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Development of the evaluation method of radioactivity in materials obtained from garious accelerator facilities

Research Project

Project/Area Number 14380240
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionHigh Energy Accerelator Research Organization (2004)
The High Energy Accelerator Research Organization (2002-2003)

Principal Investigator

SHIBATA Tokushi  High Energy Accerelator Research Organization, Radiation Science Center, Prfesssor, 放射線科学センター, 教授 (80028224)

Co-Investigator(Kenkyū-buntansha) MASUMOTO Kazuyoshi  High Energy Accerelator Research Organization, Radiation Science Center, Assistant Professor, 放射線科学センター, 助教授 (60124624)
MIURA Taichi  High Energy Accerelator Research Organization, J-PARK Project Office, Assistant Professor, 大強度陽子加速器計画推進部, 助教授 (80209717)
NUMAJIRI Masaharu  High Energy Accerelator Research Organization, Radiation Science Center, Assistant, 放射線科学センター, 助手 (20189385)
MATSUMURA Hiroshi  High Energy Accerelator Research Organization, Radiation Science Center, Asastart, 放射線科学センター, 助手 (30328661)
HIRAYAMA Hideo  High Energy Accerelator Research Organization, Radiation Science Center, Proffesor, 放射線科学センター, 教授 (00044785)
伴 秀一  高エネルギー加速器研究機構, 放射線科学センター, 教授 (70141976)
Project Period (FY) 2002 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥12,300,000 (Direct Cost: ¥12,300,000)
Fiscal Year 2004: ¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2003: ¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2002: ¥5,900,000 (Direct Cost: ¥5,900,000)
KeywordsAccelerator / Activated Materials / Clearance / Radioactivity / AMS / Concrete / Chlorine-36 / Tritium / 加速器 / 塩素-36 / EGS-4
Research Abstract

Reccently, the clearance level has been in the spotlight for the safety release from the facilities to environment. As there were only few data on activation in the case of accelerator facilities, it is very important to develop the evaluation method of various radionuclides observed in activated materials on accelerator facilities. In this work, we focused on the development of analytical technique of tritium and chroline-26, which are very difficult to determine. We adopted the IR fumace for tritium separation This method can be characterized as rapid, simple and quantitative separation of tritium form concrete samples. To determine chlorine-36, we adopted AMS method after purification of chlorine from concrete samples. It was found that this method is very high sensitive and the data of chlorine-36 are very useful to measure the integrated neutron fluence emitted from accelerator facility. Then, we analyzed the concrete samples obtained from various accelerator facilities, because the concrete is used for the structure material in the facility and their volumes are very large. It was found that the major source of activation is thermal neutrons seconarily emitted from accelerators. The maximum yield of thermal neutron capture reaction was at the depth of about 10km from the surface.
The second work was the study of the activation induced by high energy neutron reactions. We constructed tine imadiation facility of neutron produced from the thick tungsten target bombarded by 500MeV proton Neutron flux was changed exponentially in the concrete shield, but the spectra did not change thoughout the shield Not only low energy neutron reaction but also spallation reaction induced by high energy neutron observed in the various target materials were analyzed.

Report

(4 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • 2002 Annual Research Report
  • Research Products

    (24 results)

All 2004 Other

All Journal Article (16 results) Publications (8 results)

  • [Journal Article] Tritium activity induced in the accelerator building and its correlation to radioactivity of γ-nuclides2004

    • Author(s)
      Q.Wang, T.Shibata et al.
    • Journal Title

      J.Radioanal.Nucl.Chem. 262

      Pages: 587-592

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] KENS shielding experiment(1) : Establishment of high energy neutron irradiation facility and measurement of neutron attenuation through 4m concrete2004

    • Author(s)
      N.Nakao, K.Masumoto et al.
    • Journal Title

      J.Nucl.Sci.Technol. Suppl.4

      Pages: 22-25

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] KENS shielding experiment(1) : Measurement of neutron spatial distribution inside the concrete shield using activation foil and imagine plate technique2004

    • Author(s)
      Q.Wang, K.Masumoto et al.
    • Journal Title

      J.Nucl.Sci.Technol. Suppl.4

      Pages: 26-29

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Study of Radionuclides Induced in Low-activation Concrete Using the 12-GeGeV Proton Synchrotron Accelerator at KEK2004

    • Author(s)
      K.Saito, T.Miura et al.
    • Journal Title

      J.Nucl.Sci.Technol. Suppl.4

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Tritium activity induced in the accelerator building and its correlation to radioactivity of γ-nuclides2004

    • Author(s)
      Q.Wang, T.Shibata et al.
    • Journal Title

      J. Radioanal. Nucl. Chem. 262

      Pages: 587-592

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] KENS shielding experiment(1) : Establishment of high energy neutron irradiation facility and measurement of neutron attenuation through 4m concrete2004

    • Author(s)
      N.Nakao, K.Masumoto et al.
    • Journal Title

      J. Nucl. Sci. Technol Suppl.4

      Pages: 22-25

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] KENS shielding experiment(2) : Measurement of neutron spatial distribution inside the concrete shield using activation foil and imaging plate technique2004

    • Author(s)
      Q.Wang, K.Masumoto et al.
    • Journal Title

      J. Nucl. Sci. Technol Suppl.4

      Pages: 26-29

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Study of Radionuclides Induced in Low-activation Concrete Using the 12-GeGeV Proton Synchrotron Accelerator at KEK2004

    • Author(s)
      K.Saito, T.Miura et al.
    • Journal Title

      J. Nucl. Sci. Technol Suppl.4

      Pages: 78-81

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] KENS shielding experiment(1) : Measurement of neutron spatial distribution in side the concrete shield using activation foil and imaging plate technique2004

    • Author(s)
      Q.Wang, K.Masumoto et al.
    • Journal Title

      J.Nucl.Sci.Technol. Suppl.4

      Pages: 26-29

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Study of Radionuclides Induced in Low-activation Concrete Using the 12-Ge GeV Proton Synchrotron Accelerator at KEK2004

    • Author(s)
      K.Saito, T.Miura et al.
    • Journal Title

      J.Nucl.Sci.Technol. Suppl.4

      Pages: 78-81

    • Related Report
      2004 Annual Research Report
  • [Journal Article] AMS Analysis of 36Cl Induced in Concrete of Accelerator Facilities

    • Author(s)
      K.Bessho, H.Matsumura et al.
    • Journal Title

      Radiochimica Acta In press

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Target dependence of beryllium fragment production in neutron- and alpha-induced nuclear reactions at intermediate energies

    • Author(s)
      H.Matsumura, K.Masumoto et al.
    • Journal Title

      Radiochimica Acta In press

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] AMS Analysis of 36Cl Induced in Concrete of Accelerator Facilities

    • Author(s)
      K.Bessho, H.Matsumura et al.
    • Journal Title

      Radiochimica Acta (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Target dependence of beryllium fragment production in neutron- and alpha-induced nuclear reactions at intermediate energies

    • Author(s)
      H.Matsumura K.Masumoto et al.
    • Journal Title

      Radiochimica Acta (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] AMS Analysis of 36Cl Induced in Concrete of Accelerator Facilities

    • Author(s)
      K.Bessho, H.Matsumura et al.
    • Journal Title

      Radiochimica Acta (In press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Target dependence of beryllium fragment production in neutron- and alpha-induced nuclear reactions at intermediate energies

    • Author(s)
      H.Matsumura, K.Masumoto et al.
    • Journal Title

      Radiochimica Acta (In press)

    • Related Report
      2004 Annual Research Report
  • [Publications] K.Masumoto, A.Toyoda, K.Eda, Y.Izumi, T.Shibata: "Evakuation of radioactivity induced in the accelerator building and its application to decontamination work"J.Radioanal.Nucl.Chem.. 255. 465-469 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Numajiri, K.Masumoto, T.Miura, Y.Oki, T.Suzuki, K.Kondo: "Production cross sections of C-14 in aluminium by nuclear spallation"J.Radioanal.Nucl.Chem.. 255. 481-483 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Miura, K.Bessho, S.Ishihama, N.Ohtsuka: "Migration of radionuclides induced in the soil below the 12 Gev proton accelerator facility at KEK"J.Radioanal.Nucl.Chem.. 255. 543-546 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Masumoto, A.Toyoda, K.Eda, T.Ishihara: "Measurement of the spatial distribution of neutrons in an accelerator room by the combination of activation detectors and an imaging plate"Radiation. Safety Management. 1. 12-16 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Masumoto, A.Toyoda, K.Eda, Y.Izumi, T.Shibata: "Evaluation of radioactivity induced in the acceleraotor building and its application to decontamination work"J.Radioanalytical and Nuclear Chemistry. 255. 465-469 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Numajiri, K.Masumoto, T.Miura, Y.Oki, T.Suzuki, K.Kondo: "Production cross sections of 14C in aluminum by nuclear spallation"J.Radioanalytical and Nuclear Chemistry. 255. 481-483 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Miura, K.Bessho, S.Ishihama, N.Ohtsuka: "Migration of radionuclides induced in the soil below the 12 GeV proton accelerator facility at KEK"J.Radioanalytical and Nuclear Chemistry. 255. 543-546 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Masumoto, A.Toyoda, K.Eda, T.Ishihara: "Measurement of the spatial distribution of nutrons in an accelerator room by the combination of activation detectors and an imaging plate"Radiation Safety Managcment. 1. 12-16 (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2016-04-21  

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