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Development of a Compton camera using a single scattering-absorption detector fabricated from an ultrasensitive thallium bromide semiconductor

Research Project

Project/Area Number 15H02523
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Medical Physics and Radiological Technology
Research InstitutionTohoku University

Principal Investigator

Hitomi Keitaro  東北大学, 工学研究科, 准教授 (60382660)

Co-Investigator(Kenkyū-buntansha) 小野寺 敏幸  東北工業大学, 工学部, 准教授 (10620916)
渡辺 賢一  名古屋大学, 工学研究科, 准教授 (30324461)
金 聖潤  東北大学, 工学研究科, 准教授 (50574357)
長野 宣道  東北大学, 工学研究科, 助教 (60757673)
Project Period (FY) 2015-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥46,280,000 (Direct Cost: ¥35,600,000、Indirect Cost: ¥10,680,000)
Fiscal Year 2019: ¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2018: ¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2017: ¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2016: ¥16,120,000 (Direct Cost: ¥12,400,000、Indirect Cost: ¥3,720,000)
Fiscal Year 2015: ¥16,640,000 (Direct Cost: ¥12,800,000、Indirect Cost: ¥3,840,000)
Keywordsコンプトンカメラ / 臭化タリウム / ガンマ線 / 半導体検出器 / 位置敏感型検出器 / 結晶成長 / ガンマ線検出器 / 放射線、X線、粒子線
Outline of Final Research Achievements

A Compton gamma-ray imaging camera was developed using an ultrasensitive compound semiconductor, thallium bromide (TlBr). Gamma-ray detectors were fabricated from TlBr crystals grown from purified materials in this study. Images of gamma-rays of 662 keV from a 137Cs source and gamma-rays of 1173 keV and 1333 keV from a 60Co source were successfully obtained from a pixelated TlBr detector with a Compton imaging method. Because TlBr detectors exhibit high stopping power for high-energy gamma rays, the developed detectors are promising for applications in nuclear medicine for imaging of gamma rays from multiple elements, proton therapy for estimation of dose distributions, and gamma-ray imaging spectroscopies.

Academic Significance and Societal Importance of the Research Achievements

本研究では素材の純化から検出器製作までを一貫して行い、ガンマ線のイメージングへの応用が可能な高感度のTlBrガンマ線検出器の開発を行った。本研究で得られた成果は純国産の世界最高水準の新しい半導体検出器技術である。本研究の成果は核医学診断装置においては複数元素同時イメージング、粒子線治療においては線量分布の可視化につながる技術であり、その応用範囲は極めて広く、学術的・社会的意義は大きい。

Report

(6 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • Research Products

    (42 results)

All 2020 2019 2018 2017 2016 2015 Other

All Int'l Joint Research (2 results) Journal Article (7 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 5 results,  Open Access: 4 results,  Acknowledgement Compliant: 1 results) Presentation (33 results) (of which Int'l Joint Research: 14 results,  Invited: 5 results)

  • [Int'l Joint Research] University of Michigan(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Michigan(米国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Photoluminescence and scintillation of TlBr crystals at low temperatures2020

    • Author(s)
      Koshimizu Masanori、Hitomi Keitaro、Nogami Mitsuhiro、Yanagida Takayuki、Fujimoto Yutaka、Asai Keisuke
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: SC Pages: SCCB19-SCCB19

    • DOI

      10.7567/1347-4065/ab4895

    • NAID

      210000157202

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Crystalline Characterization of TlBr Semiconductor Detectors Using Wavelength-resolved Neutron Imaging2020

    • Author(s)
      Kenichi Watanabe, Kio Matsumoto, Akira Unitani, Keitaro Hitomi, Mitsuhiro Nogami, and Winfried Kockelmann
    • Journal Title

      Sensors and Materials

      Volume: -

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Transient Absorption Spectroscopy of TlBr Crystals Using Pulsed Electron Beams2020

    • Author(s)
      Masanori Koshimizu, Yusa Muroya, Shinichi Yamashita, Mitsuhiro Nogami, Keitaro Hitomi, Yutaka Fujimoto, and Keisuke Asai
    • Journal Title

      Sensors and Materials

      Volume: -

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Prompt Gamma-Ray Detection with TlBr Detectors for Proton Radiation Therapy2019

    • Author(s)
      K. Hitomi, T. Higuma, H. Hosokawa, M. Nogami, A. Terakawa
    • Journal Title

      CYRIC Annual Report 2016-2017

      Volume: - Pages: 50-52

    • Related Report
      2019 Annual Research Report
    • Open Access
  • [Journal Article] Recent results from pixelated TlBr detectors with Tl electrodes operated at room-temperature2017

    • Author(s)
      C. Leak, W. Koehler, S. O'Neal, Z. He, K. Hitomi
    • Journal Title

      Nuclear Science Symposium, Medical Imaging Conference and Room-Temperature Semiconductor Detector Workshop (NSS/MIC/RTSD), 2016

      Volume: - Pages: 1-3

    • DOI

      10.1109/nssmic.2016.8069952

    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Journal Article] Fabrication of double-sided thallium bromide strip detectors2016

    • Author(s)
      Keitaro Hitomi, Nobumichi Nagano, Toshiyuki Onodera, Seong-Yun Kim, Tatsuya Ito, Keizo Ishii
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section A

      Volume: 823 Pages: 15-19

    • DOI

      10.1016/j.nima.2016.03.107

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Study on Effects of Gamma-Ray Irradiation on TlBr Semiconductor Detectors2016

    • Author(s)
      Motohiro Matsumura, Kenichi Watanabe, Atsushi Yamazaki, Akira Uritani, Norihisa Kimura, Nobumichi Nagano, and Keitaro Hitomi
    • Journal Title

      Proceedings of International Symposium on Radiation Detectors and Their Uses (ISRD2016), JPS Conference Proceedings

      Volume: 11 Pages: 030005-030005

    • DOI

      10.7566/jpscp.11.030005

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Presentation] 波長分解中性子イメージングに基づくTlBr検出器製作過程の検討2020

    • Author(s)
      渡辺 賢一、松本 伎朗、瓜谷 章、野上 光博、人見 啓太朗
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] TlBr結晶のパルス電子ビームを用いた過渡吸収分光2020

    • Author(s)
      越水 正典、室屋 裕佐、山下 真一、野上 光博、人見 啓太朗、藤本 裕、浅井 圭介
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Characterization of 1-cm thick Thallium Bromide Gamma-Ray Detectors2019

    • Author(s)
      K. Hitomi, M. Nogami, T. Onodera, K. Watanabe, K. Matsumoto, J. Lee, K. Ishii
    • Organizer
      26th International Symposium on Room-Temperature Semiconductor X-Ray & Gamma-Ray Detectors
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Crystalline evaluation of TlBr semiconductor detectors using energy-resolved neutron imaging2019

    • Author(s)
      K. Watanabe1, K. Matsumoto, A. Uritani, Y. Kiyanagi, K. Hitomi, M. Nogami, H. Sato, W. Kockelmann
    • Organizer
      26th International Symposium on Room-Temperature Semiconductor X-Ray & Gamma-Ray Detectors
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Partial Recovery of Pixellated Thallium Bromide from Polarization through Sustained Reverse-Polarity Biasing2019

    • Author(s)
      E. Hall, K. Hitomi, Z. He
    • Organizer
      26th International Symposium on Room-Temperature Semiconductor X-Ray & Gamma-Ray Detectors
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] TlBr結晶の低温発光特性における結晶成長部位と熱履歴の影響2019

    • Author(s)
      越水 正典、人見 啓太朗、野上 光博、柳田 健之、藤本 裕、浅井 圭介
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 波長分解中性子イメージングによるTlBrの結晶性評価2019

    • Author(s)
      渡辺 賢一、松本 伎朗、人見 啓太朗、野上 光博、山﨑 淳、吉橋 幸子、瓜谷 章
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 1 cm厚ピクセル型TlBr放射線検出器の製作と評価2019

    • Author(s)
      野上光博、人見啓太朗、小野寺敏幸、渡辺賢一、松本伎朗、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第66回 応用物理学会 春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 大型TlBr放射線検出器の製作と評価2018

    • Author(s)
      野上光博、人見啓太朗、長野宣道、小野寺敏幸、渡辺賢一、松本伎朗、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第79回 応用物理学会 秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Fabrication of large volume pixelated TlBr detectors2018

    • Author(s)
      K. Hitomi, M. Nogami, N. Nagano, T. Onodera, K. Watanabe, N. Kimura, S. Kubo, S. - Y. Kim, T. Ito, K. Ishii
    • Organizer
      25th International Symposium on Room-Temperature Semiconductor Detectors
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 三次元相互作用位置情報を用いた9ピクセル型TlBr検出器の評価2017

    • Author(s)
      砂庭 広季、人見 啓太朗、長野 宣道、小野寺 敏幸、金 聖潤、伊藤 辰也、木村 乃久、高坂 充、石井 慶造
    • Organizer
      日本原子力学会2017年春の年会
    • Place of Presentation
      東海大学湘南キャンパス(神奈川県平塚市)
    • Year and Date
      2017-03-27
    • Related Report
      2016 Annual Research Report
  • [Presentation] ピクセル型TlBr半導体検出器を用いたコンプトンカメラの開発2017

    • Author(s)
      松村 基広、渡辺 賢一、山﨑 淳、吉橋 幸子、瓜谷 章、砂場 広季、長野 宣道、人見 啓太朗
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川県横浜市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] Development of Thallium Bromide Detectors for Compton Imaging2017

    • Author(s)
      K. Hitomi, M. Nogami, N. Nagano, T. Onodera, K. Watanabe, M. Matsumura, S.-Y. Kim, T. Ito, K. Ishii
    • Organizer
      24th International Symposium on Room-Temperature Semiconductor X-Ray and Gamma-Ray Detectors
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Evaluation of TlBr Detectors for Prompt Gamma-Ray Detection for Proton Therapy2017

    • Author(s)
      M. Nogami, K. Hitomi, N. Nagano, T. Onodera, H. Hosokawa, T. Higuma, S.-Y. Kim, T. Ito, A. Terakawa
    • Organizer
      24th International Symposium on Room-Temperature Semiconductor X-Ray and Gamma-Ray Detectors
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Recent Results from Pixelated TlBr Detectors with Tl Electrodes Operated at Room-Temperature2016

    • Author(s)
      C. Leak, W. Koehler, S. O'Neal, Z. He, K. Hitomi
    • Organizer
      The 23rd International Symposium on Room-Temperature Semiconductor Detectors
    • Place of Presentation
      The Strasbourg Convention Center, Strasbourg (France)
    • Year and Date
      2016-10-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Basic Study of a Compton Scattering Camera Using a Pixelated TlBr Detector2016

    • Author(s)
      M. Matsumura, K. Watanabe, A. Yamazaki, S. Yoshihashi, A. Uritani, H. Sunaba, N. Nagano, K. Hitomi
    • Organizer
      The 23rd International Symposium on Room-Temperature Semiconductor Detectors
    • Place of Presentation
      The Strasbourg Convention Center, Strasbourg (France)
    • Year and Date
      2016-10-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Growth of TlBr Crystals by the Vertical Bridgman Method and the Traveling Molten Zone Method for Gamma-Ray Detector Applications2016

    • Author(s)
      K. Hitomi, T. Onodera, N. Nagano, K. Watanabe, M. Matsumura, S.-Y. Kim, T. Ito, K. Ishii
    • Organizer
      The 23rd International Symposium on Room-Temperature Semiconductor Detectors
    • Place of Presentation
      The Strasbourg Convention Center, Strasbourg (France)
    • Year and Date
      2016-10-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ピクセル型臭化タリウム半導体検出器を用いたコンプトンカメラの研究2016

    • Author(s)
      松村基広、山崎淳、渡辺賢一、吉橋幸子、瓜谷章、砂庭広季、長野宣道、人見啓太朗
    • Organizer
      第77回応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ(新潟県新潟市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] 三次元相互作用位置情報を用いたTlBr検出器のエネルギー分解能改善2016

    • Author(s)
      砂庭広季、人見啓太朗、長野宣道、木村乃久、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      日本原子力学会2016年秋の大会
    • Place of Presentation
      久留米シティプラザ(福岡県久留米市)
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] 波形解析による臭化タリウム検出器のエネルギー分解能改善2016

    • Author(s)
      人見啓太朗、長野宣道、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第53回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学弥生講堂(東京都文京区)
    • Year and Date
      2016-07-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] Fabrication and Evaluation of Orthogonal-Strip TlBr Gamma-Ray Detectors2016

    • Author(s)
      K. Hitomi, N. Nagano, T. Onodera, T. Ito, S.-Y. Kim, K. Ishii
    • Organizer
      2016 IEEE SYMPOSIUM ON RADIATION MEASUREMENTS AND APPLICATIONS
    • Place of Presentation
      University of California, Berkeley, California (USA)
    • Year and Date
      2016-05-22
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Study on Tolerance of TlBr Semiconductor Detectors to Gamma-Ray Irradiation2016

    • Author(s)
      M. Matsumura, K. Watanabe, A. Yamazaki, A. Uritani, N. Nagano, K. Hitomi
    • Organizer
      2016 IEEE SYMPOSIUM ON RADIATION MEASUREMENTS AND APPLICATIONS
    • Place of Presentation
      University of California, Berkeley, California (USA)
    • Year and Date
      2016-05-22
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 位置敏感型TlBr検出器の製作と評価2016

    • Author(s)
      人見啓太朗、長野宣道、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      日本原子力学会「2016年春の年会」
    • Place of Presentation
      東北大学川内キャンパス(宮城県・仙台市)
    • Year and Date
      2016-03-26
    • Related Report
      2015 Annual Research Report
  • [Presentation] Tl電極の臭化タリウム半導体検出器の温度特性2016

    • Author(s)
      松村基広、山﨑淳、渡辺賢一、瓜谷章、長野宣道、人見啓太朗
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京都・目黒区)
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 3 x 3ピクセル電極を有するTlBr検出器の製作2016

    • Author(s)
      人見啓太朗、長野宣道、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京都・目黒区)
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Development of position-sensitive TlBr gamma-ray detectors2016

    • Author(s)
      K. Hitomi, N. Nagano, T. Onodera, T. Ito, S.-Y. Kim, K. Ishii
    • Organizer
      International Symposium on Radiation Detectors and Their Uses
    • Place of Presentation
      KEK (Tsukuba, Ibaraki)
    • Year and Date
      2016-01-18
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Study on the effects of exposure of TlBr semiconductor detector to gamma-ray2016

    • Author(s)
      M. Matsumura, K. Watanabe, A. Yamazaki, A. Uritani, N. Nagano, K. Hitomi
    • Organizer
      International Symposium on Radiation Detectors and Their Uses
    • Place of Presentation
      KEK (Tsukuba, Ibaraki)
    • Year and Date
      2016-01-18
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of TlBr Gamma-Ray Detectors with Single Polarity Charge Sensing Configurations2015

    • Author(s)
      K. Hitomi, N. Nagano, T. Onodera, C. Disch, S.-Y. Kim, T. Ito, K. Ishii
    • Organizer
      2015 IEEE Nuclear Science Symposium, Medical Imaging Conference, and 22nd International Symposium on Room-Temperature Semiconductor X-Ray and Gamma-ray Detectors
    • Place of Presentation
      Town and Country Hotel, San Diego, California (USA)
    • Year and Date
      2015-10-31
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] SPECT装置への応用を目指した新しい化合物半導体検出器の開発2015

    • Author(s)
      人見啓太朗、長野宣道、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第43回日本放射線技術学会秋季学術大会
    • Place of Presentation
      金沢市文化ホール(石川県・金沢市)
    • Year and Date
      2015-10-08
    • Related Report
      2015 Annual Research Report
  • [Presentation] 両面ストリップ型TlBr検出器の製作2015

    • Author(s)
      人見啓太朗、長野宣道、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県・名古屋市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] 臭化タリウム半導体検出器の耐放射線性2015

    • Author(s)
      松村基広、山﨑淳、渡辺賢一、瓜谷章、長野宣道、人見啓太朗
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県・名古屋市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] TlBr検出器を用いたガンマ線CTの検討2015

    • Author(s)
      長野宣道、人見啓太朗、小野寺敏幸、伊藤辰也、金聖潤、石井慶造
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県・名古屋市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] TlBrガンマ線検出器の信号処理法開発2015

    • Author(s)
      長野宣道、人見啓太朗、伊藤辰也、金聖潤、石井慶造、小野寺敏幸
    • Organizer
      日本原子力学会「2015年秋の大会」
    • Place of Presentation
      静岡大学静岡キャンパス(静岡県・静岡市)
    • Year and Date
      2015-09-09
    • Related Report
      2015 Annual Research Report

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Published: 2015-04-16   Modified: 2022-11-04  

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