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Construction of Four-Dimensional Luminescence-Measuring System for Physico-Chemical Research of Solid Materials

Research Project

Project/Area Number 14340231
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 分離・精製・検出法
Research InstitutionNiigata University

Principal Investigator

HASHIMOTO Tetsuo  Niigata University, Faculty of Science, Professor, 理学部, 教授 (50027439)

Co-Investigator(Kenkyū-buntansha) SAWADA Kiyoshi  Niigata University, Faculty of Science, Professor, 理学部, 教授 (40089850)
IMAIZUMI Hiroshi  Niigata University, Faculty of Engineering, Professor, 工学部, 教授 (80126391)
Project Period (FY) 2002 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥14,700,000 (Direct Cost: ¥14,700,000)
Fiscal Year 2004: ¥2,400,000 (Direct Cost: ¥2,400,000)
Fiscal Year 2003: ¥4,000,000 (Direct Cost: ¥4,000,000)
Fiscal Year 2002: ¥8,300,000 (Direct Cost: ¥8,300,000)
Keywordsradiation-induced luminescence / thermoluminescence / sensitive 3-CCD video-camera / RGB-color imaging analysis / natural white minerals / lattice defects and impurities / radiation dosimetry / archaeological dating / カラー画像解析 / 冷却型3CCDカメラ / 長石と石英 / 自動ルミネッセンス測定システム / 微弱光高感度検出 / 酸化焼成 / 赤外光励起ルミネッセンス / 熱ルミネッセンス / 発光ダイオード / 冷却型CCDカメラ / 高感度撮影 / 天然鉱物
Research Abstract

Radiation-induced luminescence phenomena from natural white minerals, including quartz and feldspar, are not only available for the radiation dosimetry, but also for archaeological and geological dating purposes. In the latter case, the accumulated radiation doses are used because the doses are proportional to the ages after the last burning or sunlight exposure. In this project, the luminescence phenomena have been investigated from aspects of physico-chemical research tool of solid dielectric materials.
A new instrumental system has been developed for four-dimensional luminescence measurements, involving luminescence intensity, wavelength of luminescence, heating temperatures, and positions, using 3-CCD video camera with high sensitivity of light detection. Finally the camera could photograph area of 10x10 mm by selecting suitable lens combination between dark box placed luminescent specimen and sensitive area of video-camera because the radiation-induced luminescence is extremely wea … More k intensity. One picture plane, consisting of 512x672 pixels and 12 bit data of RGB per one pixcel, was realized to be transferred into personal computer memory within 1 second, In the viewpoint of the elimination of dead time loss, the phographic procdure of 2 seconds for every picture was found to be preferable. The final video-camera data-numbers amounted to 350 Mbytes under thermoluminescence observation of every 2-second from 100 to 450℃.
By using the compiled luminescence data on the memory, 100 pixcels were selected out from the CRT-surface picture and followed to the desirable analysis and mutual comparison with other pixcel area with respect of glowcurve-behavior of respective RGB-color regions. As a result, it was established that luminescent difference could be easily distinguished from the data-file, for example, between BTL-quartz grains and RTL-ones. This system was found to be very hopeful for the provenance search of soils and the detection of local lattice defects in dielectric material related to material ageing. Less

Report

(4 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (34 results)

All 2005 2004 2003 Other

All Journal Article (18 results) Book (2 results) Publications (14 results)

  • [Journal Article] Comparison of naturally accumulated radiation-doses between RTL, BTL, OSL, and IRSL using white minerals from archaeological burnt materials and usefulness of RTL-dating from quartz extracts2005

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Geochemical Journal (In press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Comparison of naturally accumulated radiation-doses between RTL, BTL, OSL, and IRSL using white minerals from archaeological burnt materials and usefulness of RTL-dating from quartz extracts.2005

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Geochemical Journal (In press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Single grains dating of volcanic quartz from pyroclastic flows using Red TL.2005

    • Author(s)
      Yoshihiro Ganzawa
    • Journal Title

      Radiation Measurements 39

      Pages: 479-487

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Simultaneous determination of radionuclides belonging to three natural decay series using Time Interval Analysis (TIA)2004

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Analytical and Bioanalytical Chemistry 379

      Pages: 227-233

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Identification of the volcanic quartz origins from dune sand using a single grain RTL-measurement2004

    • Author(s)
      Takashi Yawata
    • Journal Title

      Quaternary Science Review 23

      Pages: 1183-1186

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Simultaneous determination of radionuclides belonging to three natural decay series using Time Interval Analysis(TIA).2004

    • Author(s)
      T.Hashimoto Y.Sanada, Y.Uezu
    • Journal Title

      Anal.Bioanal.Chem. 379

      Pages: 227-233

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Identification of the volcanic quartz origins from dune sand using a single grain RTL-measurement.2004

    • Author(s)
      T.Yawata, T.Hashimoto
    • Journal Title

      Quart.Sci.Rev. 23

      Pages: 1183-1186

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Surface electrofication of rocks and charge trapping centers.2004

    • Author(s)
      Akihiro Takeuchi
    • Journal Title

      Physics and Chemistry of the Earth 29

      Pages: 359-366

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Simultaneous determination of radionuclides belonging to three natural decay series using Time Interval Analysis (TIA).2004

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Anal.Bioanal.Chem. 379

      Pages: 227-233

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Identification of the volcanic quartz origins from dune sand using a single grain RTL-measurement.2004

    • Author(s)
      Takashi Yawata
    • Journal Title

      Quart.Sci.Rev. 23

      Pages: 1183-1186

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Microinfrared reflection spectroscopic mappings : application to the detection of hydrogen-related species in natural quartz.2004

    • Author(s)
      Jun Muto
    • Journal Title

      Journal of Microscopy 216

      Pages: 222-228

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Radiation-induced luminescence and hydrogen radical formation associated with thermal treatments on feldspars2003

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Journal of Radioanalytical Nuclear Chemistry 255

      Pages: 81-85

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Comparison of infrared spectrometric characteristics of Al-OH Impurities and TL-patterns in quartz slices at temperature below 0℃2003

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Radiation Measurements 37

      Pages: 479-485

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Imaging and measurement of red-infrared stimulated luminescence (R-IRSL) from feldspar samples2003

    • Author(s)
      Tetsuo Hashimoto
    • Journal Title

      Ancient TL 21

      Pages: 1-6

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Radiation-induced luminescence and hydrogen radical formation associated with thermal annealing treatments on feldspars2003

    • Author(s)
      T.Hashimoto, E.Nishiyama, Y.Yanagawa
    • Journal Title

      J.Rdioanal.Nucl.Chem. 255

      Pages: 81-85

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Comparison of infrared spectrometric characteristics of Al-OH impurities and thermoluminescence patterns in natural quartz slices at temperature below 0℃.2003

    • Author(s)
      T.Hashimoto.T.Yamaguchi, H.Fujita, Y.Yanagawa
    • Journal Title

      Radial.Meas. 37

      Pages: 479-485

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Imaging and measurement of red-infrared stimulated luminescence(R-IRSL) from feldspar samples.2003

    • Author(s)
      T.Hashimoto.H.Usuda, N.Mitamura, T.Yawata
    • Journal Title

      Ancient TL 21

      Pages: 1-6

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Comparison of naturally accumulated radiation-doses between RTL, BTL, OSL, and IRSL using white minerals from archaeological burnt materials and usefulness of RTL-dating from quartz extracts

    • Author(s)
      T.Hashimoto.T.Yawata, M.Takano
    • Journal Title

      Geochemical J. (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Book] 科学で探る歴史-発光(ルミネッセンス)現象から歴史が見えてくる2005

    • Author(s)
      橋本哲夫
    • Publisher
      新潟大学ブックレット、新潟日報事業社(印刷中)
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Book] Historical Studies from Scientific Viewpoints-In the Case of Radiation-Induced Luminescence

    • Author(s)
      T.Hashimoto
    • Publisher
      Niigata Nippo Press Co, Ltd.(in press)
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] Tetsuo Hashirnoto: "Radiation-Induced Luminescence and Hydrogen Radical Formation Associated with Thermal Annealing Treatments on Feldspars"J.Radioanal.Nucl.Chem.. 255. 81-85 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Masato Takano: "Luminescence dosimetry of archaeological and ceramics sample using a single-aliquot regenerative-dose method"J.Radioanal.Nucl.Chem.. 255. 365-368 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takahiro Nakagawa: "Optically stimulate luminescence (OSL) and thermoluminescence (TL) properties of red TL (RTL) quartz using a new automated OSL/TL measuring system"J.Radioanal.Nucl.Chem.. 255. 355-358 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "Comparison of infrared spectrometric characteristics of Al-OH impurities and thermoluminescence patterns in natural quartz slices at temperature below 0℃"Radiat.Meas.. 37. 479-485 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Takahiro Nakagawa: "Sensitivity change of OSL and RTL signal from natural RTL quartz with annealing treatment"Radiat.Meas.. 37. 397-400 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "Imaging and measurement of red-infrared stimulated luminescence(R-IRSL) from feldspar samples"Ancient TL. 21. 1-6 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 馬淵久夫(編): "文化財科学の事典(ルミネッセンス法)"朝倉書店. 522(4) (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "Retrospective dosimetry at JCO using Luminescence from ceramics pieces and quartz grains"Advances in ESR Application. 51. 197-202 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "An automatic system for both red/blue thermoluminscence (TL) and optically stimulated luminescence (OSL) measurement"J. Nucl. Sci. Technol.. 39. 108-109 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "Color images of infrared stimulated luminescence (IRSL) from granite slices exposed with radiations"Ancient TL. 20. 10-18 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] 橋本哲夫: "顕微赤外分光法を用いた天然石英の赤外吸光度特性と放射線誘起ルミネッセンス"分析化学. 51. 527-532 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Takahiro Nakagawa: "Optically stimulated luminescence (OSL) and thermoluminescence (TL) prpperties of red TL(RTL) quartz using a new automated OSL/TL measuring"J. Radioanal. Nucl. Chem.. 255. 355-358 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Tetsuo Hashimoto: "Radiation-induced luminescence and hydrogen radical formation sassociated with thermal annealing treatments on feldspars"J. Radioanal. Nucl. Chem.. 255. 81-85 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] 橋本哲夫(共著): "ルミネッセンス法:文化財科学の辞典"朝倉書店(印刷中).

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2016-04-21  

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