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Neutron Scattering Study of the One-dimensional Magnetic Anisotropy on the CuO_2 Plane of the Domain-controlled High T_c Superconductors

Research Project

Project/Area Number 15340109
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionThe University of Tokyo

Principal Investigator

HIROTA Kazuma  The University of Tokyo, Institute for Solid State Physics, Associate Professor, 物性研究所, 助教授 (90272012)

Co-Investigator(Kenkyū-buntansha) ASO Naofumi  The University of Tokyo, Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (40313118)
KIMURA Hiroyuki  Tohoku University, Institute of Multidisciplinary Research for Advanced Materials, Research Associate, 多元物質科学研究所, 助手 (50312658)
MATSUURA Masato  The University of Tokyo, Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (30376652)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥14,900,000 (Direct Cost: ¥14,900,000)
Fiscal Year 2005: ¥3,100,000 (Direct Cost: ¥3,100,000)
Fiscal Year 2004: ¥4,800,000 (Direct Cost: ¥4,800,000)
Fiscal Year 2003: ¥7,000,000 (Direct Cost: ¥7,000,000)
Keywordshigh T_c superconductivity / La_<2-x>Sr_xCuO_4 / Neutron scattering / One-dimensional spin modulation / Spin dynamics / Bi high T_c superconductors / Impurity effect / Bi_2Sr_<2-x>La_xCuO_6 / Bi_2Sr_2CaCu_2O_8 / Dewtinning / La_<2-x>Sr_XCuO_4
Research Abstract

Since it is difficult to grow large single crystals for highly anisotropic or domain-controlled high T_c superconductors, it is necessary to increase the effective volume by aligning multiple crystals to carry out neutron scattering. We thus have established a method to align many single crystals precisely and efficiently : Combination of a high-energy x-ray diffractometer and a CCD camera, as well as a supersensitive CCD camera with neutron scintillator have been developed. We have succeeded in obtaining the effective volume of 0.53cc by aligning six Bi2212 single crystals with a very high precision, which is about eight times as large as a typical sample volume in previous studies. We have been carrying out series of neutron scattering experiments at the Oak Ridge National Laboratory through the US-Japan cooperative program on neutron scattering to search for the magnetic excitation and the resonance peak.
To elucidate the relation between superconductivity and antiferromagnetic spin dynamics, we have performed a systematic inelastic neutron scattering concerning the suppression of T_c by impurities and the change of the spin excitations, using optimally doped La_<2-x>Sr_xCuO_4 single crystals with very small amount of impurities. We have focused upon the non-magnetic impurity Zn and the magnetic impurity Ni : Since the former suppresses T_c more effectively the latter, we expected to clarify how the magnetism is related to the T_c suppression mechanism by comparing both the systems. As to the Zn doped system, a novel in-gap state appears in the middle of the previously know spin gap while the overall spin dynamics does not change much. On the other hand, the spin dynamics of the Ni doped systems is renormalized to the lower energies as T_c is suppressed. It is now clear that the Zn and Ni doping effects on the superconductivity on the CuO_2 plane is qualitatively different.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (20 results)

All 2006 2005 2004 Other

All Journal Article (18 results) Publications (2 results)

  • [Journal Article] Stoner gap in the superconducting ferromagnet UGe_22006

    • Author(s)
      N.Aso, G.Motoyama, Y.Uwatoko, S.Ban, S.Nakamura, T.Nishioka, Y.Homma, Y.Shiokawa, K.Hirota, N.K.Sato
    • Journal Title

      Physical Review B 73

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spatial distribution of the B-site inhomogeneity in an as-grown Pb(In_<1/2>Nb_<1/2>)O_3 single crystal studied by a complementary use of X-ray and neutron scatterings2006

    • Author(s)
      K.Ohwada, K.Hirota, H.Terauchi, H.Ohwa, N.Yasuda
    • Journal Title

      Journal of the Physical Society of Japan 75

    • NAID

      110004086876

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Stoner gap in the superconducting ferromagnet UGe_22006

    • Author(s)
      Aso, N, Motoyama, G, Uwatoko, Y, Ban, S, Nakamura, S, Nishioka, T, Homma, Y, Shiokawa, Y, Hirota, K, Sato, NK
    • Journal Title

      PHYSICAL REVIEW B 73(5)

      Pages: 54512-54512

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Neutron diffraction study on the antiferromagnetic insulating ground state of β-Na_<0.33>V_2O_52005

    • Author(s)
      S.Nagai, M.Nishi, K.Kakurai, Y.Oohara, H.Yoshizawa, H.Kimura, Y.Noda, B.Greiner, T.Yamauchi, J.Yamamura, M.Isobe, Y.Ueda, K.Hirota
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 1297-1308

    • NAID

      110001979525

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spin-singlet ground state in two-dimensional S=1/2 frustrated square lattice : (CuCl)LaNb_2O_72005

    • Author(s)
      H.Kageyama, T.Kitano, N.Oba, M.Nishi, S.Nagai, K.Hirota, L.Biciu, J.B.Wiley, J.Yasuda, Y.Baba, Y.Ajiro, K.Yoshimura
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 1702-1705

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<17>O NMR study of the inhomogeneous electronic state in La_<2-x>Sr_xCuO_4 crystals^12005

    • Author(s)
      P.M.Singer, T.Imai, F.C.Chou, K.Hirota, M.Takaba, T.Kakeshita, H.Eisaki, S.Uchida
    • Journal Title

      Physical Review B 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Zn and Ni doping effects on the low-energy spin excitations in La_<1.85>Sr_<0.15>CuO_42005

    • Author(s)
      M.Kofu, H.Kimura, K.Hirota
    • Journal Title

      Physical Review B 72

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Neutron diffraction study on the antiferromagnetic insulating ground state of b-Na_<033>V_2O_52005

    • Author(s)
      S.Nagai, M.Nishi, K.Kakurai, Y.Oohara, H.Yoshizawa, H.Kimura, Y.Noda, B.Greiner, T.Yamauchi, J.Yamamura, M.Isobe, Y.Ueda, K.Hirota
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 1297-1308

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Spin-singlet ground state in two-dimensional S=1/2 frustrated square lattice : (CuCl)LaNb_2O_72005

    • Author(s)
      H.Kageyama, T.Kitano, N.Oba, M.Nishi, S.Nagai, K.Hirota, L.Viciu, J.B.Wiley, J.Yasuda, Y.Baba, Y.Ajiro, K.Yoshimura
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 1702-1705

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] ^<17>O NMR study of the inhomogeneous electronic state in La_<2-x>Sr_xCuO_4crystals'2005

    • Author(s)
      P.M.Singer, T.Imai, F.C.Chou, K.Hirota, M.Takaba, T.Kakeshita, H.Eisaki, S.Uchida
    • Journal Title

      Physical Review B 72

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Electronic excitations in hole-doped La_<1-x>Sr_xMnO_3 studied by resonant inelastic X-ray scattering2005

    • Author(s)
      Ishii, K, Inami, T, Ohwada, K, Kuzushita, K, Mizuki, J, Murakami, Y, Ishihara, S, Endoh, Y, Maekawa, S, Hirota, K, Moritomo, Y
    • Journal Title

      JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS 66(12)

      Pages: 2157-2162

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Hole concentration dependence of Mn e(g) orbital state in bilayer manganites studied by magnetic Compton profile measurement2005

    • Author(s)
      Koizumi, A, Nagao, T, Kakutani, Y, Hiraoka, N, Sakai, N, Arima, T, Hirota, K, Murakami, Y
    • Journal Title

      PHYSICAL REVIEW B 66(12)

      Pages: 2183-2191

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Zn and Ni doping effects on the low-energy spin excitations in La_<1.85>Sr_<0.15>CuO_42005

    • Author(s)
      Kofu, M, Kimura, H, Hirota, K
    • Journal Title

      PHYSICAL REVIEW B 72(6)

      Pages: 64502-64502

    • Related Report
      2005 Annual Research Report
  • [Journal Article] O-17 NMR study of the inhomogeneous electronic state in La_<2-x>Sr_xCuO_4 crystals2005

    • Author(s)
      Singer, PM, Imai, T, Chou, FC, Hirota, K, Takaba, M, Kakeshita, T, Eisaki, H, Uchida, S
    • Journal Title

      PHYSICAL REVIEW B 72(1)

      Pages: 14537-14537

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Neutron diffraction study on the antiferromagnetic insulating ground state of β-Na_<0.33>V_2O_52005

    • Author(s)
      Nagai, S, Nishi, M, Kakurai, K, Oohara, Y, Kimura, H, Yoshizawa, H, Noda, Y, Grenier, B, Yamauchi, T, Yamaura, J, Isobe, M, Ueda, Y, Hirota, K
    • Journal Title

      JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN 74(4)

      Pages: 1297-1308

    • NAID

      110001979525

    • Related Report
      2005 Annual Research Report
  • [Journal Article] d-f Coulomb and quadrupole-strain interactions in DyB_2C_2 observed by resonant x-ray scattering2005

    • Author(s)
      T.Matsumura, D.Okuyama, N.Oumi, K.Hirota, H.Nakao, Y.Murakami, Y.Wakabayashi
    • Journal Title

      PHYSICAL REVIEW B 71

      Pages: 12405-12405

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Resonant inelastic x-ray scattering study of the hole-doped manganites La_<1-x>Sr_xMnO_3 (x=0.2,0.4)2004

    • Author(s)
      K.Ishii, T.Inami, K.Ohwada, K.Kuzushita, J.Mizuki, Y.Murakami, S.Ishihara, Y.Endoh, S.Maekawa, K.Hirota, Y.Moritomo
    • Journal Title

      PHYSICAL REVIEW B 70

      Pages: 224437-224437

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Change in Mn 3d orbital state related to a metal-insulator transition in a bilayer manganite studied by magnetic Compton profile measurement2004

    • Author(s)
      A.Koizumi, T.Nagao, Y.Kakutani, N.Sakai, Hirota, Y.Murakami
    • Journal Title

      PHYSICAL REVIEW B 69

      Pages: 60401-60401

    • Related Report
      2004 Annual Research Report
  • [Publications] H.Kimura, M.Kofu, Y.Matsumoto, K.Hirota: "Novel in-gap spin state in Zn-doped La_<1.85>Sr_<0.15>CuO_4"Physical Review Letters. 91. 067002-1-067002-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Kubota, Y.Oohara, H.Yoshizawa, H.Fujioka, K.Hirota, Y.Moritomo, Y.Endoh: "Highly degenrate canted spin structure in bilayer manganite La_<1.1>Sr_<1.9>Mn_2O_7"Physical Review Letters. 91. 04702-1-04702-4 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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