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Measurement for Transport and Thermal Properties of Materials with anomalous thermoelectric behaviors at Low Temperatures below 1K

Research Project

Project/Area Number 15540335
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionToyama University

Principal Investigator

KUWAI Tomohiko  Toyama University, Department of Physics, Assistant Prof., 理学部, 助教授 (10251878)

Co-Investigator(Kenkyū-buntansha) ISIKAWA Yosikazu  Toyama University, Department of Physics, Prof., 理学部, 教授 (20143836)
MIZUSHIMA Toshio  Toyama University, Department of Physics, Assistant Prof., 理学部, 助教授 (50135000)
MITSUDA Akihiro  Toyama University, Department of Physics, Research Assistant, 理学部, 助手 (20334708)
Project Period (FY) 2003 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥3,200,000 (Direct Cost: ¥3,200,000)
Fiscal Year 2004: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 2003: ¥2,700,000 (Direct Cost: ¥2,700,000)
Keywordshigh resolution specific heat measurement / Non-Fermi liquid / low-temperature thermoelectric power / strongly correlated electron systems / single crystal growth / Thermal conductivity / low-temperature specific heat under high pressure / material research / 極低温熱電能 / 熱電能 / 極低温圧力下電気抵抗測定
Research Abstract

Aim for our research is as follows :
1.Construction of the measurement systems for thermoelectric power S, thermal conductivity κ and the other physical quantities characterizing properties of solid from the room temperature down to 0.1K.
2.Identification of materials with anomalous thermoelectric properties at low temperatures, and research for their nature via transport and thermal quantities such as electrical resistivity p and specific heat C.
In the research term, we finished constructing the several systems including S and κ on a ^3He-^4He dilution frigerator, C under pressure using a ^3He-cryostat, and investigated the magnetic properties of several 4f-electron compounds from experimental results obtained using these systems. The main research results are as follows :
1.We measured S and C of Ce(Ni,Pd)_2Ge_2 well below 1 K, and detected a quantitative close relation in between the Sommerfeld coefficient γ and the S/T reflecting a non-Fermi liquid nature in the lowest temperature range.
2.Mitsuda et al. reported the pressure-induced ferromagnetic transition at 2 K with small magnetic moment in a valence transition compound (Yb_<0.8>Y_<0.2>)InCu_4 by magnetization measurement. We detected a sharp peak at 2 K in C under 1.2 GPa, and obtained about 20 % of the full moment of Yb^<3+> ion is frozen with this phase transition from the entropy consideration, concluding this transition is from a bulk property and intrinsic in this compound.
3.We measured p and C of a valence fluctuator EuPd_2Si_2 and its 'isovolume' diluted alloys (Eu(La_<0.67>Y_<0.33>)Pd_2Si_2 between 2 and 300 K. We found both the resistance minimum at 20 K and the C/T upturn reaching large amount at low temperatures below 30 K for the alloys beyond 25 % of substitution of Eu by (La_<0.67>Y_<0.33>). We consider they may originate from the Kondo effect, and the measurements of S for these alloys are in progress.

Report

(3 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • Research Products

    (22 results)

All 2005 2004 Other

All Journal Article (18 results) Publications (4 results)

  • [Journal Article] Change of magnetic anisotropy in the antiferromagnetic-ferromagnetic transition in Ce(Pd_<1-x>M_x)_2Al_3 (M=Cu or AG)2005

    • Author(s)
      石川 義和 他
    • Journal Title

      Physica B (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Weak ferromagnetism stabilized by pressure and substitution of Y for Yb in YbInCu_4.2005

    • Author(s)
      光田 暁弘 他
    • Journal Title

      Physica B (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Specific heat of CeNi_2Ge_2 in wide-range of temperatures2004

    • Author(s)
      桑井 智彦 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

      Pages: 68-69

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic properties of single crystals of RCoIn_6 (R=Tb,Dy,Ho,Er,Yb)2004

    • Author(s)
      石川 義和 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

      Pages: 635-636

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] High field magnetization of TbNiAl_42004

    • Author(s)
      水島 俊雄 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Annual Research Report 2004 Final Research Report Summary
  • [Journal Article] Transport properties of Yb_<0.8>Y_<0.2>InCu_4 under high pressure2004

    • Author(s)
      光田 暁弘 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

      Pages: 56-57

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Specific heat of CeNi_2Ge_2 in wide-range of temperatures.2004

    • Author(s)
      T.Kuwai, T.Takeuchi, T.Tsuchiya, Y.Isikawa, T.Fukuhara
    • Journal Title

      J.Magn.Magn.Mater. 272-276

      Pages: 68-69

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Magnetic properties of single crystals of RCoIn_5 (R=Tb,Dy,Ho,Er,Yb).2004

    • Author(s)
      Y.Isikawa, D.Kato, A.Mitsuda, T.Mizushima, T.Kuwai
    • Journal Title

      J.Magn.Magn.Mater. 272-276

      Pages: 635-636

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] High field magnetization of TbNiAl_4.2004

    • Author(s)
      T.Mizushima, Y.Isikawa, A.Mitsuda, K.Kobayashi, F.Ishikawa, T.Goto
    • Journal Title

      J.Magn.Magn.Mater. 272-276

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Transport properties of Yb_<0.8>Y_<0.2>InCu_4 under pressure.2004

    • Author(s)
      A.Mitsuda, T.Ikeno, Y.Nakamura, T.Kuwai, Y.Isikawa, W.Zhang, K.Yoshimura
    • Journal Title

      J.Magn.Magn.Mater. 272-276

      Pages: 56-57

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Schottky peaks in specific heat induced by electronic change in the antiferromagnetic-ferromagnetic alternating Kondo system Ce(Pd_<1-x>M_x)_2Al_3(M=Cu or Ag)2004

    • Author(s)
      P.Sun, Q.Lu, K.Kobayashi, T.Kuwai, Y.Isikawa
    • Journal Title

      Phys.Rev., B 70

      Pages: 174429-8

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Specific heat of CeN_2Ni_2Ge_2 in wide-range of temperatures2004

    • Author(s)
      桑井 智彦 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

      Pages: 68-69

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Magnetic properties of single crystals of RCoIn_5 (R=Th, Dy, Ho, Er, Yb)2004

    • Author(s)
      石川 義和 他
    • Journal Title

      J.Magn.Magn.Mater. 271-276

      Pages: 635-636

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Transport properties of Yb_<0.8>Y_<0.2>InCu_4 under high pressure2004

    • Author(s)
      光田 暁弘 他
    • Journal Title

      J.Magn.Mang.Mater. 271-276

      Pages: 56-57

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Change of magnetic anisotropy in the antiferromagnetic-ferro magnetic transition in Ce(Pd_<1-x>M_x)_2Al_3(M=Cu or Ag)

    • Author(s)
      孫 培傑 他
    • Journal Title

      Physica B (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Weak ferromagnetism stabilized by pressure and substitution of Y for Yb in YbInCu_4

    • Author(s)
      光田 暁弘 他
    • Journal Title

      Physica B (印刷中)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Change of magnetic anisotropy in the antiferromagnetic-ferromagnetic transition in Ce(Pd_<1-x>M_x)_2Al_3(M=Cu or Ag)

    • Author(s)
      P.Sun, Y.Isikawa, K.Kobayaski, T.Mizushima, T.Kuwai
    • Journal Title

      Physica B (in press.)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Weak ferromagnetism established by pressure and substitution of Y for Yb in YbInCu_4.

    • Author(s)
      A.Mitsuda, H.Nihonmatsu, M.Yamada, H.Ohta, W.Zhang, K.Yoshimura, T.Goto, O.Kolomlyet, Y.Isikawa
    • Journal Title

      Physica B (in press.)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] 桑井 智彦: "Specific heat of CeNi_2Ge_2 in wide-range of temperatures"J.Magn.Magn.Mater. (掲載予定). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] 石川 義和: "Magnetic properties of single crystals of RCoIn_5 (R=Tb,Dy,Ho,Er,Yb)"J.Magn.Magn.Mater. (掲載予定). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] 水島 俊雄: "High field magnetization of TbNiAl_4"J.Magn.Magn.Mater. (掲載予定). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] 光田 暁弘: "Transport properties of Yb_<0.8>Y_<0.2>InCu_4 under high pressure"J.Magn.Magn.Mater. (掲載予定). (2004)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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