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Dating of Quaternary with ESR, TL and OSL methods : intercomparison

Research Project

Project/Area Number 15340172
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Geology
Research InstitutionOkayama University of Science

Principal Investigator

TOYODA Shin  Okayama University of Science, Department of Applied Physics, Associate Professor, 理学部, 助教授 (40207650)

Co-Investigator(Kenkyū-buntansha) NINAGAWA Kiyotaka  Okayama University of Science, Department of Applied Physics, Professor, 理学部, 教授 (80098590)
SUZUKI Takehiko  Tokyo Metropolitan University, Department of Urban Environmental Sciences, Associate Professor, 都市環境学部, 助教授 (60240941)
TSUKAMOTO Sumiko  Tokyo Metropolitan University, Department of Urban Environmental Sciences, Research Associate, 都市環境学部, 助手 (30275010)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥11,900,000 (Direct Cost: ¥11,900,000)
Fiscal Year 2005: ¥2,500,000 (Direct Cost: ¥2,500,000)
Fiscal Year 2004: ¥2,500,000 (Direct Cost: ¥2,500,000)
Fiscal Year 2003: ¥6,900,000 (Direct Cost: ¥6,900,000)
KeywordsESR / TL / OSL / dating / quaternary / tephra / natural radiation / quartz
Research Abstract

ESR(electron spin resonance), TL(thermoluminescence), and OSL(optically stimulated luminescence) dating methods, based on the same principle, have wide applications of age determination in quaternary in the range beyond that of radiocarbon method. However, these have still been considered to be viable methods. In the present project, these three methods were applied to the same tephra samples of various known ages so that the obtained ages can be compared with each other, also with the know ages. Tepharas are also appropriate samples in the present project in the aspect that they are important key layers in many geological contexts.
Quartz grains were extracted from Zenigame-Menagawa, Shibahara, Shirakawa-Ten'ei, Shirakawa-Saigo, Nantai-Shichihonzakura, Ikedako, Irito Aira-Tanzawa (Irito Ignimbrite), Aira-Shiko, Aira-Iwato, Kikai-Kuzuhara, Ata-Torihama, Kuju-1, Kuju-Handa, and AT tephras. Natural accumulated doses were obtained by ESR and isothermal TL methods. It was found in the present study that OSL is not appropriate for measurement of Japanese tephras because the rate of recupelation is too large to obtain reliable accumulated doses. Natural dose rates were obtained from the concentrations of U, Th and K concentrations in the samples which were measured by the low background gamma ray spectroscopy.
Isothermal TL ages were consistent well with the known ages while ESR ages are not so much inconsistent in the range younger than 100ka, but sometimes the ages were so much scattered in the samples of older ages. The problem should probably be the additive dose method where the gamma ray dose were applied to the samples to see the increase of the signal intensities which are extrapolated to the zero ordinate to obtain natural accumulated doses. Preliminary experiments on signal regeneration were performed to find the statistical errors become much smaller with this protocol.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (23 results)

All 2005 2004 2003 Other

All Journal Article (19 results) Publications (4 results)

  • [Journal Article] Spin-spin relaxation times of the E_1' center in quartz with and without irradiation : implications for the formation process of the oxygen vacancies in nature2005

    • Author(s)
      S.Toyoda, D.Takeuchi, T.Asai, K.Komuro, Y.Horikawa
    • Journal Title

      Radiat. Meas. 39

      Pages: 503-508

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Formation and decay of the E_1' center and its precursor in natural quartz : basics and applications2005

    • Author(s)
      S.Toyoda
    • Journal Title

      Appl. Radiat. Isot. 62

      Pages: 325-330

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Depositional environmental changes over the ast 30,000 years at Hosoike Moor, Okayama Prefecture, Western Japan2005

    • Journal Title

      Journal of Geography 114

      Pages: 811-819

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Mineral composition of clay fractions and oxygen vacancies in silt-sized quartz in soils on the Ka-Etsu Plateau, Fukui, Central Japan - possibility of eolian dust brought from northern Asia as parent material of soils2005

    • Author(s)
      Y.Kitagawa, H.Imoto, M.Saito, H.Kurihara, K.Fujie, S.Toyoda, T.Naruse
    • Journal Title

      Soil Sci.Plant Nutr. 51

      Pages: 999-1010

    • NAID

      110004706082

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Spin-spin relaxation times of the E_1' center in quartz with and without irradiation : implications for the formation process of the oxygen vacancies in nature2005

    • Author(s)
      S.Toyoda, D.Takeuchi, T.Asai, K.Komuro, Y.Horikawa
    • Journal Title

      Radiat.Meas. 39

      Pages: 503-508

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Formation and decay of the E_1' center and its precursor in natural quartz : Basics and an application to paleoenvironmental research2005

    • Author(s)
      S.Toyoda
    • Journal Title

      Proceedings for the National Conference on Luminescence and its Applications 12

      Pages: 28-31

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary 2004 Annual Research Report
  • [Journal Article] Formation and decay of the E_1' center and its precursor in natural quartz : basics and applications2005

    • Author(s)
      S.Toyoda
    • Journal Title

      Appl.Radiat.Isot. 62

      Pages: 325-330

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] 石英の不純物中心のESR測定に適切な温度及びマイクロ波の条件2005

    • Author(s)
      島田愛子, 豊田新
    • Journal Title

      Advances in ESR Applications 21

      Pages: 13-16

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 神津島流紋岩質単成火山群のESR年代2004

    • Author(s)
      横山正, 島田愛子, 梅村崇志, 豊田新
    • Journal Title

      火山 49

      Pages: 23-32

    • NAID

      110003041408

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Artificial optical bleaching of the aluminium center in quartz. Implications to ESR dating of sediments.2003

    • Author(s)
      Voinchet P., Falgueres C., Laurent M., Toyoda, S., Bahain J.J., Dolo J.M.
    • Journal Title

      Quaternary Geochronology(Quaternary Science Reviews) 22

      Pages: 1335-1338

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] The method to represent the ESR signal intensity of the aluminum hole center in quartz for the purpose of dating2003

    • Author(s)
      S.Toyoda, C.Falgueres
    • Journal Title

      Adv.ESR Appl. 20

      Pages: 7-10

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Potential use of Ti-center in ESR dating of fluvial sediment

    • Author(s)
      H.Tissoux, C.Falgueres, P.Voinchet, S.Toyoda, J.J.Bahain, J.Despriee
    • Journal Title

      Quaternary Geochronology (In press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Dating of Japanese Quaternary tephras by ESR and Luminescence methods

    • Author(s)
      S.Toyoda, S.Tsukamoto, S.Hameau, H.Usui, T.Suzuki
    • Journal Title

      Quaternary Geochronology (In press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Orbital- and Millennial-scale variations in Asian dust transport path to the Japan Sea

    • Author(s)
      K.Nagashima, R.Tada, H.Matsui, T.Irino, A.Tani, S.Toyoda
    • Journal Title

      Palaeogeography, Palaeoclimatology, Palaeoecology (In press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Dating of Japanese Quaternary tephras by ESR and Luminescence methods

    • Author(s)
      S.Toyoda, S.Tsukamoto, S, Hameau, H.Usui, T.Suzuki
    • Journal Title

      Quaternary Geochronology (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Potential use of Ti-center in ESR dating of fluvial sediment

    • Author(s)
      H.Tissoux, C.Falgueres, P.Voinchet, S, Toyoda, J.J.Bahain, J.Despriee
    • Journal Title

      Quaternary Geochronology (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Orbital- and Millennial-scale variations in Asian dust transport path to the Japan Sea

    • Author(s)
      K.Nagashima, R.Tada, H.Matsui, T.Irino, A.Tani, S.Toyoda
    • Journal Title

      Palaeogeography, Palaeoclimatology, Palaeoecology (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Dating of Japanese Quaternary tephras by ESR and Luminescence methods

    • Author(s)
      Toyoda, S., Tsukamoto, S., Hameau, S., Usui, H., Suzuki, T.
    • Journal Title

      Quatern.Geochronol. In press

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Spin-spin relaxation times of the E_1' center in quartz with and without irradiation : implications for the formation process of the oxygen vacancies in nature

    • Author(s)
      S.Toyoda, D.Takeuchi, T.Asai, K.Komuro, Y.Horikawa
    • Journal Title

      Radiation Measurements (In press)

    • Related Report
      2004 Annual Research Report
  • [Publications] 豊田新: "ウラン鉱床の生成過程及び古環境変動についての研究への応用-石英中の酸素空孔に関連したESR信号を用いて-"放射線と産業. (印刷中).

    • Related Report
      2003 Annual Research Report
  • [Publications] 横山正, 島田愛子, 梅村崇志, 豊田新: "神津島流紋岩質単成火山群のESR年代"火山. (印刷中).

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Toyoda: "Formation and decay of the E_1' center and its precursor in natural quartz : basics and applications"Appl.Radiat.Isot.. (In press).

    • Related Report
      2003 Annual Research Report
  • [Publications] S.Toyoda, C.Falgueres: "The method to represent the ESR signal intensity of the aluminum hole center in quartz for the purpose of dating"Adv.ESR Appl.. 20. 7-10 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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