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Formation of multiple tunneling junctions of quantum dots using self-organized nanoholes and its application to spintronics

Research Project

Project/Area Number 15201034
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Microdevices/Nanodevices
Research InstitutionKansai University (2005)
Hiroshima University (2003-2004)

Principal Investigator

SHINGUBARA Shoso  Kansai University, Faculty of Engineering, Professor, 工学部, 教授 (10231367)

Co-Investigator(Kenkyū-buntansha) IWABUCHI Shuichi  Nara Women's University, Physics, Professor, 理学部, 教授 (40294277)
WAKAYA Fujio  Osaka University, Ultimate Science research center, associate professor, 極限科学研究センター, 助教授 (60240454)
高萩 隆行  広島大学, 大学院・先端物質科学研究科, 教授 (40271069)
坂上 弘之  広島大学, 大学院・先端物質科学研究科, 助手 (50221263)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥50,830,000 (Direct Cost: ¥39,100,000、Indirect Cost: ¥11,730,000)
Fiscal Year 2005: ¥7,800,000 (Direct Cost: ¥6,000,000、Indirect Cost: ¥1,800,000)
Fiscal Year 2004: ¥21,060,000 (Direct Cost: ¥16,200,000、Indirect Cost: ¥4,860,000)
Fiscal Year 2003: ¥21,970,000 (Direct Cost: ¥16,900,000、Indirect Cost: ¥5,070,000)
Keywordsporous alumina / nano ferromagnetic materials / quantum dot / tunnel junction / Coulomb blockade / spintronics / ナノホール / 強磁性 / エピタキシャル成長 / 強磁性体 / トンネリング / 単一電子効果
Research Abstract

We studied formation of ferromagnetic multiple tunneling junction using nano-ferromagnetic materials buried in porous alumina nanohole array and its conduction properties in aiming at new spintronics devices. For filling of ferromagnetic materials in nanoholes, we used pulsed-DC electroplating of Ni or Co, and found that ferromagnetic column diameter could be changed between 10 to 50nm by changing anodic voltage between 20 and 5V during anodic oxidation of aluminum. The unexpected problem for tunneling junction formation was that alumina thin wall between nanoholes (i.e. between nanomagnets) are too leaky even after annealing. The conduction mechanisms within alumina layer was Pool-Frenkel conduction derived from vacancies in alumina. Thus it is essential to improve quality of tunneling barrier layer, and further study such as plasma or radical oxidation would important. In order to improve switching properties of ferromagnetic nanodots, we tried to improve crystalline structure of electrodeposited materials, because they were polycrystalline and difficult to align crystalline orientation. Then we tried to remove bottom amorphous alumina layer that existed at the nanohole bottom, and succeeded in epitaxial growth of metal nanodot array on Si (100) substrate with adequate cleaning of Si surface after annealing in vacuum.
From theoretical approach, we derived analytical formalisms of tunneling conduction currents of CSET devices that was a fundamental structure to control Coulomb blockade, by taking co-tunneling effect into account. Furthermore, we expanded this formalism in order to treat with CSET and electrode systems altogether using non-equilibrium Green functions, and succeeded in developing the method to estimate an optimum condition to increase TMR (tunneling magnetoresistance) ratio.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (34 results)

All 2006 2005 2004 2003 Other

All Journal Article (24 results) Patent(Industrial Property Rights) (3 results) Publications (7 results)

  • [Journal Article] Epitaxial growth of Cu nanodot arrays using an AAO template on a Si substrate2006

    • Author(s)
      T.Shimizu, M.Nagayanagi, S.Shingubara
    • Journal Title

      Electrochemical and Solid-State Letters 9・4

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Epitaxial growth of Cu nanodot arrays using an AAO template on a Si substrate2006

    • Author(s)
      T.Shimnizu, M.Nagayanagi, S.Shingubara
    • Journal Title

      Electrochemical and Solid-State Letters Vol.9-4

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Epitaxial growth of Cu nanodot arrays using an AAO template on a Si substrate2006

    • Author(s)
      T.Shimnizu, M.Nagayanagi, S.Shingubara
    • Journal Title

      Electrochemical and Solid-State Letters 9・4

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Fabrication of Carbon Nanotube and Nanorod Arrays Using Nanoporous Template2005

    • Author(s)
      S.Huang, T.Shimizu, H.Sakaue, S.Shingubara, T.Takahagi
    • Journal Title

      Japanese Journal of Applied Physics 44-7A

      Pages: 5289-5291

    • NAID

      10016610107

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Transport Properties of Pt Nanowires Fabricated by Beam-Induced Deposition2005

    • Author(s)
      Y.Tsukatani, N.Yamasaki, K.Marukami, F.Wakaya, M.Takai
    • Journal Title

      Japanese Journal of Applied Physics 44

      Pages: 5683-5686

    • NAID

      10016677807

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Fabrication of Carbon Nanotube and Nanorod Arrays Using Nanoporous Template2005

    • Author(s)
      S.Huang, T.Shimizu, H.Sakaue, S.Shingubara, T.Takahagi
    • Journal Title

      Japanese Journal of Applied Physics Vol.44-7A

      Pages: 5289-5291

    • NAID

      10016610107

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Transport Properties of Pt Nanowires Fabricated by Beam-Induced Deposition2005

    • Author(s)
      Y.Tsukatani, N.Yamasaki, K.Murakami, F.Wakaya, M.Takai
    • Journal Title

      Japanese Journal of Applied Physics Vol.44

      Pages: 5683-5686

    • NAID

      10016677807

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Contact Resistance Reduction Using Vacuum Loadlock System and Plasma Dry Cleaning2005

    • Author(s)
      H.Miya, S.Shingubara, H.Sakaue, T.Takahagi
    • Journal Title

      Japanese J.of Appl.Phys. 44-6A

      Pages: 3860-3863

    • NAID

      10016441158

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Control of Self-Organization Conditions of Porous Alumina Film Using a Mixture of Oxalic Acid and Sulfuric Acid2004

    • Author(s)
      S.Shingubara, et al.
    • Journal Title

      Electrochemical and Solid-state Letters 7・3

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation of ultra high density ferromagnetic column arrays beyond 1 Tera/inchi^2 using porous alumina template2004

    • Author(s)
      T.Shimizu, S.Shingubara et al.
    • Journal Title

      Transaction of Magnetic Society of Japan 4

      Pages: 231-234

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Theory on the Coulomb blockade and current-voltage characteristics in Tomonaga-Luttinger liquid C-SET2004

    • Author(s)
      C.Tanaka, S.Iwabuchi, F.Wakaya
    • Journal Title

      Physica E-22

      Pages: 288-291

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Aspect Ratio Dependence of Magnetic Hysteresis Property of High Density Co Wire Array Buried In Porous Alumina Template2004

    • Author(s)
      S.Shingubara, et al.
    • Journal Title

      J. Magnetics and Magnetic Materials 272-276, Part 2

      Pages: 1598-1599

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Control of Self-Organization Conditions of Porous Alumina Film Using a Mixture of Oxalic Acid and Sulfuric Acid2004

    • Author(s)
      S.Shingubara, et al.
    • Journal Title

      Electrochemical and Solid-state Letters vol.7-3

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation of ultra high density ferromagnetic column arrays beyond 1 Tera/inch^2 using porous alumina template2004

    • Author(s)
      T.Shimizu, S.Shingubara et al.
    • Journal Title

      Transaction of Magnetic Society of Japan vol.4

      Pages: 231-234

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Theory on the Coulomb blockade and current-voltage characteristics in Tomonaga-Luttinger liquid C-SET2004

    • Author(s)
      C.Tanaka, S.Iwabuchi, F.Wakaya
    • Journal Title

      Physica vol.E-22

      Pages: 288-291

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Aspect Ratio Dependence of Magnetic Hysteresis Property of High Density Co Wire Array Buried In Porous Alumina Template2004

    • Author(s)
      S.Shingubara, et al.
    • Journal Title

      J.Magnetics and Magnetic Materials 272-276, Part2

      Pages: 1598-1599

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Control of Self-Organization Conditions of Porous Alumina Film Using a Mixture of Oxalic Acid and Sulfuric Acid2004

    • Author(s)
      S.Shingubara, et al.
    • Journal Title

      Electrochemical and Solid-state Letters 7・8

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Growth of cobalt nano column arrays directly on Si(111) substrate using AAO template2004

    • Author(s)
      T.Shimizu, S.Shingubara et al.
    • Journal Title

      International Confernce of Microprocess and Nanotechnology 2004

      Pages: 298-299

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Formation of Nanomaterials by Porous Alumina Template2003

    • Author(s)
      Shoso Shingubara
    • Journal Title

      J. of Nanoparticle Research 5

      Pages: 17-30

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation of Aluminum Nanodot Array by Combination of Nano-indentation and Anodic Oxidation of Aluminum2003

    • Author(s)
      Shoso Shingubara, et al.
    • Journal Title

      Surface Science 532-535

      Pages: 317-323

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Thickness Dependence of Hysteresis Property of Ferromagnetic Dot2003

    • Author(s)
      Guang Ri Wu, Shoso Shingubara, et al.
    • Journal Title

      Jpn. J. Appl. Phys 42

      Pages: 5038-5039

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation of Nanomaterials by Porous Alumina Template2003

    • Author(s)
      Shoso Shingubara
    • Journal Title

      J. of Nanoparticle Research vol.5

      Pages: 17-30

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation of Aluminum Nanodot Array by Combination of Nano-indentation and Anodic Oxidation of Aluminum2003

    • Author(s)
      Shoso Shingubara, et al.
    • Journal Title

      Surface Science vol.532-535

      Pages: 317-323

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Thickness Dependence of Hysteresis Property of Ferromagnetic Dot2003

    • Author(s)
      Guang Ri Wu, Shoso Shingubara, et al.
    • Journal Title

      Japanese Journal of Applied Physics vol.42

      Pages: 5038-5039

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 磁気記録媒体及びその製造方法2004

    • Inventor(s)
      新宮原正三, 清水智弘
    • Industrial Property Rights Holder
      新宮原正三
    • Filing Date
      2004-01-05
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 陽極酸化膜の製造方法2004

    • Inventor(s)
      新宮原正三, 清水智弘
    • Industrial Property Rights Holder
      新宮原正三
    • Filing Date
      2004-03-11
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 陽極酸化アルミナ膜を具備する構造体及びその製造方法並びにその利用2004

    • Inventor(s)
      新宮原正三, 清水智弘
    • Industrial Property Rights Holder
      独立行政法人広島大学
    • Filing Date
      2004-10-25
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Publications] Shoso Shingubara, et al.: "Aspect Ratio Dependence of Magnetic Hysteresis Property of High Density Co Wire Array Buried In Porous Alumina Template"J.Magnetics and Magnetic Materials. (accepted for publication). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Shoso Shingubara: "Formation of Nanomaterials by Porous Alumina Template"J.of Nanoparticle Research. 5. 17-30 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Shoso Shingubara, et al.: "Control of Self-Organization Conditions of Porous Alumina Film Using a Mixture of Oxalic Acid and Sulfuric Acid"Electrochemical and Solid-state Letters. 7. E15-E17 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Shoso Shingubara, et al.: "Formation of Aluminum Nanodot Array by Combination of Nano-indentation and Anodic Oxidation of Aluminum"Surface Science. 532-535. 317-323 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Guang Ri Wu, Shoso Shingubara, et al.: "Thickness Dependence of Hysteresis Property of Ferromagnetic Do"Jpn.J.Appl Phys. 42. 5038-5039 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] Chika Tanaka, Fujio Wakaya, Shuichi Iwabuchi: "Theory on the Coulomb Blockade and Current-Voltage Characteristics in Tomonaga-Luttinger Liquid C-SET"Physica E : Low-dimensional Systems and Nanostructures. (in press). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Shuichi Iwabuchi et al.: "Effect of Gate-Induced Charge on the Coulomb Blockade in Ultrasmall Double Tunnel Junctions"Phys.Rev.B. (accepted). (2004)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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