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Investigation of magneto-electric optical effect

Research Project

Project/Area Number 15340112
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionThe University of Tokyo

Principal Investigator

TOKURA Yoshinori  The University of Tokyo, School of Engineering, Professor, 大学院・工学系研究科, 教授 (30143382)

Co-Investigator(Kenkyū-buntansha) MIYASAKA Shigeki  The University of Tokyo, School of Engineering, Research Associate, 大学院・工学系研究科, 助手 (70345106)
Project Period (FY) 2003 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥15,500,000 (Direct Cost: ¥15,500,000)
Fiscal Year 2004: ¥6,600,000 (Direct Cost: ¥6,600,000)
Fiscal Year 2003: ¥8,900,000 (Direct Cost: ¥8,900,000)
Keywordsmagneto-electric optical effect / magneto-chiral effect / breakdown of time reversal and space inversion symmetry / x-ray nonreciprocal directional dichroism / troidal moment / GaFeO3 / Fe3O4 / スピン軌道相互作用 / カイラリテイー
Research Abstract

We have investigated the new magneto-optical effects termed "magneto-electric optical effect" and "magneto-chiral effect". In these optical effects, the optical response of the depolarized light depends on the direction of the propagator vector. We studied the optical features in the single crystals of the ferrimagnet, GaFeO3, and spinel-type Fe3O4 in order to clarify the mechanism of the magneto-electric optical effect and magneto-chiral one. GaFeO3 has spontaneous magnetization and electric polarization at low temperatures, indicating the breakdown of the space inversion symmetry and the time reversal one, while Fe3O4 has local space inversion symmetry.
The magneto-electric optical effect, i.e., the change of optical absorption upon the reversal of the light propagation direction, has been investigated for the polar ferrimagnet GaFeO3 in the energy region of 1.0-2.5 eV. Moreover, we have found a novel magneto-optical effect, termed x-ray nonreciprocal directional dichroism, that the x-ray absorption at around the K edge of an Fe ion depends on whether the x-ray propagation vector is parallel or antiparallel to the outer production of the magnetization and electric-polarization vectors in GaFeO3. These optical responses show the obvious dependence on the electric polarization and magnetization, suggesting the relationship between these optical effects and the toroidal moment. The x-ray nonreciprocal directional dichroism spectroscopy as demonstrated here can be a useful tool to prove the local magnetism in noncentroysymmetric systems such as magnetic interferences and nanostractures. We have found the x-ray nonreciprocal directional dichroism not only in GaFeO3 but also Fe3O4.

Report

(3 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • Research Products

    (18 results)

All 2004 2003 Other

All Journal Article (15 results) Publications (3 results)

  • [Journal Article] Magnetization-Induced Second Harmonic Generation in a Polar Ferromagnet2004

    • Author(s)
      Y.Ogawa
    • Journal Title

      Physical Review Letters 92

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] X-Ray Directional Dichroism of a Polar Ferrimagnet2004

    • Author(s)
      M.Kubota
    • Journal Title

      Physical Review Letters 92

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic and crystal structures of polar ferrimagnet Ga_<2-x> Fe_xO_32004

    • Author(s)
      Y.Kaneko
    • Journal Title

      J.Mag.Mag.Mat 272-76

      Pages: 555-555

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Optical Magnetoelectric Effect in the Polar GaFeO_3 Ferrimagnet2004

    • Author(s)
      J.H.Jung
    • Journal Title

      Physical Review Letters 93

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Structural and magnetoelectric properties of Ga_<2-x>Fe_xO_3 single crystals grown by a floating-zone method2004

    • Author(s)
      T.Arima
    • Journal Title

      Physical Review B 70

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetization-induced second harmonic generation in a polar ferromagnet2004

    • Author(s)
      Y.Ogawa et al.
    • Journal Title

      Physical Review Letters 92

      Pages: 47401-47401

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] X-ray directional dichroism of a polar ferrimagnet2004

    • Author(s)
      M.Kubota et al.
    • Journal Title

      Physical Review Letters 92

      Pages: 137401-137401

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic and crystal structures of polar ferrimagnet Ga_<2-x>Fe_xO_32004

    • Author(s)
      Y.Kaneko et al.
    • Journal Title

      J.Mag.Mag.Mat. 555

      Pages: 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Optical magneto-electric properties of Ga_<2-x>Fe_xO_3 ferrimagnet2004

    • Author(s)
      J.H.Jung et al.
    • Journal Title

      Physical Review Letters 93

      Pages: 37403-37403

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Structural and magnetic properties of Ga_<2-x>Fe_xO_3 single crystals grown by a floating-zone method2004

    • Author(s)
      T.Arima et al.
    • Journal Title

      Physical Review B 703

      Pages: 64426-64426

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] X-Ray Directional Dichroism of a Polar Ferrimagnet2004

    • Author(s)
      M.Kubota, T.Arima, Y.Kaneko, J.P.He, X.Z.Yu, Y.Tokura
    • Journal Title

      Phys Rev.Lett. 92

      Pages: 137401-137401

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Optical Magnetoelectric Effect in the Polar GaFeO_3 Ferrimagnet2004

    • Author(s)
      J.H.Jung, M.Matsubara, T.Arima, J.P.He, Y.Kaneko, Y.Tokura
    • Journal Title

      Phys.Rev.Lett. 93

      Pages: 37403-37403

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Structural and magnetoelectric properties of Ga_<2-x>Fe_xO_3 single crystals grown by a floating-zone method2004

    • Author(s)
      T.Arima, D.Higashiyama, Y.Kaneko, J.P.He, (6名略), Y.Tokura
    • Journal Title

      Phys.Rev.B 70

      Pages: 64426-64426

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Magnetic control of ferroelectric polarization2003

    • Author(s)
      T.Kimura
    • Journal Title

      Nature 426

      Pages: 55-58

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic control of ferroelectric polarization2003

    • Author(s)
      T.Kimura et al.
    • Journal Title

      Nature 426

      Pages: 55-58

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] Y.Ogawa, Y.Kaneko, J.P.He, X.Z.Yu, T.Arima, Y.Tokura: "Magnetization-Induced Second Harmonic Generation in a Polar Ferromagnet"Physical Review Letters. 92(4). 047401 (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Kimura, T.Goto, H.Shintani, K.Ishizaka, T.Arima, Y.Tokura: "Magnetic control of ferroelectric polarization"Nature. 426. 55-58 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 小川佳宏, 山田浩之, 川崎雅司, 十倉好紀: "三色磁性超格子の非線形磁気光学効果"固体物理. 38. 687-693 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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