor Surface in an Accumulation-Layer Formation Process"Physical Review B. 66・20. 205309 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.YAMAGUCHI, T.INAOKA, M.HASEGAWA: "Electronic Excitations in a Nonparabolic Conduction Band of an n-Type Narrow-Gap Semiconductor"Physical Review B. 65・8. 85207 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takeshi INAOKA: "Size-Dependent Evolution of Conduction-Electron Excitations in Small Spherical Particles : in"Clusters and Nanomaterials", eds. Y.KAWAZOE et al."Springer-Verlag. 323-339 (2002)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takeshi INAOKA: "Kinematic Analysis of a Dispersion Region Probed in Reflection Electron Energy-Loss Sectroscopy"Surface Science. 493・(1-3). 687-691 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] 稲岡 毅: "高分解能電子エネルギー損失分光におけるプローブ分散領域の運動学的解析"真空. 45・3. 200-203 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.INAOKA, T.NAGAO, S.HASEGAWA, T.HILDEBRANDT, M.HENZLER: "Two-dimensional plasmon in a metallic monolayer on a semiconductor surface : exchange-correlation effects"Physical Review B. 66・24. 205320(8) (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.NAGAO, T.HILDEBRANDT, M.HENZLER, S.HASEGAWA: "Dispersion and Damping of a Two-Dimensional Plasmon in a Metallic Surface-State Band"Physical Review Letters. 85・25. 5747-5750 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.ABE, T.INAOKA, M.HASEGAWA: "Evolution of electron states at a narrow-gap semiconductor surface in an accumulation-layer formation process"Physical Review B. 66・20. 205309(8) (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.YAMAGUCHI, T.INAOKA, M.HASEGAWA: "Electronic Excitations in a Nonparabolic Conduction Band of an n-Type Narrow-Gap Semiconductor"Physical Review B. 65・8. 85207(9) (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Takeshi INAOKA: "Size-Dependent Evolution of Conduction-Electron Excitations in Small Spherical Particles : in "Clusters and Nanomaterials", eds. Y. KAWAZOE et al."Springer-Verlag. 323-329 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Takeshi INAOKA: "Kinematic Analysis of a Dispersion Region Probed in Reflection Electron Energy-Loss Spectroscopy"Surface Science. 493・(1-3). 687-691 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 稲岡 毅: "高分解能電子エネルギー損失分光におけるプローブ分散領域の運動学的解析"真空. 45・3(印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.NAGAO, T.HILDEBRANDT, M.HENZLER, S.HASEGAWA: "Dispersion and Damping of a Two-Dimensional Plasmon in a Metallic Surface-State Band"Physical Review Letters. 86・25. 5747-5750 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.NAGAO, T.HILDEBRANDT, M.HENZLER, S.HASEGAWA: "Two-Dimensional Plasmon in a Surface-State Band"Surface Science. 493・(1-3). 680-686 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.YAMAGUCHI, T.INAOKA, M.HASEGAWA: "Electronic Excitations in a Nonparabolic Conduction Band of an n-Type Narrow-Gap Semiconductor"Physical Review B. 65・8. 85207-85215 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] Takeshi INAOKA: "Size-Dependent Evolution of Conduction-Electron Excitations in Small Spherical Particles : in "Clusters and Nanomaterials", eds. Y. KAWAZOE et al."Springer-Verlag. 323-339 (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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