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Study of electronic inhomogeneity and superconductivity in high-Tc superconductors by scanning tunneling microscopy.

Research Project

Project/Area Number 15340107
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionTohoku University

Principal Investigator

KOBAYASHI Norio  Tohoku University, Institute for Materials Research, Professor, 金属材料研究所, 教授 (40111306)

Co-Investigator(Kenkyū-buntansha) NISHIZAKI Terukazu  Tohoku University, Institute for Materials Research, Research Associate, 金属材料研究所, 助手 (90261510)
YONEYAMA Naoki  Tohoku University, Institute for Materials Research, Research Associate, 金属材料研究所, 助手 (80312643)
KUDO Kazutaka  Tohoku University, Institute for Materials Research, Research Associate, 金属材料研究所, 助手 (40361175)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥16,400,000 (Direct Cost: ¥16,400,000)
Fiscal Year 2005: ¥2,800,000 (Direct Cost: ¥2,800,000)
Fiscal Year 2004: ¥5,400,000 (Direct Cost: ¥5,400,000)
Fiscal Year 2003: ¥8,200,000 (Direct Cost: ¥8,200,000)
KeywordsHigh-Tc oxide superconductor / Scanning tunneling Microscopy / Local electronic structure / Pseudogap / Vortex structure / Atomic image / impurity state / 銅酸化物超伝導体 / 電子状態 / YBa_2Cu_3O_y / Pb置換Bi2201 / 磁束状態 / 超伝導材料 / 渦糸状態 / 表面電子状態 / 不純物効果 / 低温物性実験
Research Abstract

The aim of this program is to reveal atomic-scale electronic structures of high-Tc oxide superconductors by scanning tunneling microscopy (STM/STS) and to investigate the relationship between the superconductivity and the characteristic electronic structure, such as granular structure composed of the superconducting and pseudogap regions. In this study, we have observed atomic-scale electronic structures of YBa2Cu3Oy (YBCO) and Bi2-xPbxSr2CuOy (Pbx-Bi2201) single crystals with various carrier concentrations as well as macroscopic superconducting properties.
1. YBa2Cu3Oy : (1) We have successfully prepared single crystals with different electronic coupling strength between adjacent CuO2 layers by controlling anneal conditions in nitrogen atmosphere and observed 2 to 3 dimensional transformation of the vortex system. (2) Effects of oxygen defects and impurities on the vortex structure and the electronic state have been studied macroscopically and microscopically. (3) One-dimensional elect … More ronic modulations on the BaO layer at low bias voltage have been observed along the Cu-O direction. These modulations are closely related to the electronic inhomogeneity induced by impurities and/or defects.
2. Bi2-xPbxSr2CuOy : (1) The temperature and carrier concentration dependences of the superconducting transition temperature Tc and the pseudogap formation temperature T^* have been studied for well prepared Pb substituted Bi2201 single crystals. (2) It has been clarified that there exist two types of pseudogap ; one is related to a precursor effect of superconductivity and another to a strong electron correlation. The latter exist even in the overdoped region. (3) In STM images measured at high bias-voltages above 300 mV, a clear two-dimensional atomic arrangement, which consists of Bi and Pb atoms, has been observed. On the other hand, at low bias-voltages below 150 mV, it has been found that a contrasting density forms into bright patches of 1-3 nm diameters. These results are consistent with the electronic granularity observed in Bi2212. Less

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (38 results)

All 2005 2004 2003 Other

All Journal Article (29 results) Book (3 results) Publications (6 results)

  • [Journal Article] Vortex Phase Diagram in Impurity Doped YBa2Cu3Oy Single Crystals2005

    • Author(s)
      T.Nishizaki
    • Journal Title

      Physica C 426-431

      Pages: 18-22

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Phase transition of the Josephson vortices in YBa2Cu3O7-delta single crystals with various oxygen deficiencies2005

    • Author(s)
      T.Naito
    • Journal Title

      Physica C 426-431

      Pages: 46-50

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Hole-doping and Magnetic-field Effects on the Pseudogap in Bi1.74Pb0.38Sr1.88CuO6+d Studied by the Out-of-Plane Resistivity2005

    • Author(s)
      K.Kudo
    • Journal Title

      Physica C 426-431

      Pages: 251-256

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Layered Charge-Density Waves with Nanoscale Coherence in YBa2Cu3O7-δ2005

    • Author(s)
      M.Maki
    • Journal Title

      Phys. Rev. B 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Vortex Matter in YBa2Cu3Oy Single Crystals Investigated by Scanning Tunneling Spectroscopy2005

    • Author(s)
      K.Shibata
    • Journal Title

      Phys. Rev. B 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Single-Crystal Growth and the Dependence on Hole Concentration and Magnetic Field of the Magnetic Ground State in the edge-Sharing CuO2 Chain System Ca2+xY2-xCu5O102005

    • Author(s)
      K.Kudo
    • Journal Title

      Phys. Rev. B 71

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Phase transition of the Josephson vortices in YBa2Cu3O7-d single crystals with various oxygen deficiencies2005

    • Author(s)
      T.Naito
    • Journal Title

      Physica C 426-431

      Pages: 46-50

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Layered Charge-Density Waves with Nanoscale Coherence in YBa2Cu3O7-δ2005

    • Author(s)
      M.Maki
    • Journal Title

      Phys.Rev.B 72

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Vortex Matter in YBa2Cu3Oy Single Crystals Investigated by Scanning Tunneling Spectroscopy2005

    • Author(s)
      K.Shibata
    • Journal Title

      Phys.Rev.B 72

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Single-Crystal Growth and the Dependence on Hole Concentration and Magnetic Field of the Magnetic Ground State in the edge-Sharing CuO2 Chain System Ca2+xY2-xCu5O102005

    • Author(s)
      K.Kudo
    • Journal Title

      Phys.Rev.B 71

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Hole-doping and Magnetic-field Effects on the Pseudogap in Bi1.74PbO.38Sr1.88CuO6+d Studied by the Out-of-Plane Resistivity2005

    • Author(s)
      K.Kudo
    • Journal Title

      Physica C 426-431

      Pages: 251-256

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Vortex State in YBa2Cu3Oy Crystals : Vortex Phase Diagram and Tunneling Spectroscopy in Magnetic Field2004

    • Author(s)
      N.Kobayashi
    • Journal Title

      Physica B 346-347

      Pages: 329-333

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Vortex Phase Transition under Tilted Magnetic Fields in 90-K YBa2Cu3O7-δ Single Crystals2004

    • Author(s)
      T.Naito
    • Journal Title

      Physica C 412-414

      Pages: 502-505

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Anomalous Vortex Liquid-to-Glass Transition Line in Twinned YBa2Cu3O7-δ2004

    • Author(s)
      T.Naito
    • Journal Title

      Phys. Rev. B 70

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Impurity Effect On the Electronic State of the Vortex Core in the Mixed State of YBa2Cu3Oy2004

    • Author(s)
      K.Kinoshita
    • Journal Title

      Physica C 412-414

      Pages: 530-534

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Anomalous Vortex Liquid-to-Glass Transition Line in Twinned YBa2Cu3O7-δ2004

    • Author(s)
      T.Naito
    • Journal Title

      Phys.Rev.B 70

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Substitution Effect by Deuterated Donors on Superconductivity in κ-(BEDT-TTF)2Cu[N(CN)2]Br2004

    • Author(s)
      N.Yoneyama
    • Journal Title

      J.Phys.Soc.Jpn 73

      Pages: 1434-1437

    • NAID

      210000104838

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Disorder Effect on the Vortex Pinning by the Cooling-Process Control in the Organic Superconductor κ-(BEDT-TTF)2Cu[N(CN)2]Br2004

    • Author(s)
      N.Yoneyama
    • Journal Title

      J.Phys.Soc.Jpn. 73

      Pages: 184-189

    • NAID

      210000104916

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Vortex Phase Transition and Oxygen Vacancy in YBa2Cu3Oy Single Crystals2003

    • Author(s)
      T.Nishizaki
    • Journal Title

      J. Low Temp. Phys 131

      Pages: 931-940

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Vortex Phase Diagram in Zn-Doped YBa2Cu3Oy Crystals2003

    • Author(s)
      N.Kobayashi
    • Journal Title

      J. Low Temp. Phys. 131

      Pages: 925-930

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Quasiparticle spectra and their spatial variation on YBa_2Cu_3O_y by scanning tunneling spectroscopy2003

    • Author(s)
      K.Shibata
    • Journal Title

      Physica C 388-389

      Pages: 277-278

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] LT-STM Observation of YBa2(Cu1-xZnx)3O7-δ Single Crystals2003

    • Author(s)
      M.Maki
    • Journal Title

      Physica C 388-389

      Pages: 279-280

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Shubnikov-de Haas Effect in Quantum Vortex Liquid State of the Organic Superconductor κ-(BEDT-TTF)2Cu(NCS)22003

    • Author(s)
      T.Sasaki
    • Journal Title

      Phys. Rev. B 67

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] YBa2Cu3Oy非双晶単結晶における渦糸体の物理2003

    • Author(s)
      西嵜照和
    • Journal Title

      固体物理 38

      Pages: 515-527

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Vortex Phase Transition and Oxygen Vacancy in YBa2Cu3Oy Single Crystals2003

    • Author(s)
      T.Nishizaki
    • Journal Title

      J.Low Temp.Phys. 131

      Pages: 931-940

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Vortex Phase Diagram in Zn-Doped YBa2Cu3Oy Crystals2003

    • Author(s)
      N.Kobayashi
    • Journal Title

      J.Low Temp.Phys. 131

      Pages: 925-930

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Quasiparticle spectra and their spatial variation on YBa_2Cu_3O_y by scanning tunneling spectroscopy2003

    • Author(s)
      K Shibata
    • Journal Title

      Physica C 388-389

      Pages: 277-278

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Shubnikov-de Haas Effect in Quantum Vortex Liquid State of the Organic Superconductor κ-(BEDT-TTF)2Cu(NCS)22003

    • Author(s)
      T.Sasaki
    • Journal Title

      Phys.Rev.B 67

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Vortex matter physics in untwinned YBa2Cu3Oy single crystals2003

    • Author(s)
      T.Nishizaki
    • Journal Title

      Kotai butsuri 38

      Pages: 515-527

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] Studies of High Temperature Superconductors2005

    • Author(s)
      T.Nishizaki
    • Publisher
      Nova Science Publishers, Inc.
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] Studiesdies of High Temperature Superconductors2005

    • Author(s)
      T.Nishizaki
    • Publisher
      Nova Science Publishers, Inc.
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Book] Vortex Matter Physics in YBa2Cu3Oy Single Crystals2005

    • Author(s)
      T.Nishizaki
    • Publisher
      Nova Science Publishers, Inc.
    • Related Report
      2005 Annual Research Report
  • [Publications] T.Nishizaki, K.Shibata, M.Maki, N.Kobayashi: "Vortex Phase Transition and Oxygen Vacancy in YBa2Cu3Oy Single Crystals"J.Low Temp.Phys.. 131. 931-940 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] N.Kobayashi, T.Sato, T.Nishizaki, K.Shibata.M.Maki, T.Sasaki: "Vortex Phase Diagram in Zn-Doped YBa2Cu3Oy Crystals"J.Low Temp.Phys.. 131. 925-930 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K Shibata, M Maki, T Nishizaki, N Kobayashi: "Quasiparticle spectra and their spatial variation on YBa_2Cu_3O_y by scanning tunneling spectroscopy"Physica C. 388・389. 277-278 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Maki, T.Nishizaki, N.Kobayashi: "LT-STM Observation of YBa2(Cu1-xZnx)3O7-δ Single Crystals"Physica C. 388・389. 279-280 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Sasaki, T.Fukuda, N.Yoneyama, N.Kobayashi: "Shubnikov-de Haas Effect in Quantum Vortex Liquid State of the Organic Superconductor κ-(BEDT-TTF)2Cu(NCS)2"Phys.Rev.B. 67. 144521(1-6) (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 西嵜照和, 小林典男: "YBa2Cu3Oy非双晶単結晶における渦糸体の物理"固体物理. 38. 515-527 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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