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Development of STM combined with synchrotron-radiation light source and its application to elemental analysis and spin observation

Research Project

Project/Area Number 14350016
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 表面界面物性
Research InstitutionThe University of Tokyo

Principal Investigator

HASEGAWA Yukio  The University of Tokyo, Institute for Solid State Physics, Associate Professor, 物性研究所, 助教授 (80252493)

Co-Investigator(Kenkyū-buntansha) OKUDA Aichi  The University of Tokyo, Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (80313120)
KINOSHITA Toyohiko  The University of Tokyo, Institute for Solid State Physics, Associate Professor, 物性研究所, 助教授 (60202040)
EGUCHI Toyoaki  The University of Tokyo, Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (70308196)
Project Period (FY) 2002 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥15,100,000 (Direct Cost: ¥15,100,000)
Fiscal Year 2003: ¥5,300,000 (Direct Cost: ¥5,300,000)
Fiscal Year 2002: ¥9,800,000 (Direct Cost: ¥9,800,000)
Keywordsscanning tunneling microscope / core level excitation / synchrotron radiation / elemental analysis
Research Abstract

We have developed an ultrahigh vacuum (UHV) STM system with which we can take atomically resolved STM images under an Iiradiation of synchrotron radiation light source. In order to do that, we designed an anti-vibration system including a vibration-isolation table which can be fitted in a narrow space of beamline. Since sites of beamlines in synchrotron-radiation light source are usually quite noisy electrically and mechanically, which is completely inappropriate for STM, we needed to consider carefully to avoid the noises to disturb the operation of STM, and successfully took atomically resolved STM images of the Si(111)7x7 surface under the irradiation.
We also succeeded in taking adsorption spectra of the sample element by using the probe tip as a detector; it was found that the photoinduced current increases when the irradiated light energy is above 101eV, an adsorption edge of Si 2p, demonstrating a possibility that the STM tip can detect photoelectron emitted from core states of sample. Compared with the previous work done with a X-ray tube, the photoinduced current by the synchrotron is larger by a factor of more than 100. High intensity of the light and tunability of a light energy to that of a high adsorption crosssection are the main reasons for the high detection.
After an modificatIon of the measurement system, we could also measure the photoinduced current quantitatively. From the quantitative measurement we characterized a spatial resolution of this elemental detection method by using a sample with a mixture of Au-induced 5x2 and Si7x7 surfaces and a Si substrate on which 2-micron size aluminum dots are regularly arranged. We also developed a method to focus the detection area on the tip for improving the spatial resolution by coating the tip with an insulating polymer and found successfully working.

Report

(3 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • Research Products

    (3 results)

All Other

All Publications (3 results)

  • [Publications] T.Matsushima et al.: "Development and trial measurement of synchrotron-radiation-light- illuminated scanning-tunneling-microscope"Review of Scientific Instruments. 75,6月号(印刷中). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Matsushima et al.: "Development and trial measurement of synchrotron-radiation-light-illuminated scanning-tunneling-microscope"Review of Scientific Instruments. (in press). 75 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Matsushima: "Development and trial measurement of synchrotron-radiation- light-illuminated scanning-tunneling-microscope"Review of Scientific Instruments. 75,5月号(掲載予定). (2004)

    • Related Report
      2003 Annual Research Report

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Published: 2002-04-01   Modified: 2018-02-02  

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