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Adsorption Structures and Competition of Multiple Spin Exchange Interactions in Two-dimensional Quantum Solids.

Research Project

Project/Area Number 15540330
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionUniversity of Tsukuba

Principal Investigator

MORISHITA Masashi  University of Tsukuba, Graduate School of Pure and Applied Sciences, Research Associate, 大学院・数理物質科学研究科, 助手 (90251032)

Co-Investigator(Kenkyū-buntansha) TAKAGI Takeo  Fukui University, Faculty of Technology, Assistant Professor, 工学部, 助教授 (00206723)
Project Period (FY) 2003 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥3,600,000 (Direct Cost: ¥3,600,000)
Fiscal Year 2004: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 2003: ¥2,200,000 (Direct Cost: ¥2,200,000)
KeywordsTwo-dimension System / Quantum Solid / Quantum Spin System / Multiple Spin Exchange Interaction / Adsorption Structure / Helium-3 / Graphite / Thermal Conductivity
Research Abstract

Helium-3 (^3He) solid films adsorbed on a graphite surface are considered as ideal materials of two-dimensional spin system. In the ^3He solid films, the competition of multiple spin exchange(MSE) interactions dominates the magnetic interactions and complicates the magnetism. Recently, the important roll of the corrugation of the adsorption potential, or the adsorption structures, on the MSE competition has been recognized.
In this research we measured the heat capacity of the ^3He solid films in the commensurate areal density regime down to sub-mK temperature for the first time. We observed almost inversely proportional behavior, C ∝ T^α (α【approximately equal】 -1), in the wide temperature range more than two decades as in other areal density regimes. This behavior is unusual and anomalous as the heat capacity of localized spin systems in the high temperature limit, and is attributed to the strong competition of the MSE interactions. The α value is thought to be smaller as the MSE comp … More etition is stronger. The observed absolute value of the exponent α is larger in the commensurate areal density regime than in the incommensurate regime and shows the MSE competition is very strong. This observation agrees with the prediction that in the commensurate structure the corrugation of the adsorption potential suppresses spin exchanges, especially lower-order exchanges, and the MSE competition should be stronger than in incommensurate structures.
The mechanisms of cooling ^3He films through substrates have not clearly understood either. We also measured the thermal conductivity between ^3He films and graphite substrates by the relaxation method. The measured thermal conductivity shows similar areal density variation with the strength of the MSE interaction. This observation indicates that the measured thermal conductivity is the thermal conductivity of the ^3He film itself, not of the interface, and the heat is transferred only by local spots between ^3He films and graphite substrates. It suggests the magnetic Kapitza mechanism between 3^He spins and magnetic impurities in graphite substrates. The preliminary measurements in magnetic fields, in which strong magnetic field dependence was observed, support this hypothesis. Less

Report

(3 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • Research Products

    (13 results)

All 2005 2003 Other

All Journal Article (12 results) Publications (1 results)

  • [Journal Article] Heat Capacities of Submonolayer Solid ^3He Films on Graphite at Highly Frustrated Density Regime2005

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Low Temperature Physics 138

      Pages: 367-372

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermal Relaxation of ^3He Solid Films Adsorbed on Graphite2005

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Low Temperature Physics 138

      Pages: 373-378

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Striped-honeycomb transition of domain wall structure of ^3He submonolayer solid film on graphite2003

    • Author(s)
      M.Morishita, T.Takagi
    • Journal Title

      Physica B 329-333

      Pages: 137-139

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Striped - honeycomb transition of domain wall structure of ^3He submonolayer solid film on graphite2003

    • Author(s)
      M.Morishita, T.Takagi
    • Journal Title

      Physica B 329-333

      Pages: 137-139

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Anomalous heat capacities in submonolayer solid ^3He films commensurate to graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Heat transfer between ^3He film graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Anomalous heat capacities in submonolayer solid ^3He films commensurate to graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Heat transfer between ^3He film and graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Heat Capacities of Submonolayer Solid ^3He Films on Graphite at Highly Frustrated Density Regime

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Low Temperature Physics (in press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Thermal Relaxation of ^3He Solid Films Adsorbed on Graphite

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Low Temperature Physics (in press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Anomalous heat capacities in submonolayer solid ^3He films commensurate to graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Heat transfer between ^3He film and graphite substrate

    • Author(s)
      M.Morishita
    • Journal Title

      Journal of Physics and Chemistry in Solid (in press)

    • Related Report
      2004 Annual Research Report
  • [Publications] M.Morishita, T.Takagi: "Striped honeycomb transition of domain wall structure of ^3He submonolayer solid film on graphite"Physica B. 320-333. 137-139 (2003)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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