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Study for light-emitting devices using metal-halide perovskite-type semiconductors

Research Project

Project/Area Number 15H03573
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Optical engineering, Photon science
Research InstitutionThe University of Tokyo

Principal Investigator

Kondo Takashi  東京大学, 先端科学技術研究センター, 教授 (60205557)

Co-Investigator(Renkei-kenkyūsha) MIYASAKA Tsutomu  桐蔭横浜大学, 医用工学部, 特任教授 (00350687)
EMA Kazuhiro  上智大学, 理工学部, 教授 (40194021)
Research Collaborator NAKAMURA Yuiga  
SANO Junro  
KIMURA Kohei  
TAKASHIMA Shun  
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥17,290,000 (Direct Cost: ¥13,300,000、Indirect Cost: ¥3,990,000)
Fiscal Year 2017: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2016: ¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2015: ¥8,710,000 (Direct Cost: ¥6,700,000、Indirect Cost: ¥2,010,000)
Keywordsハロゲン化鉛ペロブスカイト / ペロブスカイト型半導体 / 真空蒸着 / ヘテロ構造 / ダブルヘテロ構造 / エピタキシャル薄膜 / ヘテロエピタキシー / エピタキシャル成長 / 太陽電池 / 発光素子 / ペロブスカイト太陽電池 / 発光ダイオード / 半導体レーザ / ペロブスカイト半導体 / ハロゲン化鉛 / ヘテロ積層
Outline of Final Research Achievements

Metal-halide perovskite-type semiconductors are used in light-absorbing layers of the perovskite solar cells which have been invented by Japanese researchers. We have investigated fabrication of methylammnonium lead halide heterostructures bearing potential applications to light-emitting devises in mind. We have succeeded in fabricating polycrystalline heterostructures by using vacuum evaporation technique for the first time. Moreover, we have also succeeded in the first demonstration of hetero-epitaxial thin-film formation on single-crystal lead-bromide perovskite substrates. In addition, we have studied a novel phenomenon, photo-induced phase separation of semiconductor alloys, which will hinder band engineering of the perovskite-type semiconductors.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • Research Products

    (30 results)

All 2018 2017 2016 2015

All Journal Article (6 results) (of which Peer Reviewed: 3 results,  Open Access: 2 results,  Acknowledgement Compliant: 1 results) Presentation (24 results) (of which Int'l Joint Research: 9 results,  Invited: 3 results)

  • [Journal Article] Self-organized superlattice and phase coexistence inside thin film organometal halide perovskite2018

    • Author(s)
      T. W. Kim, S. Uchida, T. Matsushita, L. Cojocaru, R. Jono, K. Kimura, D. Matsubara, M. Shirai, K. Ito, H. Matsumoto, T. Kondo, and H. Segawa
    • Journal Title

      Adv. Mater.

      Volume: 30 Issue: 8

    • DOI

      10.1002/adma.201705230

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ハロゲン化金属ペロブスカイト型物質2018

    • Author(s)
      近藤高志
    • Journal Title

      フォトニクスニュース

      Volume: 4

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Exciton-exciton scattering in perovskite CH3NH3PbBr3 single crystal2016

    • Author(s)
      H. Kunugita, Y. Kiyota, Y. Udagawa, Y. Takeoka, Y. Nakamura, J. Sano, T. Matsushita, T. Kondo, and K. Ema
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 55 Issue: 6 Pages: 060304-060304

    • DOI

      10.7567/jjap.55.060304

    • NAID

      210000146576

    • Related Report
      2016 Annual Research Report 2015 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] ペロブスカイト型半導体CH3NH3PbI3の基礎物性2016

    • Author(s)
      近藤高志
    • Journal Title

      光機能材料研究会会報光触媒

      Volume: 49 Pages: 16-19

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Excitonic Feature in Hybrid Perovskite CH3NH3PbBr3 Single Crystals2015

    • Author(s)
      Hideyuki Kunugita, Tsubasa Hashimoto, Yuki Kiyota, Yosuke Udagawa, Yuko Takeoka, Yuiga Nakamura, Junro Sano, Tomonori Matsushita, Takashi Kondo, Tsutomu Miyasaka, and Kazuhiro Ema
    • Journal Title

      Chem. Lett.

      Volume: 44 Issue: 6 Pages: 852-854

    • DOI

      10.1246/cl.150204

    • NAID

      130005074610

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] ハロゲン化鉛ペロブスカイト型半導体の物性2015

    • Author(s)
      近藤高志
    • Journal Title

      オプトロニクス

      Volume: 7 Pages: 71-75

    • Related Report
      2015 Annual Research Report
  • [Presentation] A new discovery of double phase coexistence inside the perovskite solar cells2018

    • Author(s)
      S. Uchida, T. W. Kim, L. Cojocaru, T. Kondo, and H. Segawa
    • Organizer
      International Conference on Perovskite Thin Film Photovoltaics (ABXPV18)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Defect chemistry analysis on CH3NH3PbI3 toward conductivity control of lead-halide perovskites2018

    • Author(s)
      Y. Nakamura, T. Matsushita, S. Yamaguchi, and T. Kondo
    • Organizer
      International Conference on Perovskite Thin Film Photovoltaics (ABXPV18)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Exciton structure of perovskite single crystals (CH3NH3PbBr3 and CH3NH3PbI3)2018

    • Author(s)
      M. Schulz, Y. Udagawa, Y. Nakamura, K. Kimura, C. Yura, K. Yamamoto, T. Matsushita, T. Kondo, H. Kunugita, and K. Ema
    • Organizer
      International Conference on Perovskite Thin Film Photovoltaics (ABXPV18)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 真空蒸着法によるCH3NH3PbI3/CH3NH3PbCl3へテロ積層構造の作製2018

    • Author(s)
      高島駿, 中村唯我, 松下智紀, 近藤高志
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ハロゲン化鉛ペロブスカイト型半導体のヘテロエピタキシャル薄膜形成(II)2018

    • Author(s)
      木村浩平, 松下智紀, 近藤高志
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Direct observation of self-organized superlattices and phase coexistence in organometal halide perovskite solar cell with transmission electron microscopy2018

    • Author(s)
      T. W. Kim, S. Uchida, T. Matsushita, L. Cojocaru, T. Kondo, H. Segawa
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ハロゲン化鉛ペロブスカイト半導体のヘテロエピタキシャル薄膜形成2017

    • Author(s)
      木村浩平, 松下智紀, 近藤高志
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] ハロゲン化鉛ペロブスカイト型半導体混晶の光誘起スピノーダル分解の温度依存性2017

    • Author(s)
      佐野惇郎, 松下智紀, 近藤高志
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] Transmission electron microscopy observation of phase coexistence in organometal halide perovskite solar cell2017

    • Author(s)
      Taewoong Kim, Satoshi Uchida, Tomonori Matsushita, Ludmila Cojocaru, Takashi Kondo, Hiroshi Segawa
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] ペロブスカイト型半導体の基礎物性と結晶工学2017

    • Author(s)
      近藤高志
    • Organizer
      第146回結晶工学分科会研究会「ペロブスカイトは結晶か? 有機金属ハライド太陽電池の特殊性・一般性と可能性」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] The partial conductivity measurements on methylammonium lead tribromide perovskite materials2017

    • Author(s)
      K. Wang, Y. Nakamura, T. Kondo, K. Kobayashi, and S. Yamaguchi
    • Organizer
      21st International Conference on Solid State Ionics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] The photoelectrochemical properties of methylammonium lead tribromide perovskite materials governed by ion migration and its application to photo-electrochemical devices2017

    • Author(s)
      K. Wang, Y. Nakamura, T. Kondo, and S. Yamaguchi
    • Organizer
      21st International Conference on Solid State Ionics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Formation of Epitaxial Thin Films of Lead Halide Perovskite Semiconductor2017

    • Author(s)
      K. Kimura, T. Matsushita, and T. Kondo
    • Organizer
      Photonics@SG 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ガスソースを用いた真空蒸着によるCH3NH3PbI3多結晶薄膜の作製2017

    • Author(s)
      中村唯我, 松下智紀, 近藤高志
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 単結晶MAPbBr3の部分電気伝導度測定とその欠陥化学2017

    • Author(s)
      山口周, Kai Wang, 小林清, 中村唯我, 近藤高志
    • Organizer
      第43回固体イオニクス討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 真空蒸着を用いた高安定性ホルムアミジニウムヨウ化鉛多結晶薄膜の作製2016

    • Author(s)
      紺野晃央, 松下智紀, 佐野惇郎, 中村唯我, 近藤高志
    • Organizer
      第77回応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ(新潟)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] 有機無機ペロブスカイト物質CH3NH3PbBr3の励起子物性2016

    • Author(s)
      宇田川洋祐, 清田祐貴, 中村唯我, 佐野惇郎, 松下智紀, 欅田英之, 竹岡裕子, 近藤高志, 江馬一弘,
    • Organizer
      第77回応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ(新潟)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] ハロゲン化金属ペロブスカイト型半導体と太陽電池応用2016

    • Author(s)
      近藤高志
    • Organizer
      The 23rd International Workshop on Active-Matrix Flatpanel Displays and Devices (AM-FPD 16)
    • Place of Presentation
      龍谷大響都ホール(京都)
    • Year and Date
      2016-07-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 太陽電池応用へ向けた真空蒸着法を用いたホルムアミジニウムヨウ化鉛多結晶薄膜の作製2016

    • Author(s)
      松下智紀, 紺野晃央, 佐野惇郎, 中村唯我, 近藤高志
    • Organizer
      第13回「次世代の太陽光発電システム」シンポジウム
    • Place of Presentation
      アオーレ長岡(新潟)
    • Year and Date
      2016-05-19
    • Related Report
      2016 Annual Research Report
  • [Presentation] Excitonic properties and carrier dynamics of CH3NH3PbBr3 single crystals2015

    • Author(s)
      Y. Kiyota, Y. Udagawa, H. Kunuigta, Y. Takeoka, Y. Nakamura, T. Matsushita, T. Kondo, T. Miyasaka, and K. Ema
    • Organizer
      1st International Conference on Provskite Solar Cells and Optoelectronics
    • Place of Presentation
      ローザンヌ(スイス)
    • Year and Date
      2015-09-27
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Exciton and Bandgap Energies of Hybrid Perovskite CH3NH3PbI32015

    • Author(s)
      Y. Nakamura, J. Sano, T. Matsushita, Y. Kiyota, Y. Udagawa, H. Kunugita, K. Ema, and T. Kondo
    • Organizer
      2015 International Conference on Solid State Devices and Materials (SSDM 2015)
    • Place of Presentation
      Sapporo Convention Center(北海道・札幌市)
    • Year and Date
      2015-09-27
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 有機無機ペロブスカイト化合物の励起子物性2015

    • Author(s)
      清田祐貴, 宇田川洋祐, 中村唯我, 佐野惇郎, 松下智紀, 欅田英之, 竹岡裕子, 近藤高志, 江馬一弘
    • Organizer
      日本物理学会 2015年秋季大会
    • Place of Presentation
      関西大学千里山キャンパス(大阪府・吹田市)
    • Year and Date
      2015-09-18
    • Related Report
      2015 Annual Research Report
  • [Presentation] ハロゲン化鉛ペロブスカイト型半導体CH3NH3PbX3の電子状態と励起子2015

    • Author(s)
      近藤高志, 江馬一弘
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県・名古屋市)
    • Year and Date
      2015-09-14
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] CH3NH3PbI3/CH3NH3PbBr3ヘテロ積層真空蒸着膜の自発的混晶化2015

    • Author(s)
      佐野惇郎, 中村唯我, 松下智紀, 近藤高志
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県・名古屋市)
    • Year and Date
      2015-09-14
    • Related Report
      2015 Annual Research Report

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Published: 2015-04-16   Modified: 2019-03-29  

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