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Research and Development of Pervaporation Membrane Reactor

Research Project

Project/Area Number 15360414
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Properties in chemical engineering process/Transfer operation/Unit operation
Research InstitutionYamaguchi University

Principal Investigator

KITA Hidetoshi  Yamaguchi University, Faculty of Engineering, Professor, 工学部, 教授 (10177826)

Co-Investigator(Kenkyū-buntansha) OKAMOTO Kenichi  Yamaguchi University, Faculty of Engineering, Professor, 工学部, 教授 (20029218)
TANAKA Kazuhiro  Yamaguchi University, Faculty of Engineering, Associate Professor, 工学部, 助教授 (30188289)
吉野 真  山口大学, 工学部, 助手 (60311817)
Project Period (FY) 2003 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥13,200,000 (Direct Cost: ¥13,200,000)
Fiscal Year 2004: ¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2003: ¥9,500,000 (Direct Cost: ¥9,500,000)
KeywordsMembrane Reactor / Zeolite Membrane / Molecular Sieve Carbon Membrane / Pervaporation / Micrporous Materials / Membrane Separation
Research Abstract

We described the fabrication of a pervaporation membrane reactor for the esterification reaction in order to shift the equilibrium in favor of the ester formation and to improve the conversion of the reaction and a novel pervaporation catalytic membrane reactor for the epoxidation of ally chloride by TS-1 membranes. We have reported the performance of zeolitic membranes and carbon membranes which are the most favorable one for pervaporation. Here, we reported on the hydrothermal synthesis of zeolite MOR, BEA and TS-1 membranes and their pervaporation properties. Synthetic parameters such as the reaction time, temperature, molar ratio of the starting gel, aging, and seed coating were investigated in order to optimize the pervaporation performance of the membrane. Molecular sieve carbon membranes derived from phenolic resin and lignin derivatives were also reported.

Report

(3 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • Research Products

    (25 results)

All 2005 2004 2003 Other

All Journal Article (14 results) Book (3 results) Patent(Industrial Property Rights) (4 results) Publications (4 results)

  • [Journal Article] リグノセルカース-循環型機能材料としての新しい展開2005

    • Author(s)
      舩岡正光, 青柳充, 喜多英敏
    • Journal Title

      Cellulose Commun. 12

      Pages: 2-7

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Fabrication of TS-1 Catalytic Membrane Reactor for the Selective Oxidation Reaction2005

    • Author(s)
      X.Zhang, X.Chen Hklto, K.Okamoto
    • Journal Title

      Trans.Mat.Res.Soc.Jpn 30(in press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Lignocellulose-Advanced Technologies for Sustainable Utilization as Functional Materials2005

    • Author(s)
      M.Funaoka, M.Aoyagi, H.Kita
    • Journal Title

      Cellulose Commun. 12

      Pages: 2-7

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] リグノセルロース-循環型機能材料としての新しい展開2005

    • Author(s)
      舩岡正光, 青柳 充, 喜多英敏
    • Journal Title

      Cellulose Commun. 12

      Pages: 2-7

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Fabrication of TS-1 Catalytic Membrane Reactor for the Selective Oxidation Reaction2005

    • Author(s)
      X.Zhang, X.Chen, H.Kita, K.Okamoto
    • Journal Title

      Trans.Mat.Res.Soc.Jpn. 30(in press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Synthesis of Zeolite Beta Membrane and its Pervaporation Properties2004

    • Author(s)
      X.Li, H.Kita, K.Okamoto
    • Journal Title

      Trans.Mat.Res.Soc.Jpn. 29

      Pages: 2567-2570

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Gas Separation and Pervaporation through Microporous Carbon Membranes Derived from Phenolic Resin2004

    • Author(s)
      Hidetoshi Kita et al.
    • Journal Title

      ACS.Symp.Series 876

      Pages: 203-217

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Gas Separation and Pervaporation through Microporous Carbon Membranes Derived from Phenolic Resin2004

    • Author(s)
      H.Kita, K.Nanbu, H.Maeda, K.Okamoto
    • Journal Title

      ACS.Symp.Ser. 876

      Pages: 203-217

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Gas Separation and Pervaporation through Microporous Carbon Membranes Derived from Phenolic Resin2004

    • Author(s)
      Hidetoshi Kita et al.
    • Journal Title

      ACS Symp Series 876

      Pages: 203-217

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Fabrication and Application of Zeolite Membranes2003

    • Author(s)
      Hidetoshi Kita
    • Journal Title

      Mat.Res.Soc.Symp.Soc. 752

      Pages: 293-249

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] ゼオライト膜を用いたエステル化反応2003

    • Author(s)
      喜多英敏, 田中一宏
    • Journal Title

      分離技術 33

      Pages: 99-103

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Fabrication and Application of Zeolite Membranes2003

    • Author(s)
      H.Kita
    • Journal Title

      Mat.Res.Soc.Symp.Proc. 752

      Pages: 239-249

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Application of Zeolite Membrane to Esterification Reaction2003

    • Author(s)
      H.Kita, K.Tanaka
    • Journal Title

      Bunrigijyutsu 33

      Pages: 99-103

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Fabrication of TS-1 Catalytic Membrane Reactor for the Selective Oxidation Reaction

    • Author(s)
      X.Zhang, X.Chen, H.Kita, K.Okamoto
    • Journal Title

      Trans.Mat.Res.Soc.Jpn. (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Book] 高密度炭素骨格の応用-機能性分解膜の応用(木質系有機資源の新展開)2005

    • Author(s)
      喜多英敏, 舩岡正光
    • Total Pages
      271
    • Publisher
      シーエムシー出版
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Book] Application for Functional Membrane in Advanced Technologies for Woody Organic Resources2005

    • Author(s)
      H.Kita, M.Funaoka
    • Total Pages
      157
    • Publisher
      CMC Books
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Book] 高密度炭素骨格の応用-機能性分離膜の応用(木質系有機資源の新展開)2005

    • Author(s)
      喜多英敏, 舩岡正光
    • Total Pages
      271
    • Publisher
      シーエムシー出版
    • Related Report
      2004 Annual Research Report
  • [Patent(Industrial Property Rights)] 特許 混合物分離膜とその製造方法2004

    • Inventor(s)
      喜多 英敏 他
    • Industrial Property Rights Holder
      山口TLO
    • Industrial Property Number
      2004-077302
    • Filing Date
      2004
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 特許 メンブレンリアクター2004

    • Inventor(s)
      喜多 英敏 他
    • Industrial Property Rights Holder
      山口TLO
    • Industrial Property Number
      2004-079310
    • Filing Date
      2004
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Patent(Industrial Property Rights)] 混合物分離膜とその製造方法2004

    • Inventor(s)
      喜多英敏 他
    • Industrial Property Rights Holder
      山口TLO
    • Industrial Property Number
      2004-077302
    • Filing Date
      2004
    • Related Report
      2004 Annual Research Report
  • [Patent(Industrial Property Rights)] メンブレンリアクター2004

    • Inventor(s)
      喜多英敏 他
    • Industrial Property Rights Holder
      山口TLO
    • Industrial Property Number
      2004-079310
    • Filing Date
      2004
    • Related Report
      2004 Annual Research Report
  • [Publications] Hidetoshi Kita: "Fabrication and Application of Zeolite Membranes"Mat.Res.Soc.Symp.Proc.. 752. 239-249 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 喜多英敏, 田中一宏: "ゼオライト膜を用いたエステル化反応"分離技術. 33. 99-103 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] X.Li, H.Kita, K.Okamoto: "Synthesis of Zeolite Beta Membrane and its Pervaporation Properties"Trans.Mat.Res.Soc.Jpn. 29(in press). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] Hidetoshi Kita: "Gas Separation and Pervaporation through Microporous Carbon Membranes Derived from Phenolic Resin"ACS Symp.Series. 876(in press). (2004)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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