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Research for Physical Properties and Applications to Electronic Devices in Ferromagnetic and Ferroelectric Oxide Films Prepared by Sputtering

Research Project

Project/Area Number 13650364
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionKitakyushu National College of Technology

Principal Investigator

KAJIMA Atsushi  Kitakyushu National College of Technology, Department of Electrical and Electronic Engineering, Assistant Professor, 助教授 (70177377)

Co-Investigator(Kenkyū-buntansha) FUJII Toshitaka  Aichi University of Technology, Department of Electronics and Information Engineering, Professor, 工学部, 教授 (90023168)
Project Period (FY) 2001 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥4,200,000 (Direct Cost: ¥4,200,000)
Fiscal Year 2002: ¥1,000,000 (Direct Cost: ¥1,000,000)
Fiscal Year 2001: ¥3,200,000 (Direct Cost: ¥3,200,000)
Keywordsmagnetic oxide thin films / reactive sputtering / dielectric permeability / electric polarization / 酸化物磁性薄膜 / 反応スパッタリング
Research Abstract

In Bi_2O_3-Fe_2-O_3-PbTiO_3 system thin films prepared by rf-reactive sputtering, ε_r' the real part of dielectric permittivity, was changed by applying a magnetic field H. The Δε_r' vs. H curves of the films subjected to annealing at various temperatures were strongly correlated with their magnetization properties. The maximum relative value of |Δε_r''(H)/ε_r'| reached as much as 1.0%. A ε_r''(H) curve can be reconstructed by a simple model based on uniform magnetization rotation. Next, we measured the temperature dependence of ε_r' and Δε_r'(H)- Both quantities increase rapidly above 50℃, which suggests that softening of the glass network of the dielectric matrix takes place at this temperature to promote the charge displacement giving rise to the dielectric polarization. In addition, we measured the magnetic field dependence of the displacement current Jd(H) to confirm whether the permeability change with magnetic field Δε_r''(H) is intrinsic. It was found that Jd(H) is also subject to change in a similar manner to Δε_r'(H), indicating that the charge displacement assisted by H really occurs. Finally, we observed the dielectric polarization induced by applying a small ac magnetic field at room temperature. This is considered to be a new type of electromagnetic effect. To explain the experimental results, we propose a simple model based on magnetization rotation of ferromagnetic nano-clusters dispersed in a dielectric glassy matrix.

Report

(3 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • Research Products

    (16 results)

All Other

All Publications (16 results)

  • [Publications] T.Fujii: "Dielectric Response Against Magnetic Field in Feroelectric Nano-composite Bi_2O_3-Fe_2O_3-PbTiO_3 Films"Proceedings of the 8th Annual International Conference on Composites Engineering 2001, Tenerife, Canary Islands, Spain. 257-258 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 加島 篤: "Fe_2O_3-Bi_2O_3-PbTiO_3系酸化物薄膜における磁界による誘電率変化"日本応用磁気学会誌. 26巻4号. 445-448 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A.Kajima: "Variation of Dielectric Permeability by Applying Magnetic Field in Nano-composite Bi_2O_3-Fe_2O_3-PbTiO_3 Sputtered Films"Journal of Magnetism and Magnetic Materials. (印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Fujii: "Dielectric Permeability in Nano-composite Ferromagnetic Oxide Films Prepared by RF-Sputtering"Proceedings of International Conference on Advanced Material Processing 2002, Singapore. (印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 加島 篤: "鉄基強磁性酸化物スパッタ薄膜における磁界誘導電気分極"日本応用磁気学会誌. (印刷中). (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Fujii: "Dielectric Response Against Magnetic Field in Ferroelectric Nano-composite Bi_2O_3-Fe_2-O_3-PbTiO_3 Films"Proceedings of the 8th Annual International Conference on Composites Engineering 2001, Tenerife, Canary Islands, Spain. 257-258 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A. Kajima: "Dielectric Permittivity Changes with Magnetic Field in Fe_2-O_3-PbTiO_3 System Oxide Film"Journal of Magnetic Society of Japan. 26,No.4. 445-448 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A. Kajima: "Variation of Dielectric Permeability by Applying Magnetic Field in Nano-composite Bi_2O_3-Fe_2-O_3-PbTiO_3 Sputtered Films"Journal of Magnetism and Magnetic Materials. in print. (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Fujii: "Dielectric Permeability in Nano-composite Ferromagnetic Oxide Films Prepared by RF-Sputtering"Proceedings of International Conference on Advanced Material Processing 2002, Singapore. (in print). (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] A Kajima: "Magnetic-FieId-Induced Electric Polarization in Iron-Based Ferromagnetic Oxide Sputtered Films"Journal of Magnetic Society of Japan. (in print). (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] 加島 篤: "Fe_2O_3-Bi_2O_3-PbTiO_3系酸化物薄膜における磁界による誘電率変化"日本応用磁気学会誌. 26巻4号. 445-448 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Kajima: "Variation of Dielectric Permeability by Applying Magnetic Field in Nano-composite Bi_2O_3-Fe_2O_3-PbTiO_3 Sputtered Films"Journal of Magnetism and Magnetic Materials. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Fujii: "Dielectric Permeability in Nano-composite Ferromagnetic Oxide Films Prepared by RF-Sputtering"Proceedings of International Conference on Advanced Material Processing 2002, Singapore. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] 加島 篤: "鉄基強磁性酸化物スパッタ薄膜における磁界誘導電気分極"日本応用磁気学会誌. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Fujii: "DIELECTRIC RESPONSE AGAINST MAGNETIC FIELD IN FERROMAGNETIC NANO-COMPOSITE Bi2O3-Fe2O3-PbTiO3 FILMS"Proseedings of ICCE/8(Spain). 257-258 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 加島 篤: "Fe_2O_3-Bi_2O_3-PbTiO_3系酸化物薄膜における磁界による誘電率変化"日本応用磁気学会誌. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report

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Published: 2001-04-01   Modified: 2016-04-21  

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