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Analysis of transition process at the molecular level of dissolved organic carbon in terrestrial area by utilizing special pulse NMR method

Research Project

Project/Area Number 15H02805
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionKobe University

Principal Investigator

FUJITAKE NOBUHIDE  神戸大学, 農学研究科, 教授 (50243332)

Co-Investigator(Kenkyū-buntansha) 近藤 美由紀  国立研究開発法人国立環境研究所, 環境計測研究センター, 研究員 (30467211)
杉山 裕子  岡山理科大学, 理学部, 准教授 (40305694)
内田 雅己  国立極地研究所, 国際北極環境研究センター, 准教授 (70370096)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥17,290,000 (Direct Cost: ¥13,300,000、Indirect Cost: ¥3,990,000)
Fiscal Year 2017: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2016: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2015: ¥10,530,000 (Direct Cost: ¥8,100,000、Indirect Cost: ¥2,430,000)
Keywords溶存有機物 / 1H NMR / 北極湿原 / 炭素循環 / 溶存有機炭素 / 3D-EEM-PARAFAC分析 / SPR-W5-WATERGATE法 / 炭素動態解析法 / 炭素ストック / 地球温暖化 / 物質循環 / 炭素固定 / 土壌有機物 / 炭素フロー
Outline of Final Research Achievements

Application of 1H NMR analysis using a special pulse sequence (SPR-W5-WATERGATE) was examined on dissolved organic carbon (DOC) which is the key of the carbon cycle process in the terrestrial ecosystem. Optimization of measurement parameters in the sequence, guarantee of quantitative, and examination of pretreatment method were carried out.
As a result, it was found that a good spectrum can be obtained by measuring 0.5 to 24 hours with a sample amount of 1 mL to 50 mL even for test water having a low DOC concentration. Through application examples of DOCs taken from a wetland in the high latitude Arctic region, the utility of this method was demonstrated.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • Research Products

    (20 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (5 results) Journal Article (12 results) (of which Int'l Joint Research: 8 results,  Peer Reviewed: 12 results,  Open Access: 5 results,  Acknowledgement Compliant: 3 results) Presentation (2 results) Book (1 results)

  • [Int'l Joint Research] Kings Bay AS - Ny-Alesund(Norway)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] National University of Mongolia(Mongolia)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Buryat State University(ロシア連邦)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Chulalongkorn University/Ministry of Natural Resources Environm.(Thailand)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Texas A & M University at Galveston/Savannah River National Laboratory/Los Alamos National Laboratory(U.S.A.)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Radionuclide uptake by colloidal and particulate humic acids obtained from 14 soils collected worldwide2018

    • Author(s)
      Lin Peng、Xu Chen、Xing Wei、Sun Luni、Kaplan Daniel I.、Fujitake Nobuhide、Yeager Chris M.、Schwehr Kathleen A.、Santschi Peter H.
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1

    • DOI

      10.1038/s41598-018-23270-0

    • NAID

      120006454535

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Dissolved organic matter distribution and its association with colloidal aluminum and iron in the Selenga River Basin from Ulaanbaatar to Lake Baikal2018

    • Author(s)
      Kida Morimaru、Myangan Orgilbold、Oyuntsetseg Bolormaa、Khakhinov Viacheslav、Kawahigashi Masayuki、Fujitake Nobuhide
    • Journal Title

      Environmental Science and Pollution Research

      Volume: a head of print Issue: 12 Pages: 11948-11957

    • DOI

      10.1007/s11356-018-1462-z

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Impact of land uses on heavy metal distribution in the Selenga River system in Mongolia2017

    • Author(s)
      Myangan Orgilbold、Kawahigashi Masayuki、Oyuntsetseg Bolormaa、Fujitake Nobuhide
    • Journal Title

      Environmental Earth Science

      Volume: 76 Issue: 9 Pages: 346-361

    • DOI

      10.1007/s12665-017-6664-z

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Plutonium Partitioning Behavior to Humic Acids from Widely Varying Soils Is Related to Carboxyl-Containing Organic Compounds2017

    • Author(s)
      Peng Lin , Chen Xu, Saijin Zhang, Nobuhide Fujitake, Daniel I. Kaplan, Chris M. Yeager, Yuko Sugiyama, Kathleen A. Schwehr, and Peter H. Santschi
    • Journal Title

      Environmental Science & Technolohy

      Volume: 20 Issue: 20 Pages: 42-11751

    • DOI

      10.1021/acs.est.7b03409

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Dynamics of dissolved organic matter in the mangrove area of the Fukido River, Ishigaki Island2017

    • Author(s)
      木田 森丸, 金城 和俊, 大塚 俊之, 藤嶽 暢英
    • Journal Title

      JAPANESE JOURNAL OF ECOLOGY

      Volume: 67 Issue: 2 Pages: 85-93

    • DOI

      10.18960/seitai.67.2_85

    • NAID

      130005893365

    • ISSN
      0021-5007, 2424-127X
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High salinity leads to accumulation of soil organic carbon in mangrove soil.2017

    • Author(s)
      Morimaru Kida, Mitsutoshi Tomotsune, Yasuo Iimura, Kazutoshi Kinjo, Toshiyuki Ohtsuka, Nobuhide Fujitake
    • Journal Title

      Chemosphere

      Volume: 177 Pages: 51-55

    • DOI

      10.1016/j.chemosphere.2017.02.074

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Spatial variations in the molecular diversity of dissolved organic matter in water moving through a boreal forest in eastern Finland.2017

    • Author(s)
      Jun’ichiro Ide, Mizue Ohashi, Katsutoshi Takahashi, Yuko Sugiyama, Sirpa Piirainen, Pirkko Kortelainen, Nobuhide Fujitake, Keitaro Yamase, Nobuhito Ohte, Mina Moritani, Miyako Hara, Leena Finer
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 42102-42102

    • DOI

      10.1038/srep42102

    • NAID

      120006360176

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Role of natural organic matter on iodine and 239,240Pu distribution and mobility in environmental samples from the northwestern Fukushima Prefecture, Japan2016

    • Author(s)
      Xu, C., S. Zhang, Y. Sugiyama, N. Ohte, Y.-F. Ho, N. Fujitake, D. I. Kaplan, C. M. Yeager, K. Schwehr, and P. H. Santschi
    • Journal Title

      Journal of Environmental Radioactivity

      Volume: 153 Pages: 156-166

    • DOI

      10.1016/j.jenvrad.2015.12.022

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Determination of aquatic humic substances in Japanese lakes and wetlands by the carbon concentration-based resin isolation technique2016

    • Author(s)
      Tsuda K, Kida M, Aso S, Kato T, Fujitake N, Maruo M, Hayakawa K, Hirota M
    • Journal Title

      Limnology

      Volume: 17 Issue: 1 Pages: 1-6

    • DOI

      10.1007/s10201-015-0455-6

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Evaluation of salinity effect on quantitative analysis of aquatic humic substances using nonionic DAX-8 resin2015

    • Author(s)
      Kida M, Ohtsuka T, Kato T, Suzuki T, Fujitake N
    • Journal Title

      Chemosphere

      Volume: 146 Pages: 129-132

    • DOI

      10.1016/j.chemosphere.2015.12.031

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] 琵琶湖水中のフルボ酸のOECD試験法による水生生物への急性毒性評価2015

    • Author(s)
      早川和秀,廣瀬佳則,一瀬 諭,岡本高弘,古田世子,藤嶽暢英,田中仁志
    • Journal Title

      日本水処理生物学会誌

      Volume: 51 Pages: 105-114

    • NAID

      130006471084

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Physicochemical and ion-binding properties of highly aliphatic humic substances extracted from deep sedimentary groundwater.2015

    • Author(s)
      Saito, T., Terashima, M., Aoyagi, N., Nagao, S. Fujitake, N. and Ohnuki, T.
    • Journal Title

      Environmental Science: Processes & Impacts

      Volume: 17 Issue: 8 Pages: 1386-1395

    • DOI

      10.1039/c5em00176e

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] SPR-W5-WATERGATEパルスプログラムを用いた溶存有機物の1H NMRスペクトル測定2017

    • Author(s)
      藤嶽暢英、田邉舞、太田幸子
    • Organizer
      日本土壌肥料学会2017年度仙台大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 南極湖沼溶存有機物に光を当てる:光学的分析およびフミン物質定量2017

    • Author(s)
      木田森丸,小島汰一,田邊優貴子,林健太郎,工藤栄,眞家永光,藤嶽暢英
    • Organizer
      日本腐植物質学会2017年度山口大会
    • Related Report
      2017 Annual Research Report
  • [Book] 土のひみつ -食料・環境・生命 「2-4 土の生成に及ぼす気候(温度・水分状態) の影響」2015

    • Author(s)
      藤嶽暢英
    • Publisher
      朝倉書店
    • Related Report
      2015 Annual Research Report

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Published: 2015-04-16   Modified: 2022-08-31  

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