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Study of size dependence of optical response due to nanoscale spatial structure of the response field

Research Project

Project/Area Number 14540301
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionOsaka University

Principal Investigator

ISHIHARA Hajime  Osaka University, Graduate School of Engineering Science, Associate Professor, 基礎工学研究科, 助教授 (60273611)

Co-Investigator(Kenkyū-buntansha) ISU Toshiro  Mitsubishi electric Corp.Advanced Technology R&D center, Researcher, 先端技術総合研究所, 専任(研究職)
CHO Kikuo  Osaka University, Graduate School of Engineering Science, Professor, 基礎工学研究科, 教授 (60013489)
Project Period (FY) 2002 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2003: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 2002: ¥2,600,000 (Direct Cost: ¥2,600,000)
KeywordsNanostructures / Excitons / Polaritons / Nonlinear optical response / Ultrafast response / Thin film / GaAs / Nonlocal response / 非線系応答 / 内部電場 / ナノ空間構造 / 螺旋 / 非線形応答 / 光双安定
Research Abstract

(1) We have theoretically clarified the mode structure of the coupled system of the radiation and the excitons confined in a thin film. The eigenenergies of the respective states include the negative shift at thin region, but they jump to the energies of the upper polaritons at a particular thickness for each state. If the resonant enhancement of the components of internal field associated with the respective states occurs before these jumps, the large nonlinear response appears. For the thicker case, the radiative decay constant becomes very large for the higher levels including the non-dipole type excitonic states.
(2) By the time-resolved reflectance measurement of the GaAs multiple layers, we have verified that the radiative decay rate increases in proportion to the number of GaAs layers as predicted in the theory.
(3) We have found the optical bistablity in nanoscale thinflim due to the nanoscale spatial structure of the internal field, and the novel photofunctions due to the nanoscale polarization orientation configurations.

Report

(3 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • Research Products

    (24 results)

All Other

All Publications (24 results)

  • [Publications] H.Ishihara: "Ultra Fast Radiative Decay of Spatially Extended Non-dipole Type Excitonic State"phys.stat.sol.(a). 190. 849-853 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Ultra fine analysis of linear response of confined excitons in GaAs nano-layers"Institute of Physics Conference Series. 170. 467-472 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality induced large degenerate-four-wave mixing of spatially extended non-dipole type excitonic state"Phys.Rev.Lett. 89. 017402-1-017402-4 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality-induced multiple resonance in nonlinear optical process"Nonlinear Optics. 29. 663-669 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality induced anomalous input-intensity dependence of optical response for weakly confined excitons in a ultrathin film"Phys.Rev.B. 67. 113302-1-113302-4 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Isu: "Ultrafast and large nonlinear optical response of excitons weakly confined in a semiconductor thin film"SPIE Proceedings Series. 4992. 165-173 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Anomalous mode structure of a radiation - exciton coupled system beyond the long-wavelength approximation regime"Journal of Luminescence. 108. 343-346 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Anomalous size dependence of optical nonlinearities due to the excitonic coherence, Journal of Physics : Condensed Matter"Journal of Physics : Condensed Matter. 16. R247-R273 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Syouji: "Interchange of quantum states of confined excitons caused by radiative corrections in CuCl films"Phys.Rev.Lett. (in press). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Ultra Fast Radiative Decay of Spatially Extended Non-dipole Type Excitonic State"phys.stat.sol.(a). Vol.190. 849-853 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Ultra fine analysis of linear response of confined excitons in GaAs nano-layers"Institute of Physics Conference Series Number 170 "Compound Semiconductor 2001", (edited by Y.Arakawa, Y.Hirayama, K.Kishino, H.Yamaguchi) (IOP publishing Ltd,2002). 467-472

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality induced large degenerate-four-wave mixing of spatially extended non-dipole type excitonic state in GaAs thin layer"Phys.Rev.Lett.. Vol.89. 017402-(1-4) (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality-induced multiple resonance in nonlinear optical process, Proc.in 5thlnternational Conference on Excitonic Processes in Condensed Matter"Nonlinear Optics. Vol.29. 663-669 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocality induced anomalous input-intensity dependence of optical response for weakly confined excitons in a ultrathin film"Phys.Rev.B. Vol.67. 113302(1-4) (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Isu: "Ultrafast and large nonlinear optical response of excitons weakly confined in a semiconductor thin film"Proceedings of SPIIE, Ultrafast Phenomena in Semiconductors VII. (San Jose,2003)(SPIE Proceedings Series vol 4992). 165-173

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Anomalous mode structure of a radiation-exciton coupled system beyond the long-wavelength approximation regime"Journal of Luminescence. Vol.108. 343-346 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Anomalous size dependence of optical nonlinearities due to the excitonic coherence"Journal of Physics : Condensed Matter. Vol.1. 247-273 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Syouji: "Interchange of quantum states of confined excitons caused by radiative corrections in CuCl films"Phys.Rev.Lett. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Ishihara: "Anomalous mode structure of a radiation-exciton coupled system beyond the long-wavelength approximation regime"Journal of Luminescence. (in press). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Ishihara: "Drastic control of the radiative lifetime of nondipole-type excitons by manipulating the spatial structure of the radiation field"IQEC Technical Digest. (in press). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Ishihara: "Anomalous size dependence of optical nonlinearities due to the excitonic coherence"Journal of Physics : Condensed Matter. Vol.16. R247-R273 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Ishihara: "Nonlocality-induced multiple resonance in nonlinear optical process"Nonlinear Optics. 29. 663-669 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Ishihara: "Nonlocality induced anomalous input-intensity dependence of optical response for weakly confined excitons in a ultrathin film"Physical Review B. 67. 113302/1-113302/4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Isu: "Ultrafast and large nonlinear optical response of excitons weakly confined in a semiconductor thin film"Proceedings of SPIE, Ultrafast Phenomena in Semiconductors VII. (in press). (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2020-05-15  

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