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Material and functional study for the spin manipulation

Research Project

Project/Area Number 14076218
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionThe Institute of Physical Chemical Research (RIKEN)

Principal Investigator

ISHIBASHI Koji  Advanced Device Lab. RIKEN, Chief Scientist, 石橋極微デバイス工学研究室, 主任研究員 (30211048)

Project Period (FY) 2002 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥19,800,000 (Direct Cost: ¥19,800,000)
Fiscal Year 2005: ¥5,400,000 (Direct Cost: ¥5,400,000)
Fiscal Year 2004: ¥5,500,000 (Direct Cost: ¥5,500,000)
Fiscal Year 2003: ¥5,300,000 (Direct Cost: ¥5,300,000)
Fiscal Year 2002: ¥3,600,000 (Direct Cost: ¥3,600,000)
KeywordsCarbon nanotube / Artificial atom / Quantum dot / Zeeman effect / Single electron transport / Interacting two-electron system / 量子ビット / 単電子トランジスタ / スピン量子操作 / スピン緩和時間 / ゼーマン分裂 / GaAs / AlGaAs2次元電子ガス / アンチドット / 量子ホール効果 / エッジ状態 / 単電子輸送現象 / 電子殻構造 / スピン操作 / 電子数の偶奇性効果 / クーロンブロッケード
Research Abstract

We have explored possibilities of manipulation of election spins in quantum dots in single wall-carbon nanotubes (SWCNA) and isolated edge states in a two dimensional electron gas in GaAs/AlGaAs heterostructures under the high magnetic fields. In both cases, bound states with well defined spin direction can be expected. We found that the SWCNT quantum dots are promising building blocks for single spin generation and manipulation.
The single quantum dot was fabricated simply by depositing metallic contacts on top of an individual SWCNT, and the SWCNT between the contacts behaves as a single quantum dots. This is confirmed by the fact that the energy level spacing measured in experiments agreed with a simple one-dimensional model with a length of the gap between the contacts. Single electron transport measurements have been carried out at milli-Kelvin temperatures to investigate the artificial atom nature of the quantum dot. At low temperatures, Coulomb oscillations with a period of two a … More nd four electrons are observed. The former arises from the band degeneracy of the SWCNT in addition the spin degeneracy. The latter appears when the band degeneracy is lifted due to imperfection of the material, and the spin degeneracy remains. These observation indicates that the SWCNT quantum dot show four or two electron shell structures.
The excitation spectroscopy has been carried out by measuring a Coulomb peak with a large source drain bias voltage. Zero-dimensional confined states are observed, which split into two blanched as the magnetic field is applied, a clear evidence of the Zeeman splitting. When two elections are existing in a shell, the quantum states of the interacting two-electron system, which are the singlet and triplet states, observed. The two states have a different energy at a zero magnetic field. The gate-pulse measurements revealed that the energy relaxation time in the Zeeman levels were more than lmicro second.
The important implication of the experiments is that the shell structures are observable even many electrons in a quantum dot which is in a striking contrast to semiconductor quantum dots where shell structures are only observable with few electrons in a dot. This is due to the fact that the zero-dimensional level spacing is much larger than electron-electron interaction energy in the SWCNT quantum dot This means that single spin can be generated by putting one electron in a shell. We have tried to coherently manipulate the single spin by using the Electron Spin Resonance (ESR) technique in frequencies ranging from 10 GHz to 100GHz, but the we did not succeed in. manipulating it. The stronger coupling between the spin and the electromagnetic wave is necessary. Less

Report

(5 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (26 results)

All 2006 2005 2004 Other

All Journal Article (24 results) Publications (2 results)

  • [Journal Article] Carbon nanotubes as building blocks of quantum dots2006

    • Author(s)
      K.Ishibashi, S.Moriyama, T.Fuse, T.Yamaguchi
    • Journal Title

      Physica E 35

      Pages: 338-343

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Quantum-Dot Nanodevices with Carbon Nanotubes2006

    • Author(s)
      K.Ishibashi, S.Moriyama, D.Tsuya, T.Fuse, M.Suzuki
    • Journal Title

      J. Vac. Sci. Technol. A 24

      Pages: 1349-1355

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Pulse-excited current measurements in carbon nanotube quantum dots2006

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, T.Yamaguchi, K.Ishibashi
    • Journal Title

      J. Phys. Conference Series 38

      Pages: 9-12

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] One-Dimensional Shell Structures and Excitation Spectrum in Single-Wall Carbon Nanotube Quantum Dots2006

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, K.Ishibashi
    • Journal Title

      Jpn. J. Appl. Phys 45

      Pages: 3633-3637

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Carbon nanotubes as building blocks of quantum dots2006

    • Author(s)
      K.Ishibashi, S.Moriyama, T.Fuse, T.Yamaguchi
    • Journal Title

      Physica E35

      Pages: 338-343

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Quantum-Dot Nanodevices with Carbon Nanotubes2006

    • Author(s)
      K.Ishibashi, S.Moriyama, D.Tsuya, T.Fuse, M.Suzuki
    • Journal Title

      J. Vac. Sci. Technol A24

      Pages: 1349-1355

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] One-Dimensional Shell Structures and Excitation Spectrum in Single-Wall Carbon Nanotube Quantum Dots2006

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, K.Ishibashi
    • Journal Title

      Jpn. J. Appl. Phys. 45

      Pages: 3633-3637

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Excitation spectroscopy of two-electron shell structures in carbon nanotube quantum dots in magnetic fields2005

    • Author(s)
      S.Moriyama, T.Fuse, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Appl. Phys. Lett 87

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Four-electron shell structures and an interacting two-electron system in carbon nanotube quantum dots2005

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Phys. Rev. Lett. 94

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Resonant tunneling through edge states bounded around an antidot2005

    • Author(s)
      K.Arai, K.Ishibashi
    • Journal Title

      Physica E 26

      Pages: 469-472

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Importance of electron-electron interactions and Zeeman splitting in single-wall carbon nanotube quantum dots2005

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Physica E 26

      Pages: 473-476

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Excitation spectroscopy of two-electron shell structures in carbon nanotube quantum dots in magnetic fields2005

    • Author(s)
      S.Moriyama, T.Fuse, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Appl. Phys. Lett. 87

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Resonant tunneling through edge states bounded around an antidot2005

    • Author(s)
      K.Arai, E.Ishibashi
    • Journal Title

      Physica E26

      Pages: 469-472

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Importance of electron-electron interactions and Zeeman splitting in single-wall carbon nanotube quantum dots2005

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Physica E26

      Pages: 473-476

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Four-electron shell structures and an interacting two-electron system in carbon nanotube quantum dots2005

    • Author(s)
      S.Moriyama, T.Fuse, M.Suzuki, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Physical Review Letters 94

      Pages: 186806-186806

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Large spin injection into single-and multi-walled carbon nanotubes2005

    • Author(s)
      Y.Ishiwata, H.Maki, D.Tsuya, M.Suzuki, K.Ishibashi
    • Journal Title

      Physica Status Solidi(c) 2

      Pages: 3137-3140

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Excitation spectroscopy of two-electron shell structures in carbon nanotube quantum dots in magnetic fields2005

    • Author(s)
      S.Moriyama, T.Fuse, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Applied Physics Letters 87

      Pages: 73103-73103

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Carbon nanotube quantum dots fabricated on a GaAs/AlGaAs two-dimensional electron gas substrate2005

    • Author(s)
      T.Tsukamoto, S.Moriyama, D.Tsuya, M.Suzuki, T.Yamaguchi, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Journal of Applied Physics 98

      Pages: 76106-76106

    • Related Report
      2005 Annual Research Report
  • [Journal Article] On the realization of quantum computing devices with carbon nanotube quantum dots2004

    • Author(s)
      K.Ishibashi, Y.Moriyama, T.Fuse
    • Journal Title

      IEICE TRANSACTIONS ON ELECTRONICS E87C

      Pages: 1799-1803

    • NAID

      110003214794

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Two-electron and four-electron periodicity in single-wall carbon nanotube quantum dots2004

    • Author(s)
      T.Fuse, S.Moriyama, Y.Aoyagi, M.Suzuki, K.Ishibashi
    • Journal Title

      Superlattices and Microstructures 3

      Pages: 377-382

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Local Change of Carbon Nanotube-Metal Contacts by Current Flow through Electrodes2004

    • Author(s)
      Hideyuki Maki, Masaki Suzuki, Koji Ishibashi
    • Journal Title

      Jpn. J. Appl. Phys 43

      Pages: 2027-2030

    • NAID

      10012949225

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Local Change of Carbon Nanotube-Metal Contacts by Current Flow through Electrodes2004

    • Author(s)
      Hideyuki Maki, Masaki Suzuki, Koji Ishibashi
    • Journal Title

      Jpn. J. Appl. Phys. 43

      Pages: 2027-2030

    • NAID

      10012949225

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Two-electron and four-electron periodicity in single-wall carbon nanotube quantum dots2004

    • Author(s)
      T.Fuse, S.Moriyama, Y.Aoyagi, M.Suzuki, K.Ishibashi
    • Journal Title

      Superlattices and Microstructures 34

      Pages: 377-382

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Carbon nanotubes as a building block of quantum dot devices2004

    • Author(s)
      M.Suzuki, U.Tsuya, S.Moriyarna, T.Fuse, Y.Aoyagi, K.Ishibashi
    • Journal Title

      Physica E 24

      Pages: 10-13

    • Related Report
      2004 Annual Research Report
  • [Publications] T.Fuse, S.Moriyama, M.Suzuki, Y.Aoyagi, K.Ishibashi: "Observation of even-odd effect and fourfold degeneracy in single-wall carbon nanotube quantum dots"Superlattices and Microstructures. (掲載予定). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Ishibashi, M.Suzuki, D.Tsuya, Y.Aoyagi: "Fabrication of single electron transistors in multi-wall carbon nanotubes by using Ar beam irradiation"Microelectronic Engineering. (in press).

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2018-03-28  

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