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Multi-scale dynamics study using high-intensity neutron beam and its application to the thermoelectric materials research

Research Project

Project/Area Number 15K04742
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Quantum beam science
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

Kajimoto Ryoichi  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 J-PARCセンター, 研究主幹 (30391254)

Co-Investigator(Kenkyū-buntansha) 中村 充孝  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 J-PARCセンター, 研究主幹 (00370445)
稲村 泰弘  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 J-PARCセンター, 研究副主幹 (80343937)
Co-Investigator(Renkei-kenkyūsha) OKUDA Tetsuji  鹿児島大学, 理工学域工学系, 准教授 (20347082)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2017: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2016: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywords中性子散乱 / 熱電材料 / 遷移金属酸化物 / 磁性体 / 格子ダイナミクス / スピンダイナミクス / 中性子非弾性散乱 / フォノン / 実空間局所二体相関 / 中性子散乱データ解析
Outline of Final Research Achievements

We conducted multi-scale dynamics studies of lattice properties in the La+Mn-doped SrTiO3, a new candidate of n-type thermoelectric materials, using neutron scattering. We found a clear correlation between the inelastic neutron scattering spectra and the thermal conductivities of the samples. We further performed similar studies on related materials. In parallel, we developed data analysis methods required in the neutron scattering studies and established the evaluation method of the instrumental resolutions.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (40 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (1 results) Journal Article (8 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 8 results,  Open Access: 4 results,  Acknowledgement Compliant: 2 results) Presentation (31 results) (of which Int'l Joint Research: 9 results,  Invited: 3 results)

  • [Int'l Joint Research] Oakridge National Laboratory(米国)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Effect of rattling motion without cage structure on lattice thermal conductivity in LaOBiS2-xSex2018

    • Author(s)
      Lee C. H.、Nishida A.、Hasegawa T.、Nishiate H.、Kunioka H.、Ohira-Kawamura S.、Nakamura M.、Nakajima K.、Mizuguchi Y.
    • Journal Title

      Applied Physics Letters

      Volume: 112 Issue: 2 Pages: 023903-023903

    • DOI

      10.1063/1.5010373

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Retreat from Stress: Rattling in a Planar Coordination2018

    • Author(s)
      Koichiro Suekuni, Chul Ho Lee, Hiromi I. Tanaka, Eiji Nishibori, Atsushi Nakamura, Hidetaka Kasai, Hidetomo Usui, Masayuki Ochi, Takumi Hasegawa, Mitsutaka Nakamura, Seiko Ohira‐Kawamura, Tatsuya Kikuchi, Koji Kaneko, Hirotaka Nishiate, Katsuaki Hashikuni, Yasufumi Kosaka, Kazuhiko Kuroki, Toshiro Takabatake, 他1名
    • Journal Title

      Advanced Materials

      Volume: 30 Issue: 13 Pages: 1706230-1706230

    • DOI

      10.1002/adma.201706230

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-energy magnetic excitations in lightly oxygen-doped lanthanum nickel oxides2018

    • Author(s)
      Kenji Nakajima and Ryoichi Kajimoto
    • Journal Title

      Physica B: Condensed Matter

      Volume: - Pages: 142-145

    • DOI

      10.1016/j.physb.2017.12.015

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Instrumental Resolution of the Chopper Spectrometer 4SEASONS Evaluated by Monte Carlo Simulation2018

    • Author(s)
      Ryoichi Kajimoto, Kentaro Sato, Yasuhiro Inamura, and Masaki Fujita
    • Journal Title

      AIP Conference Proceedings

      Volume: -

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Status report of the chopper spectrometer 4SEASONS2018

    • Author(s)
      R. Kajimoto, M. Nakamura, Y. Inamura, K. Kamazawa, K. Ikeuchi, K. Iida, M. Ishikado, N. Murai, H. Kira, T. Nakatani, S. Ohira-Kawamura, R. Takahashi, N. Kubo, W. Kambara, K. Nakajima, and K. Aizawa
    • Journal Title

      Journal of Physics: Conference Series

      Volume: -

    • NAID

      120007153033

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex II: Neutron Scattering Instruments2017

    • Author(s)
      K. Nakajima, Y. Kawakita, S. Itoh, et al.
    • Journal Title

      Quantum Beam Science

      Volume: 1 Issue: 3 Pages: 9-9

    • DOI

      10.3390/qubs1030009

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Time-of-Flight Elastic and Inelastic Neutron Scattering Studies on the Localized 4d Electron Layered Perovskite La5Mo4O162017

    • Author(s)
      K. Iida, R. Kajimoto, Y. Mizuno, K. Kamazawa, Y. Inamura, A. Hoshikawa, Y. Yoshida, T. Matsukawa, T. Ishigaki, Y. Kawamura, S. Ibuka, T. Yokoo, S. Itoh, and T. Katsufuji
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 印刷中

    • NAID

      210000134410

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Effects of Mn Substitution on Thermoelectric Properties and Thermal Excitations of the Electron-Doped Perovskite Sr1-xLaxTiO32016

    • Author(s)
      T. Okuda, H. Hata, T. Eto, S. Sobaru, K. Nishina, H. Kuwahara, M. Nakamura, and R. Kajimoto
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 85 Issue: 9 Pages: 094717-094717

    • DOI

      10.7566/jpsj.85.094717

    • NAID

      210000134100

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Researches of magnetism and strongly correlated electron systems using the time-of-flight spectrometer 4SEASONS2018

    • Author(s)
      Ryoichi Kajimoto
    • Organizer
      ISSP - J-PARC Joint Workshop on Science Frontier by Neutron Scattering -The 16th Korea-Japan meeting on Neutron Science-
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] MLF 中性子分光器「四季」2018

    • Author(s)
      梶本亮一, 中村充孝, 蒲沢和也, 稲村泰弘, 池内和彦, 飯田一樹, 石角元志, 村井直樹
    • Organizer
      2017年度量子ビームサイエンスフェスタ/第9回MLFシンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] MLF中性子分光器の現状2018

    • Author(s)
      梶本亮一, 横尾哲也, 中村充孝, 柴田薫, 川北至信, 松浦直人, 遠藤仁, 瀬戸秀紀, 伊藤晋一, 中島健次, 河村聖子
    • Organizer
      2017年度量子ビームサイエンスフェスタ/第9回MLFシンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] MLF 中性子データ処理環境「空蝉」の最新トピック2018

    • Author(s)
      稲村泰弘, 伊藤崇芳, 安芳次, 大下英敏
    • Organizer
      2017年度量子ビームサイエンスフェスタ/第9回MLFシンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] Status Report of the Chopper Spectrometer 4SEASONS2017

    • Author(s)
      R. Kajimoto, M. Nakamura, Y. Inamura, K. Kamazawa, K. Ikeuchi, K. Iida, M. Ishikado, N. Murai, T. Nakatani, N. Kubo, and W. Kambara
    • Organizer
      The 22nd meeting of the International Collaboration on Advanced Neutron Sources (ICANS XXII)
    • Place of Presentation
      オックスフォード(英国)
    • Year and Date
      2017-03-27
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Utsusemi and Software Applications for the Utilization of Event-Recording Data at MLF, J-PARC2017

    • Author(s)
      Y. Inamura, T. Ito , J. Suzuki, R. Kajimoto, and M. Nakamura
    • Organizer
      The 22nd meeting of the International Collaboration on Advanced Neutron Sources (ICANS XXII)
    • Place of Presentation
      オックスフォード(英国)
    • Year and Date
      2017-03-27
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] La, Mn置換したSrTiO3の結晶構造解析2017

    • Author(s)
      梶本亮一, 中村充孝, 社本真一, 池田一貴, 大友季哉, 畑 博人, 江藤貴弘, 奥田哲治
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学豊中キャンパス(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] MLF-BL01 チョッパー分光器「四季」2017

    • Author(s)
      梶本亮一, 中村充孝, 稲村泰弘, 蒲沢和也, 池内和彦, 飯田一樹, 石角元志, 村井直樹, 中谷 健, 久保直也, 神原 理
    • Organizer
      2016年度量子ビームサイエンスフェスタ/第8回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] La, Mn置換したSrTiO3の粉末中性子回折実験2017

    • Author(s)
      梶本亮一, 中村充孝, 社本真一, 池田一貴, 大友季哉, 畑 博人, 江藤貴弘, 奥田哲治
    • Organizer
      2016年度量子ビームサイエンスフェスタ/第8回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] 「空蝉」における単結晶試料の非弾性散乱連続回転測定2017

    • Author(s)
      稲村泰弘, 中谷健, 伊藤崇芳, 梶本亮一, 中村充孝, 鈴木次郎
    • Organizer
      2016年度量子ビームサイエンスフェスタ/第8回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] J-PARC非弾性中性子散乱装置による磁性研究2017

    • Author(s)
      梶本亮一
    • Organizer
      第60回化合物新磁性材料研究会「中性子散乱を利用した化合物磁性研究の最前線」
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Time-of-Flight Direct Geometry Spectrometer 4SEASONS at J-PARC2017

    • Author(s)
      Ryoichi Kajimoto, Mitsutaka Nakamura, Kazuya Kamazawa, Yasuhiro Inamura, Kazuhiko Ikeuchi, Kazuki Iida, Motoyuki Ishikado, and Naoki Murai
    • Organizer
      The International Conference on Neutron Scattering 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Neutron Scattering Instruments of the MLF Spectroscopy Group at J-PARC2017

    • Author(s)
      Ryoichi Kajimoto, Tetsuya Yokoo, Mitsutaka Nakamura, Kaoru Shibata, Yukinobu Kawakita, Masato Matsuura, Hitoshi Endo, Hideki Seto, Shinichi Itoh, Kenji Nakajima, and Seiko Ohira-Kawamura
    • Organizer
      The International Conference on Neutron Scattering 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Performances of oscillating radial collimator for the Fermi chopper spectrometer 4SEASONS at J-PARC2017

    • Author(s)
      Mitsutaka Nakamura, Wataru Kambara, Ryoichi Kajimoto, Kazuya Kamazawa, Kazuhiko Ikeuchi, Kazuki Iida, Motoyuki Ishikado, Kazuhiro Aoyama
    • Organizer
      The International Conference on Neutron Scattering 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Phonon dynamics of NaI investigated by G(r,E) analysis2017

    • Author(s)
      Mitsutaka Nakamura, Tatsuya Kikuchi, Kazuya Kamazawa, Yukinobu Kawakita
    • Organizer
      The International Conference on Neutron Scattering 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁場中中性子回折実験によるLa5Mo4O16の磁気構造の研究2017

    • Author(s)
      梶本亮一, 飯田一樹, 中尾朗子, 茂吉武人, 松田雅昌, Feng Ye, 水野雄介, 勝藤拓郎
    • Organizer
      日本物理学会 2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] J-PARC MLF中性子分光器の現状2017

    • Author(s)
      梶本亮一, 横尾哲也, 中村充孝, 柴田薫, 川北至信, 松浦直人, 遠藤仁, 瀬戸秀紀, 伊藤晋一, 中島健次, 河村聖子
    • Organizer
      日本中性子科学会第 17 回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] MLFの中性子データ処理環境「空蝉」の現状20172017

    • Author(s)
      稲村泰弘, 中谷健, 伊藤崇芳, 安芳次, 大下英敏
    • Organizer
      日本中性子科学会第 17 回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] BL01 四季(4次元空間中性子探査装置)について2017

    • Author(s)
      梶本亮一
    • Organizer
      第6回JASRIワークショップ
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] SrTiO3の結晶構造と格子ダイナミクスにおけるLa, Mn置換効果2017

    • Author(s)
      梶本亮一
    • Organizer
      CMRC研究会「強相関電子系における局所構造変調が誘起する創発現象」
    • Place of Presentation
      KEK東海キャンパス(茨城県東海村)
    • Related Report
      2016 Research-status Report
  • [Presentation] MLFの中性子データ処理環境「空蝉」の現状20162016

    • Author(s)
      稲村泰弘, 中谷 健, 伊藤崇芳, 鈴木次郎
    • Organizer
      日本中性子科学会 第16回年会
    • Place of Presentation
      名古屋大学東山キャンパス(愛知県名古屋市)
    • Year and Date
      2016-12-01
    • Related Report
      2016 Research-status Report
  • [Presentation] Status of the Chopper Spectrometer 4SEASONS at J-PARC2016

    • Author(s)
      R. Kajimoto, M. Nakamura, Y. Inamura, K. Kamazawa, K. Ikeuchi, K. Iida, M. Ishikado, K. Nakajima, S. Ohira-Kawamura, T. Nakatani, W. Kambara
    • Organizer
      The 7th Workshop on Inelastic Neutron Spectrometers (WINS 2016)
    • Place of Presentation
      ポツダム(ドイツ)
    • Year and Date
      2016-09-08
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Instrumental Resolution of the Chopper Spectrometer 4SEASONS Evaluated by Monte Carlo Simulation2016

    • Author(s)
      R. Kajimoto, Y. Inamura, K. Sato, M. Fujita
    • Organizer
      The 7th Workshop on Inelastic Neutron Spectrometers (WINS 2016)
    • Place of Presentation
      ポツダム(ドイツ)
    • Year and Date
      2016-09-08
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] チョッパー型中性子非弾性散乱装置「四季」の現状について2016

    • Author(s)
      梶本亮一 、中村充孝 、稲村泰弘、蒲沢和也、池内和彦、飯田一樹、 石角元志、中島健次、河村聖子、中谷健、神原理 、久保直也 、青山和弘、川上一弘 、山内康弘 、細谷倫紀 、相澤一也、桐山幸治
    • Organizer
      2015年度量子ビームサイエンスフェスタ・第7回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2016-03-15
    • Related Report
      2015 Research-status Report
  • [Presentation] J-PARCチョッパー分光器四季におけるフェルミチョッパーの高度化2016

    • Author(s)
      中村充孝、梶本亮一、稲村泰弘、青山和弘、神原理、川上一弘、久保直也、蒲沢和也、池内和彦、飯田一樹、石角元志
    • Organizer
      2015年度量子ビームサイエンスフェスタ・第7回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2016-03-15
    • Related Report
      2015 Research-status Report
  • [Presentation] MLF中性子データ処理環境「空蝉」の高度化と現状2016

    • Author(s)
      稲村泰弘、伊藤崇芳、中谷健、鈴木次郎
    • Organizer
      2015年度量子ビームサイエンスフェスタ・第7回MLFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県つくば市)
    • Year and Date
      2016-03-15
    • Related Report
      2015 Research-status Report
  • [Presentation] 粉末非弾性中性子散乱によるSrTiO3のフォノンに対する元素置換効果2015

    • Author(s)
      梶本亮一、中村充孝、菊地龍弥、畑 博人、江藤貴弘、草原彰吾、奥田哲治
    • Organizer
      日本中性子科学会第15回年会
    • Place of Presentation
      和光市民文化センター(埼玉県和光市
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
  • [Presentation] J-PARC BL01 チョッパー分光器「四季」’152015

    • Author(s)
      梶本亮一、中村充孝、稲村泰弘、中島健次、河村聖子、中谷 健、神原 理、久保直也、青山和弘、川上一弘、山内康弘、細谷倫紀、相澤一也、蒲沢和也、池内和彦、飯田一樹、石角元志、桐山幸治
    • Organizer
      日本中性子科学会第15回年会
    • Place of Presentation
      和光市民文化センター(埼玉県和光市
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
  • [Presentation] モンテカルロシミュレーションによるチョッパー分光器の分解能評価2015

    • Author(s)
      梶本亮一、稲村泰弘、佐藤研太朗、藤田全基
    • Organizer
      日本中性子科学会第15回年会
    • Place of Presentation
      和光市民文化センター(埼玉県和光市
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
  • [Presentation] MLFの中性子データ処理環境「空蝉」の現状2015

    • Author(s)
      稲村泰弘、中谷健、伊藤崇芳、鈴木次郎
    • Organizer
      日本中性子科学会第15回年会
    • Place of Presentation
      和光市民文化センター(埼玉県和光市
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
  • [Presentation] SrTiO3の熱電特性に対する元素置換効果とフォノン異常2015

    • Author(s)
      梶本亮一
    • Organizer
      ミニ研究会「量子ビーム物性研究の展開」
    • Place of Presentation
      東北大学金属材料研究所(宮城県仙台市)
    • Year and Date
      2015-07-02
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2022-06-06  

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