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On the temporal variations of the atmospheric methane concentration by precise measurements of carbon and hydrogen isotopes.

Research Project

Project/Area Number 15H03722
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Meteorology/Physical oceanography/Hydrology
Research InstitutionTohoku University

Principal Investigator

MORIMOTO Shinji  東北大学, 理学研究科, 教授 (30270424)

Co-Investigator(Kenkyū-buntansha) 青木 周司  東北大学, 理学研究科, 教授 (00183129)
後藤 大輔  国立極地研究所, 研究教育系, 助教 (10626386)
Research Collaborator ISHIJIMA kentaro  
Project Period (FY) 2015-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥17,420,000 (Direct Cost: ¥13,400,000、Indirect Cost: ¥4,020,000)
Fiscal Year 2018: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2017: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2016: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2015: ¥7,540,000 (Direct Cost: ¥5,800,000、Indirect Cost: ¥1,740,000)
Keywordsメタン / 温室効果気体 / 同位体比 / 環境動態
Outline of Final Research Achievements

Systematic and precise measurements of the concentration and carbon and hydrogen isotope ratios of atmospheric methane were conducted by analyzing air samples regularly collected at northern high latitude sites, Antarctic station and in the western Pacific region, and their short-term, seasonal and long-term variations were identified. Simultaneous analysis with the concentration and isotope ratios suggested that the methane from microbial source could be responsible for the observed regrowth of the methane concentration after 2006 and after 2014. Simulations of the isotope ratios of the atmospheric methane with a three-dimensional atmospheric chemistry-transport model and prescribed methane inventory data gave isotopically lighter results than the observed values in this study. This indicates that the contribution ratio of each source category in the prescribed inventory is different from the real methane sources.

Academic Significance and Societal Importance of the Research Achievements

大気中メタン濃度観測のみからはメタン放出源に関する情報が得られないが、その炭素・水素同位体比の同時高精度観測を行うことにより、メタン放出源の変動に関する情報が得られることが示された。現在の地球表層におけるメタン循環を明らかにし、将来のメタン濃度予測精度を高めるために、メタン濃度と同位体比の同時観測が非常に有効である。

Report

(5 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • Research Products

    (27 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (4 results) Journal Article (6 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 6 results,  Open Access: 3 results) Presentation (16 results) (of which Int'l Joint Research: 7 results,  Invited: 1 results) Remarks (1 results)

  • [Int'l Joint Research] Environment and Climate Change Canada(カナダ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Environment and Climate Change Canada(カナダ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] 環境省研究所(カナダ)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] Meteorological Service of Canada(カナダ)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Temporal variations of the mole fraction, carbon and hydrogen isotope ratios of atmospheric methane in the Hudson Bay Lowlands, Canada.2018

    • Author(s)
      Fujita, R., S. Morimoto, T. Umezawa, K. Ishijima, P. K. Patra, D. E. J. Worthy, D. Goto, S. Aoki and T. Nakazawa
    • Journal Title

      J. Geophys. Res.

      Volume: 123 Issue: 9 Pages: 4695-4711

    • DOI

      10.1002/2017jd027972

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Intercomparisons of d13C and dD measurements of atmospheric CH4 for combined use of datasets from different laboratories2018

    • Author(s)
      Umezawa, T., C.A.M. Brenninkmeijer, T. Roeckmann, C. van der Veen, S. C. Tyler, R. Fujita, S. Morimoto, et al.
    • Journal Title

      Atmos. Meas. Tech.

      Volume: -

    • DOI

      10.5194/amt-2017-281

    • Related Report
      2018 Annual Research Report 2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Long-term variations of the mole fraction and carbon isotope ratio of atmospheric methane observed at Ny-Aalesund, Svalbard from 1996 to 20132017

    • Author(s)
      Morimoto Shinji、Fujita Ryo、Aoki Shuji、Goto Daisuke、Nakazawa Takakiyo
    • Journal Title

      Tellus

      Volume: 69 Issue: 1 Pages: 1380497-1380497

    • DOI

      10.1080/16000889.2017.1380497

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Seasonal and short-term variations in atmospheric potential oxygen at Ny-Aalesund, Svalbard2017

    • Author(s)
      Goto, D., S. Morimoto, S. Aoki, P.K. Patra and T. Nakazawa
    • Journal Title

      Tellus

      Volume: 69B Issue: 1 Pages: 1311767-1311767

    • DOI

      10.1080/16000889.2017.1311767

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ship-based observations of atmospheric potential oxygen and regional air-sea O2 flux in the northern North Pacific and the Arctic Ocean2016

    • Author(s)
      Ishidoya, S., H. Uchida, D. Sasano, N. Kosugi, S. Taguchi, M. Ishii, S. Morimoto, Y. Tohjima, S. Nishino, S. Murayama, S. Aoki, K. Ishijima, R. Fujita, D. Goto and T. Nakazawa
    • Journal Title

      Tellus

      Volume: 68B Issue: 1 Pages: 29972-29972

    • DOI

      10.3402/tellusb.v68.29972

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Development of an atmospheric N2O isotope model, optimization procedure, and application to source estimation2015

    • Author(s)
      Ishijima, K., M. Takigawa, K. Sudo, S. Toyoda, N. Yoshida, T. Röckmann, J. Kaiser, R. G. Prinn, S. Aoki, S. Morimoto, S. Sugawara and T. Nakazawa
    • Journal Title

      Atmos. Chem. Phys. Discuss.

      Volume: 15

    • DOI

      10.5194/acpd-15-19947-2015

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Temporal variations of the mole fraction and carbon isotope ratio of atmospheric methane observed at Ny-Aalesund, Svalbard.2018

    • Author(s)
      Morimoto, S., R. Fujita, S. Aoki, D. Goto and T. Nakazawa
    • Organizer
      14th ICACGP/15th IGAC Science Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Measurements of d13C and dD of atmospheric CH4 in the northern North Pacific and the Arctic Ocean and interpretation of Arctic CH4 sources2018

    • Author(s)
      Fujita, R., S. Morimoto, S. Ishidoya, Y. Tohjima, K. Ishijima, S. Aoki and T. Nakazawa
    • Organizer
      14th ICACGP/15th IGAC Science Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Temporal variations of the global CH4 sources estimated by mole fraction, carbon and hydrogen isotope ratios of atmospheric CH4 and an atmospheric chemistry transport model2018

    • Author(s)
      Fujita, R., S. Maksyutov, S. Morimoto, S. Aoki, T. Nakazawa, H.-S. Kim, T. Umezawam D. Goto, M. Sasakawa and T. Machida
    • Organizer
      日本地球惑星科学連合大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] スバールバル諸島ニーオルスン基地における大気中二酸化炭素、メタン、一酸化炭素濃度の変動2018

    • Author(s)
      村山昌平、森本真司、後藤大輔、青木周司、中澤高清、石島健太郎、前田高尚、石戸谷重之、菅原敏、藤田遼
    • Organizer
      日本気象学会春季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Variations of atmospheric methane and its carbon and hydrogen isotopic ratios observed in the upper troposphere/lowermost stratosphere over the Eurasian Continent2017

    • Author(s)
      Fujita, R., S. Morimoto, Y. Inai, S. Aoki, T. Machida, Y. Sawa, H. Matsueda, Y. Niwa, K. Tsuboi, K. Katsumata, T. Umezawa and T. Nakazawa
    • Organizer
      10th International Carbon Dioxide Conference
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Japanese observation programs of atmospheric greenhouse gases in polar regions2017

    • Author(s)
      Goto, D., S. Morimoto, S. Aoki, T. Nakazawa, S. Ishidoya, S. Murayama, G. Hashida and T. Yamanouchi
    • Organizer
      19th WMO/IAEA Meeting on Carbon Dioxide, Other Greenhouse Gases, and Related Measurement Techniques
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observations of mole fractions and isotope ratios of the atmospheric greenhouse gases2017

    • Author(s)
      Morimoto, S., D. Goto, R. Fujita and S. Aoki
    • Organizer
      8th Symposium on Polar Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Atmospheric methane variations observed in the upper troposphere/lowermost stratosphere over the Eurasian continent and their interpretation based on the carbon and hydrogen isotopic ratios2017

    • Author(s)
      Fujita, R., S. Morimoto, Y. Inai, S. Aoki, T. Machida, Y. Sawa, H. Matsueda, Y. Niwa, K. Tsuboi, K. Katsumata, T. Umezawa and T. Nakazawa
    • Organizer
      日本地球惑星科学連合大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] スバールバル諸島ニーオルスンにおけるメタン炭素同位体比の長期変化2016

    • Author(s)
      森本真司、藤田遼、青木周司、中澤高清、山内恭
    • Organizer
      第7回極域科学シンポジウム
    • Place of Presentation
      国立極地研究所、東京都立川市
    • Year and Date
      2016-11-29
    • Related Report
      2016 Annual Research Report
  • [Presentation] カナダ・チャーチルにおける炭素・水素同位体比の観測から推定された大気中CH4濃度変動にtaiする北方湿地の寄与2016

    • Author(s)
      藤田遼、森本真司、梅澤拓、石島健太郎、P.K. Patra, D.E.J. Worthy
    • Organizer
      第7回極域科学シンポジウム
    • Place of Presentation
      国立極地研究所、東京都立川市
    • Year and Date
      2016-11-29
    • Related Report
      2016 Annual Research Report
  • [Presentation] ユーラシア大陸上空の対流圏界面領域における大気中CH4濃度とその炭素・水素同位体比の季節変動の解析2016

    • Author(s)
      藤田遼、森本真司、青木周司、町田 敏暢,澤 庸介,松枝 秀和,坪井一寛,勝又啓一,梅澤拓,中澤高清
    • Organizer
      日本気象学会秋季大会
    • Place of Presentation
      名古屋大学、愛知県名古屋市
    • Year and Date
      2016-10-26
    • Related Report
      2016 Annual Research Report
  • [Presentation] Source identification of atmospheric methane variations at Churchill, Canada using carbon and hydrogen isotope analyses2016

    • Author(s)
      Fujita, R., S. Morimoto, T. Umezawa, K. Ishijima, P.K. Patra, D.E.J. Worthy, D. Goto, S. Aoki and T. Nakazawa
    • Organizer
      IGAC Science Conference
    • Place of Presentation
      Breckenridge, CO, U.S.A.
    • Year and Date
      2016-09-26
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Regional methane (CH4) emission estimation based on observed atmospheric concentrations (2002-2012)2016

    • Author(s)
      Patra, P. K., T. Saeki, E.J. Dlugokencky, K. Ishijima, T. Umezawa, A. Ito, S. Aoki, S. Morimoto, E.A. Kort, A. Crotwell, K. Ravi Kumar and T. Nakazawa
    • Organizer
      日本地球惑星科学連合大会
    • Place of Presentation
      幕張メッセ、千葉県幕張市
    • Year and Date
      2016-05-22
    • Related Report
      2016 Annual Research Report
  • [Presentation] 放出源別モデル計算を用いたメタンフラックスの最適化について2015

    • Author(s)
      石島健太郎、Prabir Patra、Ed Dlugokencky, 伊藤昭彦、町田敏暢、梅澤拓、青木周司 、森本真司、中澤高清
    • Organizer
      日本気象学会秋季大会
    • Place of Presentation
      京都テルサ、京都府京都市
    • Year and Date
      2015-10-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] カナダ・チャーチルにおける大気中CH4濃度の季節変動とその起源解析2015

    • Author(s)
      藤田遼、森本真司、石島健太郎、Prabir Patra、梅澤拓、Doug Worthy、青木周司、中澤高清
    • Organizer
      第21回大気化学討論会
    • Place of Presentation
      東京工業大学、東京都目黒区
    • Year and Date
      2015-10-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Methane isotope measurements of CARIBIC air samples and preliminary intercomparison results2015

    • Author(s)
      Umezawa,T., C.A.M. Brenninkmeijer, T. Roeckmann, S.C.Tyler, S. Aoki and S. Morimoto
    • Organizer
      InGOS International Conference
    • Place of Presentation
      Utrecht, the Netherlands
    • Year and Date
      2015-09-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Remarks] 温室効果気体観測ネットワーク

    • URL

      http://caos.sakura.ne.jp/tgr/observation/network-2

    • Related Report
      2016 Annual Research Report

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Published: 2015-04-16   Modified: 2020-03-30  

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