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Nonlinear optical response and quantum critical phase control in orbital-ordered oxides

Research Project

Project/Area Number 15540351
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionSophia University

Principal Investigator

KUWAHARA Hideki  Sophia University, Faculty of Science and Technology, Associate Professor (90306986)

Project Period (FY) 2003 – 2004
Project Status Completed (Fiscal Year 2004)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2004: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2003: ¥2,000,000 (Direct Cost: ¥2,000,000)
KeywordsDimensionality / Oxide / Relaxation Process / Ferroelectric / Pump-Probe Method / Ferromagnetism / Femto-Second-Laser / Reflectivity / 相図 / 光学測定
Research Abstract

Photoinduced effects in a single crystal of bilayered manganites, La_2-2xSr_1+2xMn_2O_7 (x=0.38), were investigated in a wide range of temperatures by pump-probe measurement at a photon energy of 1.6 eV. In a ferromagnetic metallic state, significant enhancement of positive rise in differential reflectivity with a slow relaxing time of 100 ps was observed just below Tc=127 K, indicating that the reflectivity change with the slow relaxation time constant is induced by laser heating. We have also observed an unconventional fast relaxing component that has a time constant of the order of 10 ps. This fast relaxing component, whose absolute value has an asymmetric peak at Tc, is presumably due to short-range correlation of Jahn-Teller distortion.
The Hall resistivity and magnetization have been investigated in the ferromagnetic state of the bilayered manganite La_<2-2x>Sr_<1+2x>Mn_2O_7 (x=0.36). The Hall resistivity shows an increase in both the ordinary and anomalous Hall coefficients at low temperatures below 50 K, a region in which experimental evidence for the spin glass state has been found in a low magnetic field of 1mT. The origin of the anomalous behavior of the Hall resistivity relevant to magnetic states may lie in the intrinsic microscopic inhomogeneity in a quasi-two-dimensional electron system.

Report

(3 results)
  • 2004 Annual Research Report   Final Research Report Summary
  • 2003 Annual Research Report
  • Research Products

    (23 results)

All 2005 2004 2003 Other

All Journal Article (17 results) Publications (6 results)

  • [Journal Article] Transient differential reflectivity of ferromagnetic and paramagnetic phases in the bilayered manganite La_<1.24>Sr_<1.76>Mn_2O_72005

    • Author(s)
      Y. Hirobe, et al.
    • Journal Title

      Solid State Communications 133

      Pages: 449-453

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Transient differential reflectivity of ferromagnetic anc paramagnetic phases in the bilayered manganite La_<1.24>Sr_<1.76>Mn_2O_72005

    • Author(s)
      Y. Hirobe, et al.
    • Journal Title

      Solid State Communications 133

      Pages: 449-453

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Spin Wave and Orbital Ordering in the C-type Antiferromagnetic Phase of Nd_<1-x>Sr_xMnO_32005

    • Author(s)
      R.Kajimoto et al.
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 502-503

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Transient differential reflectivity of ferromagnetic and paramagnetic phases in the bilayered manganite La_<1.24>Sr_<1.76>Mn_2O_72005

    • Author(s)
      Y.Hirobe et al.
    • Journal Title

      Solid State Communicatioins 133

      Pages: 449-453

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Magnetic-Field and External-Pressure Control of Ferroelectricity in Multiferroic Manganites2005

    • Author(s)
      H.Kuwahara et al.
    • Journal Title

      Physica B(印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Magnetic-Field and External-Pressure Effect on Ferroelectricity in Manganites : Comparison between GdMnO_3 and TbMnO_32005

    • Author(s)
      K.Noda et al.
    • Journal Title

      Journal of Applied Physics (印刷中)

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Spin Wave and Orbital Ordering in the C-type Antiferromagnetic Phase of Nd_<1-x>Sr_xMnO_32004

    • Author(s)
      R. Kajimoto, et al.
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 502-503

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Effects of magnetic field on Raman spectra in (Nd_<0.5>Sr_<0.5>)MnO_32004

    • Author(s)
      H. Kuroe, et al.
    • Journal Title

      Journal of magnetism and magnetic materials 272-276

      Pages: 816-817

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermoelectric properties of filling controlled manganites2004

    • Author(s)
      H. Kuwahara, et al.
    • Journal Title

      Journal of magnetism and magnetic materials 272-276

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Spin Wave and Orbital Ordering in the C-type Antiferromagnetic Phase of Nd_<1-x>Sr_xMnO_32004

    • Author(s)
      R. Kajimoto, et at.
    • Journal Title

      Journal of the Physical Society of Japan 74

      Pages: 502-503

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Thermoelectric properties of filling controlled manganites2004

    • Author(s)
      H.Kuwahara et al.
    • Journal Title

      Journal of magnetism and magnetic materials 272-276

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Effects of magnetic field on Raman spectra in (Nd_<0.5>Sr_<0.5>)MnO_32004

    • Author(s)
      H.Kuroe et al.
    • Journal Title

      Journal of Magnetism and magnetic materials 272-276

      Pages: 816-817

    • Related Report
      2004 Annual Research Report
  • [Journal Article] Orbital order and a canted phase in the paramagnetic and ferromagnetic states of 50% hole-doped colossal magnetoresistance manganites2003

    • Author(s)
      H. Kawano-Furukawa, et al.
    • Journal Title

      Physical Review B 67

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Optical study in the charge-ordered phase of (Nd_<1-x>Sr_x)MnO_32003

    • Author(s)
      H. Kuroe, et al.
    • Journal Title

      Physica B 329-333

      Pages: 822-823

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Phase Diagram and Magneto-Transport Properties in Nd_<1-x>Sr_xMnO_3 Crystals2003

    • Author(s)
      H. Kuwahara, et al.
    • Journal Title

      Physica B 329-333

      Pages: 850-851

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Anomalous Hall effect and magnetoresistance in Nd_<1-x>Sr_xMnO_3 single crystals2003

    • Author(s)
      H. Kuwahara, et al.
    • Journal Title

      Journal of Applied Physics 93

      Pages: 7367-7369

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Journal Article] Orbital order and a canted phase in the paramagnetic and ferromagnetic states of 50 % hole-doped colossal magnetore sistance manganites2003

    • Author(s)
      H. Kawano-Furukawa, et al.
    • Journal Title

      Physical Review B 67

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2004 Final Research Report Summary
  • [Publications] H.Kuwahara et al.: "Anomalous Hall effect and magnetoresistance in Nd_<1-x>Sr_xMnO_3 single crystals"Journal of Applied Physics. 93. 7367-7369 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Kuroe et al.: "Optical study in the charge-ordered phase of (Nd_<1-x>Sr_x)MnO_3"Physica. B 329-333. 822-823 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Kuwahara et al.: "Phase Diagram and Magneto-Transport Properties in Nd_<1-x>Sr_xMnO_3 Crystals"Physica. B 329-333. 850-851 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Kawano-Furukawa et al.: "Orbital order and a canted phase in the paramagnetic and ferromagnetic states of 50% hole-doped colossal magnetoresistance manganites"Physical Review. B 67. 174422-1-174422-5 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] H.Kuwahara et al.: "Thermoelectric properties of filling controlled manganites"Journal of magnetism and magnetic materials. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.Kajimoto et al.: "Spin wave and orbital ordering in the C-type antiferromagnetic phase of Nd_<1-x>Sr_xMnO_3"Journal of magnetism and magnetic materials. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report

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Published: 2003-04-01   Modified: 2020-05-15  

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