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Sub-10 attoseconds manipulation of quantum phases and single-molecule quantum computing

Research Project

Project/Area Number 15204034
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field 原子・分子・量子エレクトロニクス・プラズマ
Research InstitutionInstitute for Molecular Science (2004-2005)
Okazaki National Research Institutes (2003)

Principal Investigator

OHMORI Kenji  Institute for Molecular Science, Department of Electronic Structure, Professor, 電子構造研究系, 教授 (10241580)

Co-Investigator(Kenkyū-buntansha) KATSUKI Hiroyuki  Institute for Molecular Science, Department of Electronic Structure, Research Associate, 電子構造研究系, 助手 (10390642)
HOSAKA Kouichi  Institute for Molecular Science, Department of Electronic Structure, Guest Researcher, 電子構造研究系, 特別協力研究員 (00419855)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥43,420,000 (Direct Cost: ¥33,400,000、Indirect Cost: ¥10,020,000)
Fiscal Year 2005: ¥7,150,000 (Direct Cost: ¥5,500,000、Indirect Cost: ¥1,650,000)
Fiscal Year 2004: ¥7,150,000 (Direct Cost: ¥5,500,000、Indirect Cost: ¥1,650,000)
Fiscal Year 2003: ¥29,120,000 (Direct Cost: ¥22,400,000、Indirect Cost: ¥6,720,000)
Keywordswave packet / attosecond / quantum interference / coherent control / quantum information / quantum phase / molecule / quantum computer
Research Abstract

We have succeeded in controlling quantum interference of two vibrational wave-packets in a molecule almost completely, and in observing its temporal evolution in real time. In this real-time observation, we have demonstrated that the temporal evolution of a wave packet is sensitive to the relative phases among the vibrational eigenstates within the wave packet. By using our high-precision interferometric technique, it is possible to read and write a "population code" which is a population ratio among the vibrational eigenstates of a molecule. In the present study, we have demonstrated that the combination of the real-time observation and the population code can provide full quantum information of a wave packet. Moreover we have developed a novel technique to visualize quantum standing-waves (quantum ripples) generated transiently by the wave-packet interference with picometer and femtosecond spatiotemporal resolution. Very recently we have succeeded in tailoring such a visualized spatiotemporal Image (quantum fabric).
We have also succeeded in developing a molecular memory based on our advanced interferometric techniques. This molecular memory is a quantum memory where each vibrational eigenstate serves as a bit, and both amplitude and phase information can be read and written. The superposition of those vibrational eigenstates can be used as a qubit. Moreover we have developed quantum gate and algorithm to apply this molecular memory to quantum information processing. A series of these achievements indicates a possibility of molecule-based optical-phase memory and quantum computer.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (8 results)

All 2006 2004 Other

All Journal Article (6 results) Publications (2 results)

  • [Journal Article] Visualizing Picometric Quantum Ripples of Ultrafast Wave-Packet Interference2006

    • Author(s)
      H.Katsuki, H.Chiba, B.Girard, C.Meier, K.Ohmori
    • Journal Title

      Science 311

      Pages: 1589-1589

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Real-Time Observation of Phase-Controlled Molecular Wave-Packet Interference2006

    • Author(s)
      K.Ohmori, K.Katsuki, H.Chiba et al.
    • Journal Title

      Physical Review Letters 96

      Pages: 93002-93002

    • NAID

      120003781041

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Implementation of quantum gate operations in molecules with weak laser fields2006

    • Author(s)
      Y.Teranishi, Y.Ohtsuki, K.Hosaka, H.Chiba, H.Katsuki, K.Ohmori
    • Journal Title

      The Journal of Chemical Physics 124

      Pages: 114110-114110

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Real-Time Observation of Phase-Controlled Molecular Wave-Packet Interference2006

    • Author(s)
      K.Ohmori, H.Katsuki, H.Chiba, et al.
    • Journal Title

      Physical Review Letters 96

      Pages: 93002-93002

    • NAID

      120003781041

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] アト秒精度のコヒーレント制御-分子振動波束への応用-2004

    • Author(s)
      大森賢治
    • Journal Title

      日本物理学会誌 59

      Pages: 615-615

    • NAID

      110002069671

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Coherent Control with Attosecond Precision Applied to Vibrational Wave-Packets in Molecules2004

    • Author(s)
      K.Ohmori
    • Journal Title

      Butsuri (Monthly Journal of the Physical Society of Japan) 59

      Pages: 615-615

    • NAID

      110002069671

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Publications] Kenji Ohmori: "High precision molecular wave-packet interferometry with Hg-Ar dimers"Phys.Rev.Lett.. 91. 243003 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] E.I.Dashevskaya: "Energy dependence of the intramultiplet mixing cross section in Hg-N_2 collisions : conical intersection mechanism, indication at tunneling and interference"Phys.Chem.Chem.Phys.. 5. 1198-1204 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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