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NEUTRON DIFFRACTION STUDIES OF TWO-DIMENSIONAL HIGH-ORDER MAGNETIC MODULATION IN RRru_2Si_2 (R: Tb, Dy)

Research Project

Project/Area Number 13640362
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

KAWANO Shinji  RESEARCH REACTOR INSTITUTE, KYOTO UNIVERSITY, ASSOCIATE PROFESSOR, 原子炉実験所, 助教授 (70027457)

Project Period (FY) 2001 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥3,200,000 (Direct Cost: ¥3,200,000)
Fiscal Year 2002: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2001: ¥2,300,000 (Direct Cost: ¥2,300,000)
KeywordsLONG-PERIOD MAGNETIC MODULATION / TWO-DIMENSIONAL MODULATION / FRUSTRATION / NEUTRON DIFFRACTIN / MAGNETIC SATELLITES / DyRu_2Si_2 / TbRu_2Si_2 / 中性子回析
Research Abstract

(1)DyRu_2Si_2
From pulsed-neutron diffraction measurements of single crystal DyRu_2Si_2, we have confirmed that at the high temperature phase the magnetic modulation is one-dimensional with Q=(2/9 0 0). On the other hand, at the intermediate temperature phase many magnetic satellites on low-symmetry lines as well as high-symmetry lines have been observed in the a^*-b^* reciprocal plane. This is the evidence for the modulation being not one-dimensional but two-dimensional. The distribution of the magnetic satellites is reproduced by a magnetic unit cell of 9a×9a×c, in which the corner and the body-centered Dy ions are effectively paramagnetic due to frustration. Furthermore, pulsed-neutron experiments under magnetic fields at the ISIS, we have made clear the magnetic modulation of the four metamagnetic phases at low temperatures .
(1) TbRu_2Si_2
From single crystal neutron diffraction studies of TbRu_2Si_2 at Risoe National Laboratory, Denmark we have confirmed that the magnetic modulation is one-dimensional with Q=(3/13 0 0), but established the modulation for the intermediate temperature phase (ITP) to be two-dimensional of the magnetic unit cell being 13a×13a×c, including two frustrated Tb ions at the corner and body-centered positions, similar to the modulation of DyRu_2Si_2. Furthermore, for the low temperature phase two domains of a domain with Q=(3/13 1/4 0) and the ITP domain slightly distorted monoclinically in the a-b plane coexist.

Report

(3 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report

Research Products

(41 results)

All Other

All Publications (41 results)

  • [Publications] 川野眞治, 小杉武史, 高橋美和子, 繁岡透, 岩田允夫: "希土類化合物TbRu_2Ge_2における2次元高次磁気構造のパルス中性子回折"京都大学原子炉実験所学術講演会報文集. 35. 124-129 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, T.Kosugi, N.Iwata: "Higher order 2D magnetic modulations in TbRu_2Ge_2 and DyRu_2Si_2"京都大学原子炉実験所学術講演会報文集. 36. 18-22 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 岩田允夫, 繁岡透, 川野眞治: "DyRu_2Si_2の二次元磁気構造"京都大学原子炉実験所学術講演会報文集. 36. 131-134 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, T.Kosugi, M.Takahashi, T.Shigeoka, N.Iwata: "Neutron diffraction studies of two-dimensional magnetic ordering in TbRu_2Ge_2 at low temperatures"J.Phys.Soc.Jpn.Suppl. A. 70. 209-211 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Long-period two-dimensionally magnetic modulations in TbRu_2Si_2 and TbRu_2Ge_2"Proceedings of Aperiodic Structures 2001,Krakow, Poland. 57-60 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in DyRu_2Si_2"Applied Phys. A. 74[Suppl.]. S646-S648 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, B.Lebech, T.Shigeoka, N.Iwata: "Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in TbRu_2Si_2"Applied Phys. A. 74[Suppl.]. S643-S645 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N.Iwata, K.Hattori, M.Kadota, M.Takahashi, S.Kawano, T.Shigeoka: "Two-dimensional high-order commensurate structure in DyRu_2Si_2"J.Magn.Magn.Mater.. 256. 189-194 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Shigeoka, N.Iwata, S.Kawano: "Re-entrant double-Q magnetic structure in HoRu_2Si_2"J.Phys.Soc.Jpn.Suppl. A. 70. 206-208 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Two-dimensional magnetic modulations in TbRu_2Si_2, TbRu_2Ge_2 and DyRu_2Si_2"Book of Abstracts of Satellite to the XIX Congress of the IUCr on Neutron and Synchrotron X-ray Scattering in Condensed-Matter Research. 29-31 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, T.Kosugi, N.Iwata: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering of Single Crystals, TbRu_2Ge_2 and DyRu_2Si_2"KENS REPORT-XIII. 74-77 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kawano, B.Lebech, T.Shigeoka, N.Iwata: "Neutron diffraction studies of the magnetic structures of TbRu_2Si_2"Physica B. 276-278. 572-573 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, T. Kosugi, M. Takahashi, T. Shigeoka, N. Iwata: "Pulsed-neutron investigations of two-dimensional magnetic modulation in TbRu_2Ge_2 (in Japanese)"Report of Scientific Meeting of Kyoto University Reseach Reactor Institute. 35. 124-129 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, M. Takahashi, T. Shigeoka, T. Kosugi, N. Iwata: "Higher-order 2D magnetic modulations in TbRu_2Ge_2 and DyRu_2Si_2"Report of Scientific Meeting of Kyoto University Research Reactor Institute. 36. 18-22 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N. Iwata, T. Shigeoka, S. Kawano: "Two-dimensional magnetic structure of DyRu_2Si_2 (in Japanese)"Report of Scientific Meeting of Kyoto University Research Reactor Institute. 36. 131-134 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, T. Kosugi, M. Takahashi, T. Shigeoka, N. Iwata: "Neutron diffraction studies of two-dimensional magnetic ordering in TbRu_2Ge_2 at low temperatures"J. Phys. Soc. Jpn.. 70 Suppl. A. 209-211 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. kwano, B. Lebech, M. Takahashi. T. Shigeoka N. Iwata, T. Kosugi: "Long-period two-dimensionally magnetic modulations in TbRu_2Si_2 and TbRu_2Ge_2"Proceedings of Aperiodic Structures 2001, Krakow, Poland. 57-60

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, M. Takahashi, T. Shigeoka, N. Iwata, T. Kosugi: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in DyRu_2Si_2"Applied Phys. A. 74[Suppl.]. s646-s648 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, B. Lebech, T. Shigeoka N. Iwata: "Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in TbRu_2Si_2"Applied Phys. A. 74 [Suppl.]. s643-s645 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N. Iwata, K. Hattori, M. Kadota, M. Takahashi, S. Kawano, T. Shigeoka: "Two-dimensional high-order commensurate structure in DyRu_2Si_2"J. Magn. Magn. Mater.. 256. 189-194 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Shigeoka, N. Iwata, S. Kawano: "Re-entrant double-Q magnetic structure in HoRu_2Si_2"J. Phys. Soc. Jpn.. 70 Suppl. A. 206-208 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, B. Lebech, M. Takahashi, T. Shigeoka, N. Iwata, T. Kosugi: "Two-dimensional magnetic modulations in TbRu_2Si_2, TbRu_2Ge_2 and DyRu_2Si_2"Bock of Abstracts of Satellite to the XIX Congress of the IUCr on Neutron and Synchrotron X-ray Scattering in Condensed-Matter Research. 29-31 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, M. Takahashi, T. Shigeoka, T. Kosugi, N. Iwata: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering of Single Crystals, TbRu_2Ge_2 and DyRu_2Si_2"KENS REPORT-XIII. 74-77 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kawano, B. Lebech, T. Shigeoka and N. Iwata: "Neutron diffraction studies of the magnetic structures of TbRu_2Si_2"Physica B. 276-278. 572-573 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 川野眞治, 小杉武史, 高橋美和子, 繁岡透, 岩田允夫: "希土類化合物TbRu_2Ge_2における2次元高次磁気構造のパルス中性子回折"京都大学原子炉実験所学術講演会報文集. 35. 124-129 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, T.Kosugi, N.Iwata: "Higher order 2D magnetic modulations in TbRu_2Ge_2 and DyRu_2Si_2"京都大学原子炉実験所学術講演会報文集. 36. 18-22 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 岩田允夫, 繁岡透, 川野眞治: "DyRu_2Si_2の二次元磁気構造"京都大学原子炉実験所学術講演会報文集. 36. 131-134 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, T.Kosugi, M.Takahashi, T.Shigeoka, N.Iwata: "Neutron diffraction studies of two-dimensional magnetic ordering in TbRu_2Ge_2 at low temperatures"J. Phys. Soc. Jpn. Suppl. A. 70. 209-211 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Long-period two-dimensionally magnetic modulations in TbRu_2Si_2 and TbRu_2Ge_2"Proceedings of Aperiodic Structures 2001, Krakow, Poland. 57-60 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in DyRu_2Si_2"Applied Phys. A. 74[Suppl.]. s646-s648 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, B.Lebech, T.Shigeoka, N.Iwata: "Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering in TbRu_2Si_2"Applied Phys. A. 74[Suppl.]. s643-s645 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] N.Iwata, K.Hattori, M.Kadota, M.Takahashi, S.Kawano, T.Shigeoka: "Two-dimensional high-order commensurate structure in DyRu_2Si_2"J. Magn. Magn. Mater.. 256. 189-194 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Shigeoka, N.Iwata, S.Kawano: "Reentrant double-Q magnetic structure in HoRu_2Si_2"J. Phys. Soc. Jpn. Suppl. A. 70. 206-208 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwata, T.Kosugi: "Two-dimensional magnetic modulations in TbRu_2Si_2, TbRu_2Ge_2 and DyRu_2Si_2"Book of Abstracts of Satellite to the XIX Congress of the IUCr on Neutron and Synchrotron X-ray Scattering in Condensed-Matter Research. 29-31 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, M.Takahashi T.Shigeoka, T.Kosugi, N.Iwata: "Pulsed-Neutron Diffraction Studies of Two-Dimensional Magnetic Ordering of Single Crystals, TbRu_2Ge_2 and Ru_2Si_2"KENS REPORT-XIII. 74-77 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kawano, B.Lebech, T.Shigeoka, N.Iwata: "Neutron diffraction studies ofthe magnetic structures of TbRu_2Si_2"Physica B. 276-278. 572-573 (2000)

    • Related Report
      2002 Annual Research Report
  • [Publications] 川野眞治, 小杉武史, 高橋美和子, 繁岡透, 岩田允夫: "希土類化合物TbRu_2Ge_2における2次元高次磁気構造のパルス中性子回折"京都大学原子炉実験所学術講演会報文集. 35. 124-129 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kawano, M.Takahashi, T.Shigeoka, T.Kosugi, N.Iwata: "Higher order 2D magnetic modulations in TbRu_2Ge_2 and DyRu_2Si_2"京都大学原子炉実験所学術講演会報文集. 36. 18-22 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] 岩田允夫, 繁岡透, 川野眞治: "DyRu_2Si_2の二次元磁気構造"京都大学原子炉実験所学術講演会報文集. 36. 131-134 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kawano, T.Kosugi, M.Takahashi, T.Shigeoka, N.Iwata: "Neutron diffraction studies of two-dimensional magnetic ordering in TbRu_2Ge_2 at low temperatures"J. Phys. Soc. Jpn. Suppl. A. 70. 209-211 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kawano, B.Lebech, M.Takahashi, T.Shigeoka, N.Iwala, T.Kosugi: "Long-period two-dimensionally magnetic modulations in TbRu_2Si_2 and TbRu_2Ge_2"Proceedings of Aperiodic Structures 2001, Krakow, Poland. 57-60 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2001-03-31   Modified: 2020-05-15  

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