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Experimental study on the interaction of multiply-charged ions with rare gas solid surfaces

Research Project

Project/Area Number 14340125
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 物理学一般
Research InstitutionRikkyo University

Principal Investigator

HIRAYAMA Takato  Rikkyo University, Faculty of Science, Professor Associate, 理学部, 助教授 (40218821)

Co-Investigator(Kenkyū-buntansha) FURUHASHI Osamu  RCMAS, Post-Doctoral Fellow, 研究員 (50350327)
Project Period (FY) 2002 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥14,500,000 (Direct Cost: ¥14,500,000)
Fiscal Year 2004: ¥3,100,000 (Direct Cost: ¥3,100,000)
Fiscal Year 2003: ¥6,300,000 (Direct Cost: ¥6,300,000)
Fiscal Year 2002: ¥5,100,000 (Direct Cost: ¥5,100,000)
KeywordsRare Gas Solid / DIET / Multiply-charged ions / Kinetic Sputtering / Potential Sputtering / Cluster / Exciton / Van der Waals固体 / 角度分布 / 同時計測
Research Abstract

Experimental study has been done on the interaction of multiply-charged ions and low-energy electrons with rare gas solid surfaces. Following results have been obtained.
・Time-of-Flight spectra have been measured for the desorbed metastable atoms from the surface of solid Ne by low energy electron impact. By annealing the sample surface at the temperature of 7.0K, the kinetic energy of desorbed atoms was increased, and the sharpness of the angular distribution was also increased toward the normal direction of the sample surface. These results have been explained by considering the crystallization of the sample surface by annealing.
・Cluster ions desorbed from the surface of solid Ne by multiply charged ion impact have been measured. Surprisingly large clusters the size of which reached to 100 was observed.
・Absolute desorption yields have been measured from the surface of solid Ne by Ar^<q+>(q=1〜6) and Ne^<q+>(<q=1〜5) impact. We have succeeded in separating the contribution of 'Potential Sputtering' and 'Kinetic Sputtering' by measuring the dependence of the desorption yield on the incident ion energy. The present results show that 'Kinetic Sputtering' yield was 2.5 atoms per 1 eV incident energy, and 'Potential sputtering' was 3.8 atoms per 1 eV internal energy. We have also shown that the threshold energy for the 'Potential Sputtering' for solid Ne was about 20 eV, which corresponds to the exciton creation energy and band gap energy of solid Ne.

Report

(4 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (19 results)

All 2005 2004 2003 Other

All Journal Article (13 results) Publications (6 results)

  • [Journal Article] Double charge transfer spectroscopy of O_2^<2+> : band analyses of low-lying repulsive states2005

    • Author(s)
      O.Furuhashi, T.Kinugawa, T.Hirayama et al.
    • Journal Title

      Physical Review A70

      Pages: 52501-52501

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Photodesorption of ionized water clusters from water physisorbed on rare gas solids2005

    • Author(s)
      T.Tachibana, Y.Yamauchi, H.Nagasaki, T.Miura, T.Hirayama, M.Sakurai, I.Arakawa
    • Journal Title

      Surf.Sci. (to appear)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Double charge transfer spectroscopy of O_2^<2+> : band analyses of low-lying repulsive states2004

    • Author(s)
      O.Furuhashi, T.Kinugawa, T.Hirayama, T.Koizumi, C.Yamada, S.Ohtani
    • Journal Title

      Phys.Rev.A 70

      Pages: 52501-52501

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Double charge transfer spectroscopy of O^<2+>_2 : band analyses of low-lying repulsive states2004

    • Author(s)
      O.Furuhashi, T.Kinugawa, T.Hirayama, (他3名)
    • Journal Title

      Phys.Rev.A 70

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Double charge transfer spectroscopy of NO^<2+> at vibrational resolution : application of Franck-Condon analyses to a dicationic system2003

    • Author(s)
      O.Furuhashi, T.Kinugawa, T.Hirayama et al.
    • Journal Title

      Chemical Physics 295

      Pages: 185-193

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Absolute yields of the exciton induced desorption at the surface of a solid rare gas2003

    • Author(s)
      I.Arakawa, T.Adachi, T.Hirayama, M.Sakurai
    • Journal Title

      Fizika Nizkikh Temperatur (Low Temperature Physics) 29

      Pages: 259-265

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Absolute measurements of the total PSD and ESD yields at the surface of solid krypton2003

    • Author(s)
      T.Adachi, T.Hirayama, et al.
    • Journal Title

      Surface Science 528

      Pages: 60-66

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Lateral compression of a Xe film physisorbed on Ag(111)2003

    • Author(s)
      S.Igarashi, A.Tosaka, T.Hirayama, et al.
    • Journal Title

      Langmuir 19

      Pages: 4627-4632

    • NAID

      10004562141

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Double charge transfer spectroscopy of NO^<2+> at vibrational resolution : application of Franck-Condon analyses to a dicationic system2003

    • Author(s)
      O.Furuhashi, T.Kinugawa, T.Hirayama, T.Koizumi, C.Yamada, S.Ohtani
    • Journal Title

      Chem.Phys. 295

      Pages: 185-193

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Absolute yields of the exciton induced desorption at the surface of a solid rare gases2003

    • Author(s)
      I.Arakawa, T.Adachi, T.Hirayama, M.Sakurai
    • Journal Title

      Fizika Nizkikh Temperatur (Low Temperature Physics) 29

      Pages: 259-265

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Absolute measurements of the total PSD and ESD yields at the surface of solid krypton2003

    • Author(s)
      T.Adachi, T.Hirayama, T.Miura, I.Arakawa, M.Sakurai
    • Journal Title

      Surf.Sci. 528

      Pages: 60-66

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Lateral Compression of a Xe Film Physisorbed on Ag(111)2003

    • Author(s)
      S.Igarashi, A.Tosaka, T.Hirayama, I.Arakawa
    • Journal Title

      Langmuir 19

      Pages: 4627-4632

    • NAID

      10004562141

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Absolute desorption yield from rare gas solid surfaces by multiply-charged ion impact-Potential sputtering and Kinetic sputtering-

    • Author(s)
      S.Fujita, O.Furuhashi, T.Koizumi, T.Hirayama
    • Journal Title

      (in preperation)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] O.Furuhashi, T.Kinugawa, T.Hirayama, (他3名): "Double charge transfer spectroscopy of NO^<2+> at vibrational resolution : application of Franck-Condon analyses to a dicationic system"Chemical Physics. 295. 185-193 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] I.Arakawa, T.Adachi, T.Hirayama, M.Sakurai: "Absolute yields of the exciton induced desorption at the surface of a solid rare gases"Fizika Nizkikh Temperatur (Low Temperature Physics). 29. 259-265 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Adachi, T.Hirayama, T.Miura, I.Arakawa, M.Sakurai: "Absolute measurements of the total PSD and ESD yields at the surface of solid krypton"Surface Science. 528. 60-66 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Igarashi, A.Tosaka, T.Hirayama, I.Arakawa: "Lateral Compression of a Xe Film Physisorbed on Ag(111)"Langmuir. 19. 4627-4632 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] I.Arakawa, T.Adachi, T.Hirayama, M.Sakurai: "Absolute yields of the exciton induced desorption at the surface of a solid rare gases"Fizika Nizkikh Temperatur (Low Temperature Physics). 29(印刷中). (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Adachi, T.Hirayama, T.Miura, I.Arakawa, M.Sakurai: "Absolute measurements of the total PSD and ESD yields at the surface of solid krypton"Surface Science. (印刷中). (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2016-04-21  

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