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Diagnostics of Atmospheric-Pressure Non-thermal plasmas for Air Polluion Control using Laser-induced Fluorescence Spectroscopy

Research Project

Project/Area Number 13650313
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 電力工学・電気機器工学
Research InstitutionOita University

Principal Investigator

KANAZAWA Seiji  Oita University, Department of Electrical and Electronic Engineering, Associate Professor, 工学部, 助教授 (70224574)

Co-Investigator(Kenkyū-buntansha) OHKUBO Toshikazu  Oita University, Department of Electrical and Electronic Engineering, Associate Professor, 工学部, 教授 (00094061)
NOMOTO Yukiharu  Oita University, Department of Electrical and Electronic Engineering, Professor, 工学部, 教授 (90037953)
Project Period (FY) 2001 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2002: ¥900,000 (Direct Cost: ¥900,000)
KeywordsLIF / NOx / Streamer / Non-thermal plasma / Gaseous pollution control / Ionic wind / Environmental protecion technology / 非熱平衡プラズマ / 大気圧放電プラズマ / 反応器内NO分布
Research Abstract

Non-thermal plasma process has been considered to be an effective method to remove NOx from flue gas. In order to optimize the reactor and provide the information for numerical simulation of NOx removal, it is important to study directly the discharge induced plasma chemical processes responsible for NOx removal in the reactor. Laser-induced fluorescence (LIF) is a useful diagnostic method for in-situ observation of the phenomena during the NOx removal. The main objective of the presented work is visualization of two-dimensional NO concentration and monitoring the process of NOx removal inside the corona radical shower reactor. Planar laser induced fluorescence (PLIF) was employed for this purpose. The corona radical shower reactor consists of a nozzle-to-plate electrode system, having an electrode gap of 50mm. Stable dc streamer corona discharge was generated and laser pulses in the form of the sheet were shot between the electrodes during the discharge. LIF signal emitted at 90 degree to the laser sheet was imaged onto a gated ICCD camera and the two-dimensional LIF images from the various regions of the reactor were recorded. By the wide range imaging of NO (image size: 240mm in width and 160mm in height), two-dimensional distributions of NO could be observed not only the discharge zone but also both the downstream and the upstream regions of the reactor. In the present reactor at a low main gas flow rate, electrohydrodynamic (EHD) flow became dominant, and the flow towards the upstream affected the decrease of NO along the reactor from the upstream region. It is considered that this information is important for modeling and optimizing the plasma processes and designing the non-thermal plasma reactors.

Report

(3 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • Research Products

    (36 results)

All Other

All Publications (36 results)

  • [Publications] S.Kanazawa: "Two-Dimensional Imaging of NO Density Profiles by LIF Technique in a Pipe With Nozzles Electrode During NO Treatment"IEEE Transactions on Industry Applications. 39・2(印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Ohkubo: "Streamer Corona Discharge Induced by Laser Pulses During LIF Measurements in a DC Non-thermal Plasma Reactor for NO Oxidation"Journal of Adv.Oxid.Technol.. 5・2. 129-134 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Ohkubo: "LIF Diagnostics of Ground-State NO Density in a Reactor with Streamer Corona Plasma"Proceedings of SPIE Selected Research Papers on Spectroscopy of Nonequilibrium Plasma at Elevated Pressures. 4460. 318-329 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kanazawa: "Two-dimensional Distribution of Ground-State NO Density by LIF Technique in DC Needle-to-Plate Positive Streamer Coronas During NO Removal Processing IEEE"IEEE Transactions on Industry Applications. 37・6. 1663-1667 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kanazawa: "Two-Dimensional Observation of Laser-Induced Streamer Corona Discharge Under a Non-uniform Field"Proceedings of 2001 Japan-Korea Joint Symposium on Electrical Discharge and High Voltage Engineering. 317-320 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 首藤康之: "レーザ誘起蛍光法による大気圧非熱平衡プラズマ中のNO計測"大分大学工学部研究報告. 44. 35-39 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y. Shuto, N. Sato, S. Akamine, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "NO Molecule Measurements in Atmospheric Pressure Non-thermal Plasmas by Laser Induced Fluorescence"Reports of the Faculty of Engineering Oita University. 44. 35-39 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, T. Ito, Y. Shuto, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "Two-dimensional Distribution of Ground-State NO Density by LIF Technique in DC Needle-to-Plate Positive Streamer Coronas During NO Removal Processing"IEEE Transantions on Industry Applications. 37. 1663-1667 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, Y. Shuto, N. Sato, T. Ohkubo, Y. Nomoto, J. Mizeraczyk,: "Measurement of NO Molecules in DC Streamer Corona Discharges by Laser Induced Fluorescence"Proc. of the Second Polish-Japanese Hakone Group Symposium on Non-Thermal Plasma Processing of Water and Air. 38-42 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y. Shuto, N. Sato, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "Observation of NO Molecules in DC Streamer Corona by Laser Induced Fluorescence"Proc. of 2001 Annual Meeting of The Institute of Electrostatics Japan. 11a-B2. 5-6 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y. Shuto, N. Sato, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "NO Molecule Measurements in Atmospheric Pressure DC Streamer Coronas by LIF Technique"Papers of Techincal Meeting on Pulsed Power and Electrical Discharges, PPT-01-87, ED-01-141, IEE Japan. 47-52 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y. Shuto, N. Sato, S. Akamine, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "LIF Diagnostic in DC Positive Sreamer Coronas fot NO Treatment"Proceedings of 2001 Japan-Korea Joint Symposium on Electrical Discharge and High Voltage Engineering. 129-132 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, Y. Shuto, N. Sato, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "Two-dimensional Observation of Laser-Induced Streamer Corona Discharge Under a Non-uniform Field"Proceedings of 2001 Japan-Korea Joint Symposium on Electrical Discharge and High Voltage Engineering. 317-320 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, Y. Shuto, N. Sato, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "Two-Dimensional Observatin of NO Molecules in Atmospheric Pressure Discharge Plasmas by Laser-Induced Fluorescence"Japan Congress on High Speed Photography and Photonics 2001. 8-12. 195-198 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Ohkubo, S. Kanazawa, Y. Shuto, Y. Nomoto, J. Mizeraczyk: "LIF Diagnostics of Ground-State NO Density in a Reactor with Streamer Corona Plasma"Proceedings of SPIE Selected Research Papers on Spectroscopy of Nonequilibrium Plasma at Elevated Pressures. 4460. 318-329 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, T. Ito, Y. Shuto, T. Ohkubo, Y. Nomoto, J. Mizeraczyk: "Characteristics of Laser Induced Streamer Corona Discharge in a Needle-to-Plate Electrode Dydtem"Journal of Electrostatics. 55. 343-350 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Ohkubo, T. Ito, Y. Shuto, S. Akamine, S. Kanazawa, Y. Nomoto, J. Mizeraczyk: "Streamer Corona Discharge Induced by Laser Pulses During LIF Measurements in a DC Non-thermal Plasma Reactor for NO Oxidation"Journal of Adv. Oxid. Technol.. 5. 129-134 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N. Sato, Y. Shuto, S. Kanazawa, T. Ohukubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "Wide Space NO LIF Observation in Atmospheric-Pressure DC Streamer Coronas"2002 National Convention Record IEE Japan. 1. 64-64 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N. Sato, T. Sumi, S. Kanazawa, T. Ohkubo, J. Mizeraczyk, J.S. Chang: "Wide Range Measurement of NO Molecules in Atmospheric Pressure DC Streamer Coronas by Laser-Induced Fluorescence"Proc. of 2002 Annual Meeting of The Institute of Electrostatics Japan. 29pB-2. 103-104 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] N. Sato, T. Sumi, S. Akamine, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "Wide Range Measurement of NO Density Profiles in Atmospheric Pressure DC Streamer Coronas by LIF Technique"Record of 2002 Joint Conference of Electrcal and Electronics Engineers in Kyushu. 733. 371-371 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Sumi, N. Sato, S. Kanazawa, T. Ohkubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "NO Molecule Measurements in Atmospheric Pressure DC Streamer Coronas by LIF Technique - Part 2 -"Papers of Technical Meeting on Electrical Discharges. ED-02-137, IEE Japan. 41-44 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, N. Sato, T. Sumi, T. Ohkubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "Two-Dimensional Observation of NO Molecules in Atmosperic Pressure Non-Thermal Plasmas by Laser Induced Fluorescence"Reports on the 305th Topical Meeting of The Laser Society of Japan. RTM-02-45. 19-23 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, N. Sato, T. Sumi, T. Ohkubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "Observation of NO Concentration Distribution in a DC Streamer Coronas Discharge Reactor by Laser Induced Fluorescence"Record of 2002 The Japan Society of Applied Physics in Kyushu. 1Ap-1. 16-16 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S. Kanazawa, Y. Shuto, N. Sato, T. Ohukubo, Y. Nomoto, J. Mizeraczyk, J.S. Chang: "Two-Dimensional Imaging of NO Density Pofiles by LIF Technique in a Pipe With Nozzles Electrode During NO Treatment"IEEE Transactions on Industry Applications. 39. (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.Kanazawa: "Two-Dimensional Imaging of NO Density Profiles by LIF Technique in a Pipe With Nozzles Electrode During NO Treatment"IEEE Transactions on Industry Applications. 39・2(印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Ohkubo: "Streamer Corona Discharge Induced by Laser Pulses During LIF Measurements in a DC Non-thermal Plasma Reactor for NO Oxidation"Journal of Adv. Oxid. Technol.. 5・2. 129-134 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Ohkubo: "LIF Diagnostics of Ground-State NO Density in a Reactor with Streamer Corona Plasma"Proceedings of SPIE Selected Research Papers on Spectroscopy of Nonequilibrium Plasma at Elevated Pressures. 4460. 318-329 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kanazawa: "Two-dimensional Distribution of Ground-State NO Density by LIF Technique in DC Needle-to-Plate Positive Streamer Coronas During NO Removal Processing IEEE"IEEE Transactions on Industry Applications. 37・6. 1663-1667 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kanazawa: "Two-Dimensional Observation of Laser-Induced Streamer Corona Discharge Under a Non-uniform Field"Proceedings of 2001 Japan-Korea Joint Symposium on Electrical Discharge and High Voltage Engineering. 317-320 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] 首藤康之: "レーザ誘起蛍光法による大気圧非熱平衡プラズマ中のNO計測"大分大学工学部研究報告. 44. 35-39 (2001)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Kanazawa: "NO LIF Measurements During NOx Removal in a Corona Radical Shower Reactor"Non-Thermal Plasma Technology for Pollution Control Proceedings of The Third International Symposium. 136-141 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 首藤 康之: "レーザ誘起蛍光法による大気圧非熱平衡プラズマ中のNO計測"大分大学工学部研究報告. 44. 35-39 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 金沢 誠司: "レーザー誘起蛍光法による大気圧放電プラズマ中のNO分子の2次元観測"高速度撮影とフォトニクスに関する総合シンポジウム2001講演論文集. 8-12. 195-198 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kanazawa: "Measurement of NO molecules in DC Streamer Corona Discharges by Laser Induced Fluorescence"Proc. of the Second Polish-Japanese Hakone Group Symp. on Non-Thermal Plasma Processing of Water and Air. 38-42 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kanazawa: "Two-dimensional Distribution of Ground-State NO Density by LIF Technique in DC Needle-to-Plate Positive Streamer Coronas During NO Removal Processing"IEEE Transactions on Industry Applications. 37.6. 1663-1667 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Kanazawa: "Two-dimensional Imaging of NO Density During NOx Removal by LIF Technique in a Corona Radical Shower Reactor"Conference Record of the 2001 IEEE Industry Applications Conference. 1082-1086 (2001)

    • Related Report
      2001 Annual Research Report

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Published: 2002-04-01   Modified: 2016-04-21  

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