Nonlinear optical response and quantum critical phase control in orbital-ordered oxides
Project/Area Number |
15540351
|
Research Category |
Grant-in-Aid for Scientific Research (C)
|
Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Condensed matter physics II
|
Research Institution | Sophia University |
Principal Investigator |
KUWAHARA Hideki Sophia University, Faculty of Science and Technology, Associate Professor (90306986)
|
Project Period (FY) |
2003 – 2004
|
Project Status |
Completed (Fiscal Year 2004)
|
Budget Amount *help |
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2004: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2003: ¥2,000,000 (Direct Cost: ¥2,000,000)
|
Keywords | Dimensionality / Oxide / Relaxation Process / Ferroelectric / Pump-Probe Method / Ferromagnetism / Femto-Second-Laser / Reflectivity / 相図 / 光学測定 |
Research Abstract |
Photoinduced effects in a single crystal of bilayered manganites, La_2-2xSr_1+2xMn_2O_7 (x=0.38), were investigated in a wide range of temperatures by pump-probe measurement at a photon energy of 1.6 eV. In a ferromagnetic metallic state, significant enhancement of positive rise in differential reflectivity with a slow relaxing time of 100 ps was observed just below Tc=127 K, indicating that the reflectivity change with the slow relaxation time constant is induced by laser heating. We have also observed an unconventional fast relaxing component that has a time constant of the order of 10 ps. This fast relaxing component, whose absolute value has an asymmetric peak at Tc, is presumably due to short-range correlation of Jahn-Teller distortion. The Hall resistivity and magnetization have been investigated in the ferromagnetic state of the bilayered manganite La_<2-2x>Sr_<1+2x>Mn_2O_7 (x=0.36). The Hall resistivity shows an increase in both the ordinary and anomalous Hall coefficients at low temperatures below 50 K, a region in which experimental evidence for the spin glass state has been found in a low magnetic field of 1mT. The origin of the anomalous behavior of the Hall resistivity relevant to magnetic states may lie in the intrinsic microscopic inhomogeneity in a quasi-two-dimensional electron system.
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Report
(3 results)
Research Products
(23 results)