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Kondo effect on Nucler Quadrupole Interaction

Research Project

Project/Area Number 13640351
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionThe University of Tokyo

Principal Investigator

KARAKI Yoshitomo  The University of Tokyo, The Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (30186027)

Project Period (FY) 2001 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2004: ¥100,000 (Direct Cost: ¥100,000)
Fiscal Year 2003: ¥400,000 (Direct Cost: ¥400,000)
Fiscal Year 2002: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 2001: ¥2,700,000 (Direct Cost: ¥2,700,000)
Keywordsnuclear quadrupole interaction / hyperfine enhanced nuclear magnet / Nuclear magnetic ordering / coexistence of nuclear ferromagnetism and superconductivity / PrPt5 / PrOs4Sb12 / P-wave superconductor / 自己誘起渦糸状態 / 時間反転対称性の破れ / 核四重極モーメント / 近藤効果 / PrPt_5 / 増加核磁性 / 増強核磁性 / 第二種超伝導 / インジュウム / LaIn3 / レニウム / 電気抵抗
Research Abstract

PrPt5 is a hyperfine enhanced nuclear magnet. By specific heat measurement, Nuclear magnetic ordering was observed at 2mK. Furthermore, we observed a strongly enhanced nuclear quadrupole interaction of about 6mK. Owing to the large nuclear quadrupole interaction, we can study the effect of nuclear quadrupole interaction on resistance at rather higher temperature range of mK. To our's surprise, PrPt5 with Pt impurity phase became superconductivity. Then, we study on the coexistence of nuclear ferromagnetism and type-II superconductivity in PrPt5 with Pt impurity phase. It exhibits superconductivity at Ts=213 mK in zero field and a remarkable suppression (but finite) of the upper critical field Hc2 below a ferromagnetic nuclear ordering temperature (Tc〜2 mK). The lower critical field Hc1(〜1mT) is suppressed to 0.5mT by the presence the ferromagnetic order. The spontaneous nuclear magnetization coexists with superconductivity of Type II at field lager than 1mT down to the lowest measured temperature of 0.2 mK. At zero field, we think that a Domain-like magnetic state discussed by M.L.Kulic, A.I.Buzdin and L.N.Bulaevskii co-exists with the Meissner state. However, In a single phase sample of PrPt5, a superconductivity was not observed. We do not know the reason. We also study P-wave superconductor and a hyperfine enhanced nuclear magnet PrOs4Sb12. But nuclear magnetic ordering was not observed down to 0.2 mK.

Report

(5 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • Research Products

    (16 results)

All 2005 2004 2003 2002 Other

All Journal Article (14 results) Publications (2 results)

  • [Journal Article] A Dinuclear Mn^<III>-Cu^<II> Single-Molecule Magnet2005

    • Author(s)
      H.Oshio, M.Nihei, A.Yoshida, H.Nojiri, M.Nakao, A.Yamaguchi, Y.Karaki, H.Ishimoto
    • Journal Title

      Chem.Eur.J. 11

      Pages: 843-848

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] A Dinuclear Mn^<III>-CU^<II> Singlet-Molecule Mganet2005

    • Author(s)
      H.Oshio, M.Nihei, A.Yoshida, H.Nojiri, M.Nakao, A.Yamaguchi, Y.Karaki, H.Ishimoto
    • Journal Title

      Chem.Eur.J. 11

      Pages: 843-848

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] A Dinuclear Mn^<111>-Cu^<111> Single Magnet2005

    • Author(s)
      H.Oshio, M.Nihei, A.Yoshida, H.Nojiri, M.Nakano, A.Yamaguchi, Y.Karaki, H.Ishimoto
    • Journal Title

      Chem.Eur.J 11

      Pages: 843-848

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Gapless Spin Liquid Behavior in Two-Dimensional Solid ^3H2004

    • Author(s)
      R.Masutomi, Y.Karaki, H.Ishimoto
    • Journal Title

      Phys.Rev.Lett. 92

      Pages: 25301-25304

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Direct nuclear demagnetization of two dimensional solid ^3He adsorbed on Graphit2004

    • Author(s)
      R.Masutomi, Y.Karaki, H.Ishimoto
    • Journal Title

      J.Low Temp.Phys. 134

      Pages: 49-54

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Gapless Spin Liquid Behavior in Two-Dimensional Solid ^3He2004

    • Author(s)
      R.Masutomi, Y.Karaki, H.Ishimoto
    • Journal Title

      Phys.Rev.Lett. 92

      Pages: 25301-25304

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Direct nuclear demagnetization of two dimensional solid ^3He adsorbed on Graphite2004

    • Author(s)
      R.Masutomi, Y.Karaki, H.Ishimoto
    • Journal Title

      J.Low Temp.Phys. 134

      Pages: 49-54

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Magnetic ordering of quasi-1D S=1/2 Heisenberg antiferromagnet Cu benzoate at sub-mK temperatures2003

    • Author(s)
      Y.Karaki, R.Masutomi, M.Kubota, H.Ishimoto, T.Asano, Y.Aji
    • Journal Title

      Physica B 329-333

      Pages: 1002-1003

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic ordering of quasi-1D S=1/2 Heisenberg antiferromagnet Cu benzoate at sub-mK temperatures2003

    • Author(s)
      Y.Karaki, R.Masutomi, M.Kubota, H.Ishimoto, T.Asano, Y.Ajiro
    • Journal Title

      Physica B 1002

      Pages: 329-333

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Ferromagnetic interaction and superconductivity of CeCu_2Si_22002

    • Author(s)
      M.Ishikawa, N.Takeda, P.Ahmet.Y.Karaki, H.Ishimoto, D.Huo, J.Sakurai
    • Journal Title

      J.Phys.Chem.Solid 63

      Pages: 1165-1168

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Low Temperature Magnetization of Two Dimensional 3He on Three Layers of HD Preplate Graphite2002

    • Author(s)
      R.Masutomi, Y.Karaki, H.Ishimoto
    • Journal Title

      J.Low Temp.Phys. 126

      Pages: 241-246

    • NAID

      110002047567

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Electrical resistivity of intermetallic compound PrInAg2 at ultra low temperatures2002

    • Author(s)
      H.Mitamura, Y.Karaki, R.Masutomi, N.Takeshita, A.Yamaguchi, Y.Uwatoko, T.Goto, H.Ishimoto, N.Mori
    • Journal Title

      J.Magn.Magn Mat 239

      Pages: 31-32

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Ferromagnetic interaction and superconductivity of COCu_2Si_22002

    • Author(s)
      M Ishikawa, N Takeda, P Ahmet, Y Karaki, H Ishimoto, D.Huo, J.Sakurai
    • Journal Title

      J.Phys.Chem.Solid 63

      Pages: 1165-1165

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Electrical resistivity of intermetallic compound PrInAg2 at ultra low temperatures2002

    • Author(s)
      Mitamura, Y.Karaki, R.Masutomi, N, Takeshita, A.Yamaguchi, Y.Uwatoko, T.Goto, H.Ishimoto, N.Mori
    • Journal Title

      J.Magn.Magn Mat. 239

      Pages: 31-32

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] R.Masutomi, Y.Karaki, H.Ishimoto: "Direct nuclear demagnetization of two dimensional solid He-3 adsorbed on Graphite"Physical Review Letters. 92. 025301-023501-4 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Y.Karaki, R.Masutomi, M.Kubota, H.Ishimoto, T.Asano, Y.Ajiro: "Magnetic ordering of quasi-1 D S=1/2 Heisenberg antiferromagnet Cu benzoate at sub-mK temperatures"PHYSICA B. 予定(to be published). (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2001-04-01   Modified: 2020-05-15  

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