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Study on spin structures and electron-lattice interaction of nanomaterials using nuclear resonant scattering.

Research Project

Project/Area Number 15540308
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics I
Research InstitutionKyoto University

Principal Investigator

SETO Makoto  Kyoto University, Research Reactor Institute, Associate Professor, 原子炉実験所, 助教授 (40243109)

Co-Investigator(Kenkyū-buntansha) KOBAYASHI Yasuhiro  Kyoto University, Research Reactor Institute, Instructor, 原子炉実験所, 助手 (00303917)
KITAO Shinji  Kyoto University, Research Reactor Institute, Instructor, 原子炉実験所, 助手 (00314295)
Project Period (FY) 2003 – 2005
Project Status Completed (Fiscal Year 2005)
Budget Amount *help
¥3,300,000 (Direct Cost: ¥3,300,000)
Fiscal Year 2005: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 2004: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2003: ¥1,600,000 (Direct Cost: ¥1,600,000)
KeywordsNuclear resonant scattering / Synchrotron radiation / Nanomaterials / Spin structure / Electron-lattice interaction / Hyperfine interactions / 電子・格子相互作用
Research Abstract

Nanostructured materials like quantum wires have attracted much interest for their novel properties and the possibilities for new devices. It is well known that nanostructured materials show different electric and thermodynamical properties as compared to ordinary macroscopic materials. For the further understanding and new applications, microscopic studies on nanosized materials are indispensable.
We have measured the time and energy spectra of nuclear resonant scattering of synchrotron radiation from magnetic Fe nanowires to investigate the electronic states and lattice dynamics of the Fe nanowires, As for the electronic states, we studied the correlation between the spin structure and the shape of the wires. From the measured time spectra of the Fe nanowires, the value of internal magnetic field is obtained to be 32.9 T. This agrees with the value of the bulk Fe (33 T), and this result indicates the electronic state of Fe atoms in our nanowire sample is almost the same as that of Fe atoms in a bulk sample. Furthermore, it was confirmed that the direction of the magnetic field is anisotropic and coincides with the direction of the nanowires. Our results show that this method is useful for the study of electronic states of nanomaterilas. As for the vibrational states, we studied the difference between the bulk state and the nanowires. Because it is possible to obtain the information on the specific elements by using nuclear resonant scattering, we can obtain the intrinsic lattice dynamics of nanoweires without the vibration of the substrate material. The observed phonon spectra show the dependence on the size of the samples, and we concluded it is due to the anharmonic effect.

Report

(4 results)
  • 2005 Annual Research Report   Final Research Report Summary
  • 2004 Annual Research Report
  • 2003 Annual Research Report
  • Research Products

    (3 results)

All 2003 Other

All Journal Article (2 results) Publications (1 results)

  • [Journal Article] 放射光核共鳴前方散乱によるFe量子ワイヤーの内部磁場分布についての研究2003

    • Author(s)
      瀬戸 誠
    • Journal Title

      ナノテクノロジー総合支援プロジェクトSPring-8研究成果報告書 2

      Pages: 31-31

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Journal Article] Study on distribution of internal magnetic fields in Fe nanowires using nuclear resonant forward scattering2003

    • Author(s)
      Makoto SETO
    • Journal Title

      Nanotechnology in SPring-8 2

      Pages: 31-31

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2005 Final Research Report Summary
  • [Publications] 瀬戸 誠: "放射光核共鳴前方散乱によるFe量子ワイヤーの内部磁場分布についての研究"ナノテクノロジー総合支援プロジェクト Spring-8研究成果報告書. 2. 31-33 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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