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Study on origin and behavior of radionuclides and trace elements in atmospheric environment

Research Project

Project/Area Number 15510012
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionMusashi Institute of Technology

Principal Investigator

HONDA Teruyuki  Musashi Institute of Technology, Faculty of Engineering, Associate Professor, 工学部, 助教授 (30139414)

Co-Investigator(Kenkyū-buntansha) HIROSE Katsumi  Meteorological Research Institute, Geochemical Research Department, Department Head, 気象研究所・地球化学研究部, 部長 (70343895)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥3,300,000 (Direct Cost: ¥3,300,000)
Fiscal Year 2005: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 2004: ¥600,000 (Direct Cost: ¥600,000)
Fiscal Year 2003: ¥2,000,000 (Direct Cost: ¥2,000,000)
KeywordsAtmospheric environment / Particulate matter / Atmospheric deposition / Yellow soil dust (Kosa) / Trace element / Radionuclide / Soil dust / Fallout / 土壌起源元素 / 人工放射性核種 / 天然放射性核種 / 中性子放射化分析 / Wash out効果 / γ線スペクトロメトリ
Research Abstract

In this study, major/trace elements and radionuclides in various atmospheric samples, i.e. particulate matter (PM) samples collected weekly at Kawasaki from October 2002 to January 2005 and the bulk deposition samples collected monthly at Fukuoka, Nagasaki, Tsukuba and Kawasaki in 1964 and 2000 to 2004, were determined by using ICP-AES, neutron activation analysis and γ-ray spectrometry. Consequently, we obtained some valuable information in this study as follows ;
1.From the correlation coefficient between the concentrations of determined elements, Br-Sb and Sc-Fe-La showed a good correlation, respectively. Considering the size distributions in PM10, it was seen that the contribution of PM10 was higher than that of larger one in Br-Sb and Se-Fe-La, respectively.
2.In the average concentrations of radioactivities of ^<210>Pb and ^7Be each direction of the wind, those when the south wind blew were higher than those when the north wind did. It could be seen that ^<222>Rn, the ancestor of ^ … More <210>Pb, was diffusing 1000 times much or more as in the continent compared with in the ocean and ^7Be was influenced by the latitude effect of cosmic rays. Furthermore, it was found that the concentrations of both nuclides in those samples would be dominated by the rainfall.
3.It can be seen that the lanthanoid abundance patterns in the Nagasaki depositions from March to May are very similar to that of the yellow soil dust (Kosa) in Nagasaki. This fact shows that the Nagasaki depositions during those months would be strongly influenced by Kosa. In addition, it became clear from the Th/Sc ratios in those samples that the contribution of Kosa was higher in the depositions in recent years (2000 to 2004) than in those in 1964.
4.The temporal variation of the elements (Si,Al, lanthanides, Th etc) originated in soil was almost coincided with total amounts of the samples excluding those collected at Fukuoka in summer in 2000. It was suggested that the soil dusts dominated the total amounts of the depositions.
5.The concentrations of uranium, radioactivities of ^<137>Cs and the U/Th ratios in the deposition samples in 1964 were apparently higher between March and May than those in other months. It seems that the deposition samples in 1964 reflected the active stratosphere-troposphere air exchange in the springtime and were affected by the nuclear test during 1962-1963. Less

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (27 results)

All 2006 2005 2004 2003 Other

All Journal Article (21 results) Publications (6 results)

  • [Journal Article] 2003-2004年川崎大気環境中の^<210>Pbおよび^7Beの存在量と挙動2006

    • Author(s)
      本多照幸, 後藤仁美
    • Journal Title

      フィッション・トラック ニュースレター 通巻・19(印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Abundance and behavior of ^<210>Pb and ^7Be in atmospheric samples collected at Kawasaki in 2003 and 20042006

    • Author(s)
      T.Honda, H.Goto
    • Journal Title

      Fission Track News Letter 19(in print)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] 1964年福岡降下物中のウラン、トリウム及び核分裂生成物2005

    • Author(s)
      北原照央, 本多照幸, 廣瀬勝己, 五十嵐康人, 青山道夫
    • Journal Title

      フィッション・トラック ニュースレター 通巻・18

      Pages: 41-45

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Annual Research Report 2005 Final Research Report Summary
  • [Journal Article] Study on uranium, thorium and fission products of deposition samples collected at Fukuoka in 19642005

    • Author(s)
      A.Kitahara, T.Honda, K.Hirose, Y.Igarashi, M.Aoyama
    • Journal Title

      Fission Track News Letter 18

      Pages: 41-45

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] 鹿児島湾並びに島原湾における鉛210およびウラン、トリウム等微量元素の分布と特徴2005

    • Author(s)
      本多照幸, 佐藤裕介
    • Journal Title

      フィッション・トラック ニュースレター 通巻・18

      Pages: 37-40

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 中性子放射化分析による草津白根山西麓源泉(万座温泉)のヒ素,臭素の定量2005

    • Author(s)
      佐野淳子, 川井智, 木川田喜一, 本多照幸, 大井隆夫
    • Journal Title

      武蔵工業大学原子力研究所研究所報 通巻・30

      Pages: 24-27

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 鹿児島湾並びに島原湾海底堆積物における微量元素の分布と挙動2005

    • Author(s)
      本多照幸, 佐藤裕介
    • Journal Title

      2005年度日本地球化学会第52回年会講演要旨集 2005

      Pages: 187-187

    • NAID

      130004592470

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 1964年福岡降下物における微量元素並びにセシウム137の分布と挙動2005

    • Author(s)
      北原照央, 本多照幸, 五十嵐康人, 青山道夫, 廣瀬勝己
    • Journal Title

      2005日本放射化学会年会研究発表要旨集 2005

      Pages: 141-141

    • Related Report
      2005 Annual Research Report
  • [Journal Article] 1964年福岡降下物中のウラン、トリウムおよび核分裂生成物2005

    • Author(s)
      北原照央, 本多照幸, 廣瀬勝己, 五十嵐康人, 青山道夫
    • Journal Title

      フィッション・トラックニュースレター 通巻・18(印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Deposition behavior of ^<210>Pb, ^7Be and thorium isotopes observed in Tsukuba and Nagasaki, Japan2004

    • Author(s)
      K.Hirose, T.Honda, S.Yagishita, Y.Igarashi, M.Aoyama
    • Journal Title

      Atmospheric Environment 38

      Pages: 6601-6608

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Distribution of radionuclides and trace elements and sedimentary environment in marine sediments from coastal areas of Japan2004

    • Author(s)
      T.Honda, E.Suzuki
    • Journal Title

      Book of extended synopsis (IAEA); International Conference on Isotopes in Environmental Studies CN-118

      Pages: 530-531

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] 大気降下物中の^<210>PBおよび^7Be濃度の変動とその要因2004

    • Author(s)
      本多照幸, 五十嵐康人, 青山道夫, 廣瀬勝己
    • Journal Title

      フィッション・トラック ニュースレター 通巻・17

      Pages: 47-49

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] The fluctuations of contents of ^<210>Pb and ^7Be in deposition samples and their factors2004

    • Author(s)
      T.Honda, Y.Igarashi, M.Aoyama, K.Hirose
    • Journal Title

      Fission Track News Letter 17

      Pages: 47-49

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Deposition behavior of ^<210>Pb, ^7Be and thorium isotopes observed in Tsukuba and Nagasaki, Japan2004

    • Author(s)
      K.Hirose, T.Honda, S.Yagishita, Y.Igarashi.M.Aoyama
    • Journal Title

      Atmospheric Environment 38

      Pages: 6601-6608

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Distribution of radionuclides and trace elements and sedimentary environment in marine sediments from coastal areas of Japan2004

    • Author(s)
      T.Honda, E.Suzuki
    • Journal Title

      Book of extended synopsis (IAEA);International Conference on Isotopes in Environmental Studies CN-118

      Pages: 530-531

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Spatial distribution of ^3H, ^<90>Sr, ^<137>Cs and ^<239+240>Pu in surface waters of the Pacific and Indian Oceans-GLOMARD database2004

    • Author(s)
      P.P.Povinec, K.Hirose, T.Honda, T.Ito, E.M.Scott, O.Togawa
    • Journal Title

      Journal of Environmental Radioactivity 76

      Pages: 113-137

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Mobility of lanthanides accompanying the formation of alunite group minerals2004

    • Author(s)
      K.Kikawada, M.Uruga, T.Oi, T.Honda
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry 261・3

      Pages: 651-659

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 大気降下物中の^<210>Pbおよび^7Be濃度の変動とその要因2004

    • Author(s)
      本多照幸, 五十嵐康人, 青山道夫, 廣瀬勝己
    • Journal Title

      フィッション・トラック ニュースレター 通巻・17

      Pages: 47-49

    • Related Report
      2004 Annual Research Report
  • [Journal Article] 東京湾、陸奥湾および噴火湾海底堆積物における主要並びに微量元素の分布と挙動2003

    • Author(s)
      本多照幸, 木村賢一郎
    • Journal Title

      日本海水学会誌 57・3

      Pages: 166-180

    • NAID

      80015983859

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Distribution and behavior of major and trace elements in Tokyo Bay, Mutsu Bay and Funka Bay marine sediments2003

    • Author(s)
      T.Honda, K.Kimura
    • Journal Title

      Bull.Soc. Sea Water Sci.Jpn. 57

      Pages: 166-180

    • NAID

      80015983859

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Distribution of radionuclides and trace elements and sedimentary environment in marine sediments from coastal areas of Japan

    • Author(s)
      T.Honda, E.Suzuki
    • Journal Title

      Book of extended synopsis (IAEA) ; International Conference on Isotopes in Environmental Studies CN-118

      Pages: 530-531

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Publications] 本多照幸, 五十嵐康人, 青山道夫, 廣瀬勝己: "大気降下物中の^<210>Pbおよび^7Be濃度の変動とその要因"フィッション・トラック ニュースレター. 通巻・17(印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] 本多照幸, 木村賢一郎, 森本隆夫, 鈴木頴介: "噴火湾海底堆積物の鉛210堆積年代と昭和新山の形成"フィッション・トラック ニュースレター. 通巻・16. 31-33 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 本多照幸, 川村 茂: "中性子放射化分析による東京湾海底堆積物中のランタノイド,トリウム及びウランの定量とその挙動"日本放射化学会誌(別冊). 4. 48 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 鈴木健二, 本多照幸: "愛知県内15地点における浮遊粒子状物質の中性子放射化分析"日本放射化学会誌(別冊). 4. 49 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 本多照幸, 石田幸三, 五十嵐康人, 青山道夫, 廣瀬勝己: "2001年つくば降下物における主要並びに微量元素濃度とその特徴"第50回日本地球化学会年会講演要旨集. 2003. 1 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] 本多照幸, 木村賢一郎, 森本隆夫: "東京湾,陸奥湾および噴火湾海底堆積物における主要並びに微量元素の分布と挙動"日本海水学会誌. 57・3. 166-180 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2016-04-21  

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