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STUDY ON EXCESS HEAT PRODUCTION FROM DEUTERATED METAL-ELECTRODE DURING DISCHARGE IN GAS AND ON ELEMENTS PRODUCTION AT ELECTRODE SURFACE

Research Project

Project/Area Number 14550255
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 電力工学・電気機器工学
Research InstitutionIWATE UNIVERSITY

Principal Investigator

YAMADA Hiroshi  IWATE UNIVERSITY, ELECTRICAL AND ELECTRONIC ENGINEERING, PROFESSOR, 工学部, 教授 (60125482)

Co-Investigator(Kenkyū-buntansha) NARITA Shinya  IWATE UNIVERSITY, ELECTRICAL AND ELECTRONIC ENGINEERING, SENIOR ASSISTANT, 工学部, 助手 (80322965)
Project Period (FY) 2002 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2003: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2002: ¥2,000,000 (Direct Cost: ¥2,000,000)
KeywordsDeuterium / Palladium / Excess heat / Loading of hydrogen / Glow discharge / Transmutation / γ-ray measurement / TOF-SIMS / バラジウム
Research Abstract

DC discharge experiment was performed to measure gamma-ray emitted from the discharge test cell using deuterated and hydrated palladium foil cathodes in deuterium and hydrogen gas, respectively. Anomalous 5 gamma emission peaks of 57-228 keV in energy spectrum were rarely observed during DC glow-like discharge for 30-90 minutes for deuterium system at latm. No such anomalous gamma ray was detected for hydrogen system, which indicates that the gamma emission was induced by the nuclear reaction related to deuterium. However, anomalous gamma ray with energy more than 300 keV was observed in two runs for hydrogen system at latm. The palladium foil after DC discharge was analyzed by secondary ion mass spectroscopy (TOF-SIMS), which revealed considerably increase in the count intensity corresponding to several metal elements and barium on the palladium surface. Furthermore, the TOF-SIMS has shown the change in natural isotopic ratio of barium, potassium for hydrogen system and magnesium for deuterium system after the DC discharge experiment.
The controlled out-diffusion method was employed to induce a nuclear reaction in a palladium plate with a gold film. The time-resolved mass spectra for palladium hydride daring the out-diffusion experiment revealed increase in ion currents corresponding to mass number 2, 3 and 4, which may be correspond to deuterium, tritium and helium, respectively,. Anomalous increase in temperature of the palladium hydride was observed during the experiment. Initial large increase in temperature of the sample by Joule heating and enough evacuation of the test chamber were required to induce the anomalous increase in temperature of the sample at next stage. It seems that non-uniform flow of protons in the palladium bulk during the out-diffusion process was necessary to induce the anomalous excess heat generation. All the results suggest that a nuclear reaction possibly occurs for the deuterium system as well as hydrogen system.

Report

(3 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • Research Products

    (28 results)

All Other

All Publications (28 results)

  • [Publications] A.Arapi, H.Yamada et al.: "New Element Production on/in Deuteratd and Hydrated Palladium Electrode by DC Glow Discharge"Jpn.J.Appl.Phys.. 41. L1181-L1183 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Narita, H.Yamada et al.: "Gamma Ray Detection in DC Glowlike Discharge with Deuterated Palladium Electrode"Jpn.J.Appl.Phys.. 42. L1185-L1187 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ohmori, S.Narita H.Yamada et al.: "Enrichment of ^<41>K isotope in potassium formed on and in a rhenium electrode during plasma electrolysis in K_2CO_3/H_2O and K_2CO_3/D_2O solutions"Journal of Applied Electrochemistry. 33. 643-646 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Narita, H.Yamada et al.: "Anomalous Heat Evolution for Palladium Hydride in Controlled Gas Out-diffusion"Proceedings of the 9^<th> International Conference on Cold Fusion. 280-283 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Yamada, S.Narita, et al.: "Production of Ba and Several Anomalous Elements in Pd under Light Water Electrolysis"Proceedings of the 9^<th> International Conference on Cold Fusion. 420-423 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Yamada, S.Narita et al.: "Elemental Analysis on Pd-foil after Hydrogen Permeation at Room Temperature by TOF-SIMS"Proceedings of 5^<th> Meeting of Japan CF Research Society. 69-73 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Arapi, H.Yamada et al.: "New Element Production on/in Deuteratd and Hydrated Palladium Electrode by DC Glow Discharge"Jpn.J.Appl.Phys.. Vol.41. L1182-L1183 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] N.Tanaka, S.Narita, H.Yamada et al.: "Observation of Heat Evolution with Palladium Hydride in the Evacuated Chamber"Proceedings of 4th Meeting of Japan CF Research Society. 46-49 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Naoki SATO, Shinya NARITA, Hiroshi YAMADA et al.: "Gamma Ray Measurement and Surface Analysis on Deuterated and Hydrated Palladium Electrode under DC Glow-like Discharge"Proceedings of 4th Meeting of Japan CF Research Society. 50-53 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Narita, H.Yamada et al.: "Gamma Ray Detection in DC Glowlike Discharge with Deuterated Palladium Electrode"Jpn.J.Appl.Phys.. Vol.42. L1185-L1187 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ohmori, S.Narita, H.Yamada et al.: "Enrichment of ^<41>K isotope in potassium formed on and in a rhenium electrode during plasma electrolysis in K_2CO_3/H_2O and K_2CO_3/D_2O solutions"Journal of Applied Electrochemistry. Vol.33. 643-646 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Arapi, S.Narita, H.Yamada et al.: "Experimental Observation of the New Elements Production in the Deuterated and/or Hydride Palladium Electrodes, Exposed to the Low Energy DC Glow Discharge"Proceedings of 9th International Conference on Cold Fusion. 1-4 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Narita, H.Yamada et al.: "Anomalous Heat Evolution for Palladium Hydride in Controlled Gas Out-diffusion"Proceedings of 9th International Conference on Cold Fusion. 280-283 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Yamada, S.Narita et al.: "Production of Ba and Several Anomalous Elements in Pd under Light Water Electrolysis"Proceedings of 9th International Conference on Cold Fusion. 420-423 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] S.Narita, H.Yamada et al.: "Observation of Nuclear Reaction in Glow Discharge Experiment Using Deuterated Palladium Electrode"Proceedings of 5th Meeting of Japan CF Research Society. 14-18 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] H.Yamada, S.Narita et al.: "Elemental Analysis on Pd-foil after Hydrogen Permeation at Room Temperature by TOF-SIMS"Proceedings of 5th Meeting of Japan CF Research Society. 69-73 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Ohmori, S.Narita, H.Yamada et al.: "Enrichment of ^<41>K isotope in potassium formed on and in a rhenium electrode during plasma electrolysis in K_2CO_3/H_2O and K_2CO_3/D_2O solutions"Journal of Applied Electrochemistry. 33. 643-646 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Narita, H.Yamada et al.: "Gamma Ray Detection in DC Glowlike Discharge with Deuterated Palladium Electrode"Jpn.J.Appl.Phys.. 42. L1185-L1187 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Arapi, S.Narita, H.Yamada et al.: "Experimental Observation of New Elements Production in Deuterated and/or Hydride Pd Electrodes, Exposed to Low Energy DC Glow Dischar"Proceedings of the 9^<th> International Conference on Cold Fusion. 1-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Narita, H.Yamada et al.: "Anomalous Heat Evolution for Palladium Hydride in Controlled Gas Out-diffusion"Proceedings of the 9^<th> International Conference on Cold Fusion. 280-283 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Ohmori, H.Yamada, S.Narita et al.: "Excess Energy and Anomalous Concentration of ^<41>K Isotopes in K Formed on/in a Re Electrode during the Plasma Electrolysis in K_2CO_3 Solution"Proceedings of the 9^<th> International Conference on Cold Fusion. 284-287 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Yamada, S.Narita et al.: "Production of Ba and Several Anomalous Elements in Pd under Light Water Electrolysis"Proceedings of the 9^<th> International Conference on Cold Fusion. 420-423 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Arapi, H.Yamada et al.: "New Element Production on/in Deuterated and Hydrated Palladium Electrodes by DC Glow Discharge"Jpn. J. Appl. Phys.. 401・10B. L1181-L1183 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sato, S.Narita, H.Yamada et al.: "Analysis of Production Elements on Pd Surface after Light and Heavy Water Electrolysis"Proceedings of the 4^<th> Meeting of Japan CF Research Society. 9-12 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Onodera, S.Narita, H.Yamada et al.: "Analysis of Nuclear Products in Hydrogen Penetration through Palladium"Proceedings of the 4^<th> Meeting of Japan CF Research Society. 42-45 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] N.Tanaka, S.Narita, H.Yamada et al.: "Observation of Heat Evolution with Palladium Hydride in the Evacuated Chamber"Proceedings of the 4^<th> Meeting of Japan CF Research Society. 46-49 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] Naoki Sato, Shinya Narita, Hiroshi Yamada et al.: "Gamma Ray Measurement and Surface Analysis on Deuterated and Hydrated Palladium Electrode under DC Glow-like Discharge"Proceedings of the 4^<th> Meeting of Japan CF Research Society. 50-53 (2003)

    • Related Report
      2002 Annual Research Report
  • [Publications] 佐藤直樹, 成田晋也, 山田 弘他4名: "グロー放電法によるパラジウム中の低エネルギー核反応"電気学会・プラズマ研究会資料. PST-03-2. 7-11 (2003)

    • Related Report
      2002 Annual Research Report

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Published: 2002-04-01   Modified: 2016-04-21  

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