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Study of giant thermal conductivity due to magnons in low-dimensional quantum spin system copper oxides

Research Project

Project/Area Number 14340097
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTohoku University

Principal Investigator

KOIKE Yoji  Tohoku University, Graduate School of Engineering, Professor, 大学院・工学研究科, 教授 (70134038)

Co-Investigator(Kenkyū-buntansha) KATO Masatsune  Tohoku University, Graduate School of Engineering, Associate Professor, 大学院・工学研究科, 助教授 (50211850)
NOJI Takashi  Tohoku University, Graduate School of Engineering, Research Associate, 大学院・工学研究科, 助手 (50180740)
ADACHI Tadashi  Tohoku University, Graduate School of Engineering, Research Associate, 大学院・工学研究科, 助手 (40333843)
Project Period (FY) 2002 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥17,000,000 (Direct Cost: ¥17,000,000)
Fiscal Year 2004: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2003: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 2002: ¥13,800,000 (Direct Cost: ¥13,800,000)
Keywordsquantum spin system / low-dimensional system / thermal conductivity / magnon / spin gap / antiferromagnetism / spin flop transition / Bose-Einstein condensation / 高温超伝導 / 磁場誘起磁気秩序 / ストライプ秩序 / 銅酸化物 / 強磁性
Research Abstract

We have studied the thermal conductivity and other physical properties of several copper oxides regarded as low-dimensional quantum spin systems, in order to clarify the mechanism of the giant thermal conductivity due to magnons and also to clarify whether the thermal conductivity measurement is powerful for the detection of a phase transition or not.
We have discovered large thermal conductivity due to magnons in the four-leg spin-ladder system La_2Cu_2O_5 and the two-dimensional spin system Cu_3B_2O_6.
In one-dimensional spin systems Sr_2CuO_3 and SrCuO_2, we have proved from the study of the impurity effects that the thermal conductivity due to magnons is very large and that the thermal conduction is ballistic as theoretically expected.
From these results, it has been concluded that both the large antiferromagnetic interaction between spins and the large dispersion of magnons give rise to the large thermal conductivity due to magnons.
Moreover, marked changes of the thermal conductivity have been observed at the following phase transitions; the spin-flop transition in the antiferromagnetically ordered state of Ca_2Y_2Cu_5O_<10> and Cu_3B_2O_6, the Bose-Einstein condensation transition off magnons in TlCuCl_3 under high magnetic fields at low temperatures, and the field-induced magnetic order in La_<2-x>Sr_xCUO_4 and La_<2-x>Ba_xCuO_4. Accordingly, we have concluded that the thermal conductivity measurement is a powerful probe to detect and study a phase transition.

Report

(4 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (52 results)

All 2005 2004 2003 Other

All Journal Article (41 results) Publications (11 results)

  • [Journal Article] Single-crystal growth and the dependence on hole concentration and magnetic field of the magnetic ground state in the edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>2005

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 71

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Effects of hole doping on the magnetic ground state and excitation in the edge-sharing CuO_2 chain of Ca_<2+x>Y_<2-x>Cu_5O_<10>2005

    • Author(s)
      M.Matsuda
    • Journal Title

      Physical Review B 71

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced and impurity-induced magnetic order in La_<2-x>Sr_xCuO_4 studied by the thermal conductivity and μSR2005

    • Author(s)
      Y.Koike
    • Journal Title

      International Journal of Modern Physics B 19・1,2&3(印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] μSR and thermal conductivity studies on inhomogeneity of the impurity- and field-induced magnetism and superconductivity in high-T_c cuprates2005

    • Author(s)
      Y.Koike
    • Journal Title

      Physica C (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Fieldinduced magnetic order and thermal conductivity in La_<1.87>Sr_<0.13> Cu_<1-y>MyO_4(M=Zn,Ni)2005

    • Author(s)
      T.Kawamata
    • Journal Title

      Physica C (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Single-crystal growth and the dependence on hole concentration and magnetic field of the magnetic ground state in the edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>.2005

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 71

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Effects of hole doping on magnetic ground and excited states in the edge-sharing CuO_2 chains of Ca_<2+x> Y_<2-x>Cu_5O_<10>.2005

    • Author(s)
      M.Matsuda
    • Journal Title

      Physical Review B 71

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced and impurity-induced magnetic order in La_<2-x>Sr_xCuO_4 studied by the thermal conductivity and μSR.2005

    • Author(s)
      Y.Koike
    • Journal Title

      International Journal of Modern Physics B 19Nos.1,2&3(in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced and impurity-induced magnetic order in La_<2-x>Sr_xCuO_4 studied by the thermal conductivity and MSR2005

    • Author(s)
      Y.Koike
    • Journal Title

      International Journal of Modern Physics B 19・1,2&3(印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Effects of hole-doping on the magnetic ground state and excitations in the edge-sharing CuO_2 chain of Ca_<2+x>Y_<2-x>Cu_5O_<10>2005

    • Author(s)
      M.Matsuda
    • Journal Title

      Physical Review B 71(印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] MSR and thermal conductivity studies on inhomegeneity of the imparity- and field-induced magnetism and superconductivity in high-T cuprates2005

    • Author(s)
      Y.Koike
    • Journal Title

      Physica C (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Field-induced magnetic order and thermal conductivity in Ld_<1.87>Sr_<0.13>Cu_<1-y>M_yO_4(M=Zn,Ni)2005

    • Author(s)
      T.Kawamata
    • Journal Title

      Physica C (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Single-crystal growth and the dependence on hole concentration and magnetic field of the magnetic ground state in the edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>2005

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 71(印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Drastic Enhancement of Thermal Conductivity in the Bose-Einstein Condensed State of TlCuCl_32004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73

      Pages: 2358-2361

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnon thermal conductivity in the spin-gap state and the antiferromagnetically ordered state of low-dimensional copper oxides2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 94-95

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity in Bose-Einstein condensed state of TlCuCl_32004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 214-215

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced magnetic order in La_<2-x>Sr_xCuO_4 (x = 0.10,0.115,0.13) studied by in-plane thermal conductivity measurements2004

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 70

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Multi-Triplet Magnon in SrCu_2(BO_3)_2 Studied by Thermal Conductivity Measurements in Magnetic Fields2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73

      Pages: 3497-3498

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Drastic enhancement of thermal conductivity in the Bose-Einstein condensed state of TlCuCl_3.2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73

      Pages: 2358-2361

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnon thermal conductivity in the spin-gap state and the antiferromagnetically ordered state of low-dimensional copper oxides.2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 94-95

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity in the Bose-Einstein condendsed state of TlCuCl_3.2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 214-215

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced magnetic order in La_<2-x>Sr_xCuO_4(x=0.10, 0.115, 0.13) studied by in-plane thermal conductivity measurements.2004

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 70

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Multi-triplet magnons in SrCu_2(BO_3)_2 studied by thermal conductivity measurements in magnetic fields.2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73

      Pages: 3497-3498

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity in the Bose-Einstein condensed state of TlCuCl_32004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Magnetism and Magnetic Materials 272-276

      Pages: 214-215

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Drastic Enhancement of Thermal Conductivity in the Bose-Einstein Condensed State of TlCuCl_32004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73・9

      Pages: 2358-2361

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Field-induced magnetic order in La_<2-x>Sr_xCuO_4(x=0.10,0.115,0.13) studied by in-plane thermal conductivity measurements2004

    • Author(s)
      K.Kudo
    • Journal Title

      Physical Review B 70

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Multi-Triplet Magnons in SrCu_2(BO_3)_2 Studied by Thermal Conductivity Measurements in Magnetic Fields2004

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 73・12

      Pages: 3497-3498

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Anisotropic Magnetic Properties and Anomalous Thermal Conductivity in the bc Plane of the Quasi-Two-Dimensional Spin System Cu_3B_2O_62003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 72

      Pages: 569-575

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Antiferromagnetic ordering in the one-dimensional edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>2003

    • Author(s)
      S.Kurogi
    • Journal Title

      Journal of Low Temperature Physics 131

      Pages: 353-357

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity of the four-leg spin-ladder system La_2Cu_2O_5 single crystal2003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Low Temperature Physics 131

      Pages: 725-729

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Zn-Substitution Effects on the Thermal Conductivity of the Two-Dimensional Spin-Gap System SrCu_2(BO_3)_2 and the Two-Dimensional Antiferromagnetic System Cu_3B_2O_6 Single-Crystals2003

    • Author(s)
      K.Kudo
    • Journal Title

      Physica B 329-333

      Pages: 910-911

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Single-Crystal Growth and Thermal Conductivity of the Four-Leg Spin-Ladder System La_2Cu_2O_52003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 72

      Pages: 2551-2555

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] 低次元量子スピン系の熱伝導2003

    • Author(s)
      工藤一貴
    • Journal Title

      固体物理 38

      Pages: 889-902

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Anisotropic magnetic properties and anomalous thermal conductivity in the be plane of the quasi-two-dimensional spin system Cu_3B_2O_6 : Relation between the thermal conductivity and the spin state in magnetic fields.2003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 72

      Pages: 569-575

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Antiferromagnetic ordering in the one-dimensional edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>.2003

    • Author(s)
      S.Kurogi
    • Journal Title

      Journal of Low Temperature Physics 131

      Pages: 353-357

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity of the four-leg spin-ladder system La_2Cu_2O_5 single crystal.2003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of Low Temperature Physics 131

      Pages: 725-729

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Zn-substitution effect on the thermal conductivity of the two-dimensional spin-gap system SrCu_2(BO_3)_2 and the two-dimensional antiferromagnetic system Cu_3B_2O_6 single-crystals.2003

    • Author(s)
      K.Kudo
    • Journal Title

      Physica B 329-333

      Pages: 910-911

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Single-crystal growth and thermal conductivity of the four-leg spin-ladder system La_2Cu_2O_5.2003

    • Author(s)
      K.Kudo
    • Journal Title

      Journal of the Physical Society of Japan 72

      Pages: 2551-2555

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal conductivity in low-dimensional quantum spin systems.2003

    • Author(s)
      K.Kudo
    • Journal Title

      Solid State Physics[in Japanese] 38

      Pages: 889-902

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] μSR and thermal conductivity studies on inhomogeneity of the impurity-and field-induced magnetism and superconductivity in high-T_c cuprates.

    • Author(s)
      Y.Koike
    • Journal Title

      Physica C. (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Field-induced magnetic order and thermal conductivity in La_<1.87>Sr_<0.13>Cu_<1-y>M_yO_4(M=Zn, Ni).

    • Author(s)
      T.Kawamata
    • Journal Title

      Physica C. (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] K.Kudo: "Anisotropic Magnetic Properties and Anomalous Thermal Conductivity in the bc Plane of the Quasi-Two- Dimensional Spin System Cu_3B_2O_6"Journal of the Physical Society of Japan. 72・3. 569-575 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Kurogi: "Antiferromagnetic ordering in the one-dimensional edge-sharing CuO_2 chain system Ca_<2+x>Y_<2-x>Cu_5O_<10>"Journal of Low Temperature Physics. 131・3/4. 353-357 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Kudo: "Thermal conductivity of the four-leg spin-ladder system La_2Cu_2O_5 single crystal"Journal of Low Temperature Physics. 131・3/4. 725-729 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Kudo: "Zn-Substitution Effect on the Thermal Conductivity of the Two-Dimensional Spin-Gap System SrCu_2 (BO_3)_2 and the Two-Dimensional Antiferromagnetic System Cu_3B_2O_6 Single-Crystals"Physica B. 329-333. 910-911 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Kudo: "Single-Crystal Growth and Thermal Conductivity of the Four-Leg Spin-Ladder System La_2Cu_2O_5"Journal of the Physical Society of Japan. 72・10. 2551-2555 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Kudo: "Magnon thermal conductivity in the spin-gap state and the antiferromagnetically ordered state of low-dimensional copper oxides"Journal of Magnetism and Magnetic Materials. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Kudo: "Thermal conductivity in the Bose-Einstein condensed state of TlCuCl_3"Journal of Magnetism and Magnetic Materials. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Kazutaka Kudo: "Anisotropic Magnetic Properties and Anomalous Thermal Conductivity in the be Plane of the Quasi-Two-Dimensional Spin System Cu_3B_2O_6"Journal of the Physical Society of Japan. 72・3(印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Kazutaka Kudo: "Thermal conductivity of the four-leg spin-ladder system La_2Cu_2O_5 single crystal"Journal of Low Temperature Physics. 131(印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Shogo Kurogi: "Antiferromagnetic ordering in the one-dimensional edge-sharing CuO_2 chain system Ca_<2+X>Y_<2-X>Cu_5O_<10>"Journal of Low Temperature Physics. 131(印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Kazutaka Kudo: "Zn-Substitution Effect on the Thermal Conductivity of the Two-Dimensional Spin-Gap System SrCu_2(BO_3)_2 and the Two-Dimensional Antiferromagnetic System Cu_3B_2O_6 Single-Crystals"Physica B. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2020-05-15  

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