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Strongly Correlated Electrons in Quasicrystals

Research Project

Project/Area Number 15H03685
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionNagoya University

Principal Investigator

DEGUCHI Kazuhiko  名古屋大学, 理学研究科, 講師 (40397584)

Co-Investigator(Renkei-kenkyūsha) SATO NORIAKI  名古屋大学, 大学院理学研究科, 教授 (30170773)
ISHIMASA TSUTOMU  公益財団法人豊田理化学研究所, フェロー事業部門, フェロー (10135270)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥17,030,000 (Direct Cost: ¥13,100,000、Indirect Cost: ¥3,930,000)
Fiscal Year 2017: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2016: ¥5,720,000 (Direct Cost: ¥4,400,000、Indirect Cost: ¥1,320,000)
Fiscal Year 2015: ¥7,930,000 (Direct Cost: ¥6,100,000、Indirect Cost: ¥1,830,000)
Keywords強相関電子系 / 低温物性 / 金属物性 / 磁性 / 超伝導 / スピンエレクトロニクス / 物性実験
Outline of Final Research Achievements

The Au-Al-Yb quasicrystal with Tsai-type cluster exhibits novel quantum critical phenomena as observed in Yb-based heavy fermion materials with intermediate Yb valence, while the Au-Al-Yb approximant shows heavy Fermi liquid behavior. The quantum critical state of the Au-Al-Yb quasicrystal might correspond to an electronic state unique to the quasicrystals. In the process of material research, we have found superconductivity of Au-Ge-Yb approximants with Tsai-type cluster. Furthermore, we have confirmed the emergence of bulk superconductivity of Al-Zn-Mg quasicrystal at a very low transition temperature [1]. Comparison between the quasicrystal and the approximants demonstrate that the effective interaction between electrons remains attractive under variation of the atomic arrangement. In superconducting quasicrystal, the fractal geometry might interplay with superconductivity: fractal superconductivity.
[1] K. Kamiya, K. Deguchi et al., Nature Communications 9, 154 (2018).

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • Research Products

    (34 results)

All 2018 2017 2016 2015

All Journal Article (17 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 17 results,  Open Access: 4 results,  Acknowledgement Compliant: 6 results) Presentation (17 results) (of which Int'l Joint Research: 8 results,  Invited: 8 results)

  • [Journal Article] Discovery of superconductivity in quasicrystals2018

    • Author(s)
      K. Kamiya, T. Takeuchi, N. Kabeya, N. Wada, T. Ishimasa, A. Ochiai, K. Deguchi, K. Imura, N.K. Sato
    • Journal Title

      Nature Communications

      Volume: 9 Issue: 1 Pages: 154-154

    • DOI

      10.1038/s41467-017-02667-x

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] First Observation of Heavy Fermion Behavior in Ce-Based Icosahedral Approximant2017

    • Author(s)
      K. Imura, K. Nobe, K. Deguchi, M. Matsunami, H. Miyazaki, A. Yasui, E. Ikenaga, N. K. Sato
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 86 Issue: 9 Pages: 093702-093702

    • DOI

      10.7566/jpsj.86.093702

    • NAID

      210000134491

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantum critical behavior in magnetic quasicrystals and approximant crystals2017

    • Author(s)
      N. K. Sato, S.Matsukawa, K. Nobe, K. Imura, K. Deguchi, T. Ishimasa
    • Journal Title

      J. Physics Conf. Series

      Volume: 868 Pages: 012005-012005

    • DOI

      10.1088/1742-6596/868/1/012005

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Direct observation of heterogeneous valence state in Yb-based quasicrystalline approximants2017

    • Author(s)
      M. Matsunami, M. Oura, K. Tamasaku, T. Ishikawa, S. Ideta, K. Tanaka, T. Takeuchi, T. Yamada, A.P. Tsai, K. Imura, K. Deguchi, N.K. Sato, T. Ishimasa
    • Journal Title

      Physical Review B

      Volume: 96 Issue: 24

    • DOI

      10.1103/physrevb.96.241102

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Discovery of Quantum-Criticality-Like Behavior in Dilute Kondo System:CexLa1-xCu5.62Au0.382017

    • Author(s)
      T. Shiino, Y. Shinagawa, K. Imura, K. Deguchi, N. K. Sato
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 86 Issue: 12 Pages: 123705-123705

    • DOI

      10.7566/jpsj.86.123705

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Observation of Systematic Variation in Yb Ion Valence as a Function of Interatomic Spacing in Icosahedral Approximant Crystals2017

    • Author(s)
      M. Hayashi, K. Deguchi, S. Matsukawa, K. Imura, and N. K. Sato
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 86 Issue: 4 Pages: 043702-043702

    • DOI

      10.7566/jpsj.86.043702

    • NAID

      210000134324

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Magnetic Properties of the Au-Al-Yb Approximant under Hydrostatic Pressure2017

    • Author(s)
      S. Matsukawa, K. Deguchi, K. Imura, T. Ishimasa, and N. K. Sato
    • Journal Title

      Journal of Physics: Conf. Series

      Volume: 809 Pages: 012013-012013

    • DOI

      10.1088/1742-6596/809/1/012013

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Anticorrelation between polar lattice instability and superconductivity in the Weyl semimetal candidate MoTe22017

    • Author(s)
      H. Takahashi, T. Akiba, K. Imura, T. Shiino, K. Deguchi, N. K. Sato, H. Sakai, M. S. Bahramy, and S. Ishiwata
    • Journal Title

      Phys. Rev. B

      Volume: 95 Issue: 10

    • DOI

      10.1103/physrevb.95.100501

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Aging effects of dodecagonal quasicrystal formed in Mn-Cr-Ni-Si alloys2017

    • Author(s)
      K. Toyonaga, and T. Ishimasa
    • Journal Title

      Journal of Physics: Conf. Series

      Volume: 809 Pages: 012015-012015

    • DOI

      10.1088/1742-6596/809/1/012015

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pressure-Driven Quantum Criticality and T/H Scaling in the Icosahedral Au-Al-Yb Approximant2016

    • Author(s)
      S. Matsukawa, K. Deguchi, K. Imura, T. Ishimasa, and Noriaki K. Sato
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 85 Issue: 6 Pages: 063706-063706

    • DOI

      10.7566/jpsj.85.063706

    • NAID

      40020851813

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Mysteries of icosahedral quasicrystals: how are the atoms arranged ?2016

    • Author(s)
      T. Ishimasa
    • Journal Title

      IUCrJ

      Volume: 3 Issue: 4 Pages: 230-231

    • DOI

      10.1107/s2052252516009842

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Localized Electron Magnetism in the Icosahedral Au-Al-Tm Quasicrystal and Crystalline Approximant2015

    • Author(s)
      M. Nakayama, K. Tanaka, S. Matsukawa, K. Deguchi, K. Imura, T. Ishimasa, and N. K. Sato
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84

    • NAID

      210000133450

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Crystal Structure of Superconducting 1/1 Cubic Au-Ge-Yb Approximant with Tsai-type Cluster2015

    • Author(s)
      K. Deguchi, M. Nakayama, S. Matsukawa, K. Imura, K. Tanaka, T. Ishimasa, N. K. Sato
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 1 Pages: 015002-015002

    • DOI

      10.7566/jpsj.84.015002

    • NAID

      210000133413

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Superconductivity of Au-Ge-Yb Approximants with Tsai-type Clusters2015

    • Author(s)
      K. Deguchi, M. Nakayama, S. Matsukawa, K. Imura, K. Tanaka, T. Ishimasa, N. K. Sato
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 2 Pages: 023705-023705

    • DOI

      10.7566/jpsj.84.023705

    • NAID

      40020360598

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Origin of the black-golden transition in Sm1-xYxS2015

    • Author(s)
      K. Imura, M. Saito, M. Kaneko, T. Ito, T. Hajiri, M. Matsunami, S. Kimura, K. Deguchi, H. S. Suzuki, N. K. Sato
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 592 Pages: 0120281-6

    • DOI

      10.1088/1742-6596/592/1/012028

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Tsai型クラスターをもつAu-Ge-Yb近似結晶の超伝導-準結晶とをつなぐ物質で発現した超伝導-2015

    • Author(s)
      出口和彦,佐藤憲昭,石政勉
    • Journal Title

      固体物理

      Volume: 50 Pages: 497-507

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] ウラン系強磁性超伝導における強磁性ゆらぎが誘起するスピン三重項超伝導2015

    • Author(s)
      石田憲二,服部泰佑,佐藤憲昭,出口和彦,多田靖啓,藤本聡
    • Journal Title

      固体物理

      Volume: 50 Pages: 123-132

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Presentation] 量子臨界現象と高次元性2018

    • Author(s)
      出口和彦
    • Organizer
      日本物理学会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 正20面体準結晶の磁性と超伝導2018

    • Author(s)
      出口和彦
    • Organizer
      J-Physics:多極子伝導系の物理 平成29年度領域全体会議
    • Related Report
      2017 Annual Research Report
  • [Presentation] Au-Ga-Yb準結晶・近似結晶の磁性と電子状態2018

    • Author(s)
      出口和彦, 廣川慎之介, 米山祐樹, 横田晋次郎, 坂本和司、井村敬一郎, 佐藤憲昭, 豊永詞, 石政勉, 山本義哉, 川井拓真, 水木純一郎, 山岡人志, 平岡望, 石井啓文
    • Organizer
      第22回準結晶研究会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Tsai型クラスター構造をもつAu-Al-Yb準結晶の置換効果2017

    • Author(s)
      出口和彦, 難波慶介, 松川周矢, 廣川慎之介, 米山祐樹, 井村敬一郎, 石政勉, 佐藤憲昭
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] Tsai 型クラスター構造をもつAu-Al-Yb 準結晶の置換効果(II)2017

    • Author(s)
      出口和彦, 難波慶介, 松川周矢, 廣川慎之介, 米山祐樹, 横田晋次郎,井村敬一郎, 佐藤憲昭, 豊永詞, 石政勉, 山本義哉, 山岡人志, 平岡望, 石井啓文
    • Organizer
      第21回準結晶研究会
    • Place of Presentation
      北海道大学
    • Year and Date
      2017-03-02
    • Related Report
      2016 Annual Research Report
  • [Presentation] Quantum Criticality and Superconductivity in icosahedral Yb quasicrystals and approximants2017

    • Author(s)
      Kazuhiko Deguchi
    • Organizer
      Open space between aperiodic order and strong electronic correlations
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Magnetic quasicrystal with Yb icosahedron2017

    • Author(s)
      Kazuhiko Deguchi
    • Organizer
      J-Physics 2017: International Workshop on Multipole Physics and Related Phenomena
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 中間価数のYbをもつ磁気準結晶・近似結晶2017

    • Author(s)
      出口和彦
    • Organizer
      J-Physicsトピカルミーティング「局在多極子と伝導電子の相関による新現象」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Physics hidden in open space between heavy fermions and quasicrystals2016

    • Author(s)
      Noriaki K. Sato
    • Organizer
      13th International conference on quasicrystals (ICQ13)
    • Place of Presentation
      Dhulikhel Lodge Resort (Kathmandu, Nepal)
    • Year and Date
      2016-09-18
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Magnetism and superconductivity in icosahedral quasicrystals and approximants with Tsai-type clusters2016

    • Author(s)
      K. Deguchi
    • Organizer
      13th International conference on quasicrystals (ICQ13)
    • Place of Presentation
      Dhulikhel Lodge Resort (Kathmandu, Nepal)
    • Year and Date
      2016-09-18
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dodecagonal quasicrystal in Mn-based alloy2016

    • Author(s)
      T. Ishimasa
    • Organizer
      13th International conference on quasicrystals (ICQ13)
    • Place of Presentation
      Dhulikhel Lodge Resort (Kathmandu, Nepal)
    • Year and Date
      2016-09-18
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] クラスター構造をもつ正20面体準結晶・近似結晶の磁性と超伝導2016

    • Author(s)
      出口和彦
    • Organizer
      J-Physics:多極子伝導系の物理 平成28年度領域全体会議
    • Place of Presentation
      北海道大学
    • Year and Date
      2016-05-26
    • Related Report
      2016 Annual Research Report
  • [Presentation] Quantum Criticality and Superconductivity in Icosahedral Quasicrystals and Approximants with Tsai-type Clusters2016

    • Author(s)
      K. Deguchi
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2016)
    • Place of Presentation
      Zhejiang University (Hangzhou, China)
    • Year and Date
      2016-05-08
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] f電子系準結晶・近似結晶の量子臨界と超電導2016

    • Author(s)
      出口和彦
    • Organizer
      日本物理学会
    • Place of Presentation
      仙台、日本
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Quantum Criticality and Superconductivity in icosahedral Yb quasicrystals and approximants2015

    • Author(s)
      K. Deguchi
    • Organizer
      Toyota RIKEN International Workshop 2015
    • Place of Presentation
      Nagoya, Japan
    • Year and Date
      2015-11-17
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Au-Al-Yb準結晶における量子臨界現象とスケーリング2015

    • Author(s)
      出口和彦,松川周矢,井村敬一郎,佐藤憲昭,石政勉
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪、日本
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Superconductivity of Icosahedral Yb Approximants with Tsai-type Clusters2015

    • Author(s)
      K. Deguchi, M. Nakayama, S. Matsukawa, K. Imura, N. K. Sato, K. Tanaka, and T. Ishimasa
    • Organizer
      International Conference on Magnetism (ICM2015)
    • Place of Presentation
      Spain, Barcelona
    • Year and Date
      2015-07-05
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2020-05-15  

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