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Dynamics of valence fluctuation in quantum criticalities for Yb valence fluctuation compounds

Research Project

Project/Area Number 15K05182
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionUniversity of Hyogo

Principal Investigator

Kobayashi Hisao  兵庫県立大学, 物質理学研究科, 教授 (40250675)

Co-Investigator(Kenkyū-buntansha) 池田 修悟  兵庫県立大学, 物質理学研究科, 助教 (80414580)
Co-Investigator(Renkei-kenkyūsha) NAKATSUJI Satoru  東京大学, 物性研究所, 教授 (70362431)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2017: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2016: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2015: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywordsメスバウー分光 / 価数揺動 / 量子臨界性 / 電荷揺らぎダイナミックス / メスバウアー分光 / 放射光X線 / 量子臨界点 / 多重極限 / X線吸収分光
Outline of Final Research Achievements

The synchrotron-radiation based 174Yb Mossbauer spectroscopy is a state-of-the-art technique to investigate the Yb electronic states in materials. We have carried out the first measurement under multi-extreme conditions in the world. The 174Yb ossbauer spectra of b-YbAlB4 observed at lower temperature than 5 K are revealed that the valence fluctuation time is slower than 1 ns. Furthermore, our measurements of 174Yb Mossbauer spectra for b-YbAlB4 under high-pressure at 2K indicate that this slower valence fluctuation in b-YbAlB4 is suppressed at about 2 GPa by external pressure. These results make it clear that the slower valence fluctuation in b-YbAlB4 at a lower temperature and ambient pressure corresponds to the anomalous quantum criticalities. This is a first clear experimental evidence of the relation between quantum criticalities and valence fluctuations.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (38 results)

All 2018 2017 2016 2015

All Journal Article (8 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Open Access: 6 results,  Acknowledgement Compliant: 2 results) Presentation (30 results) (of which Int'l Joint Research: 5 results,  Invited: 3 results)

  • [Journal Article] Valence fluctuating compound a-YbAlB4 studied by 174Yb Mossbauer spectroscopy and X-ray diffraction using synchrotron radiation.2018

    • Author(s)
      M. Oura, et al.
    • Journal Title

      Physica B

      Volume: 印刷中

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 57Fe Mossbauer and Co Kb x-ray emission spectroscopic investigations of La-Co and La substituted strontium hexaferrite.2018

    • Author(s)
      M. Oura, et al.
    • Journal Title

      J. Appl. Phys.

      Volume: 123 Pages: 0339071-6

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Charge ordering in Sm4Bi3 under pressure2017

    • Author(s)
      H. Kobayashi, et al.
    • Journal Title

      J. Phys.: Conf. Series

      Volume: 950 Pages: 0420351-5

    • DOI

      10.1088/1742-6596/950/4/042035

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Pressure-induced Phase Transition in KxFe2-yS22017

    • Author(s)
      Y. Tsuchiya, S. Ikeda, X.-W. Zhang, S. Kishimoto, T. Kikegawa, N. Hirao, S.I. Kawaguchi, Y. Ohishi, and H. Kobayashi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 86 Issue: 3 Pages: 033705-033705

    • DOI

      10.7566/jpsj.86.033705

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Single-crystalline M-type Sr hexaferrite studied by 57Fe Mossbauer spectroscopy2016

    • Author(s)
      N. Nagasawa, S. Ikeda, A. Shimoda, T. Waki, Y. Tabata, H. Nakamura, and H. Kobayashi
    • Journal Title

      Hyperfine Interact.

      Volume: 238 Issue: 1

    • DOI

      10.1007/s10751-016-1272-y

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Pressure-Induced Local Structural Changes in Heavy Fermion b-YbAlB42016

    • Author(s)
      Y. Sakaguchi, et al.
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 85 Issue: 2 Pages: 023602-023602

    • DOI

      10.7566/jpsj.85.023602

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 57Fe Mossbauer spectroscopic studies of single-crystalline KxFe2-yS2 and KxFe2-ySe22016

    • Author(s)
      Y. Tsuchiya, et al.
    • Journal Title

      Hyperfine Interact.

      Volume: 237 Issue: 1

    • DOI

      10.1007/s10751-016-1278-5

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Pressure-induced unusual metallic state in EuNiO32015

    • Author(s)
      H. Kobayashi, et al.
    • Journal Title

      Phys. Rev. B

      Volume: 91 Issue: 19 Pages: 195148-195148

    • DOI

      10.1103/physrevb.91.195148

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] 重い電子系化合物 a-YbAlB4 の低温における磁場下物性2018

    • Author(s)
      大浦桃子 他
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 価数揺動物質 YbAlB4 の低温・高圧力下 174Yb 放射光メスバウアー分法による研究2018

    • Author(s)
      小林寿夫 他
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] RNiO3 (R: 希土類)の圧力誘起金属 絶縁体転移とNiの電子状態2018

    • Author(s)
      永澤延元 他
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 圧力下超伝導におけるSrFe2As2の磁性と構造2018

    • Author(s)
      池田修悟 他
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 反強磁性EuNiIn4 の 151Eu メスバウアー分光測定2017

    • Author(s)
      池田修悟, 本間佳哉, 花島隆泰, 中尾朗子, 鬼柳亮嗣, 金子耕士, 小林寿夫
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大(大阪府豊中市)
    • Year and Date
      2017-03-20
    • Related Report
      2016 Research-status Report
  • [Presentation] YbNiO3 における高圧下でのNiの電子状態とNi近傍の結晶構造2017

    • Author(s)
      永澤延元, 池田修悟, 河口沙織, 平尾直久, 大石泰生, 平岡望, J.A. Alons, M.J. Martinez-Lope, M.M. Abd-Elmeguid, 小林寿夫
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大(大阪府豊中市)
    • Year and Date
      2017-03-18
    • Related Report
      2016 Research-status Report
  • [Presentation] Snフラックス法によるEu(Fe1-xCox)2As2の純良単結晶育成とその物性2017

    • Author(s)
      南野良介, 池田修悟, 小林寿夫
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大(大阪府豊中市)
    • Year and Date
      2017-03-18
    • Related Report
      2016 Research-status Report
  • [Presentation] 重い電子系化合物 a-YbAlB4 の低温における圧力・磁場下物性2017

    • Author(s)
      大浦桃子, 池田修悟, 増田亮, 小林康浩, 瀬戸誠, 依田芳卓, 平尾直久. 河口沙織, 大石泰生, 鈴木慎太郎, 久我健太郎, 中辻知, 小林寿夫
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] Unusual magnetic ordered metallic state in EuNiO3 under pressure.2017

    • Author(s)
      H. Kobayashi
    • Organizer
      XXIV Congress of Inter. Union of Crystallography
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Physical properties of heavy fermion compound YbAlB4 at low temperature under pressure and magnetic fields2017

    • Author(s)
      M. Oura 他
    • Organizer
      The International Conference on Strongly Correlated Electron Systems
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Synchrotron-Radiation-Based 174Yb Mossbauer spectroscopic studies on a-YbAlB4 with external magnetic field2017

    • Author(s)
      H. Kobayashi 他
    • Organizer
      The International Conference on Strongly Correlated Electron Systems
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 重い電子系化合物 α-YbAlB4の低温における圧力・磁場下物性Ⅱ2017

    • Author(s)
      大浦桃子 他
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 価数不均化を示すRNiO3 の Ni の電子状態2017

    • Author(s)
      永澤延元 他
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Sn フラックス法によるEu(Fe1-xCox)2As2 の磁性と超伝導の Co 置換量依存性2017

    • Author(s)
      南野良介 他
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 鉄系超伝導体 SrFe2As2 高圧力下粉末X線回折実験2017

    • Author(s)
      池田修悟 他
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 放射光を用いた高圧力下核共鳴散乱法の現状と将来展望2016

    • Author(s)
      小林寿夫
    • Organizer
      第57回高圧討論会
    • Place of Presentation
      筑波大学(茨城県つくば市)
    • Year and Date
      2016-10-28
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] X線発光分光を用いたYbNiO3のNi価数の圧力依存性2016

    • Author(s)
      永澤延元, 大浦桃子, 池田修悟, 平岡望, J.A.~Alonso, M.J. Martinez-Lope, M.M. Abd-Elmeguid, 小林寿夫
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-15
    • Related Report
      2016 Research-status Report
  • [Presentation] KxFe2-yS2の圧力誘起相転移の研究II2016

    • Author(s)
      土屋 優
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-15
    • Related Report
      2016 Research-status Report
  • [Presentation] EuFe2As2におけるセンタセンターシフトの圧力依存性2016

    • Author(s)
      池田修悟, 土屋 優, 張 小威, 岸本俊二, 亀掛川卓美, 小林寿夫:
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-14
    • Related Report
      2016 Research-status Report
  • [Presentation] 価数揺動物質YbAlB4の磁場中174Yb放射光メスバウアー分法による研究2016

    • Author(s)
      小林寿夫大, 浦桃子, 阪口友唯, 池田修悟, 増田亮, 瀬戸誠, 依田芳卓, 鈴木慎太郎, 久我健太郎, 中辻知
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-14
    • Related Report
      2016 Research-status Report
  • [Presentation] La置換M型Srフェライトの57Feメスバウアー分光法による研究2016

    • Author(s)
      大浦桃子 他
    • Organizer
      第40回日本磁気学会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-06
    • Related Report
      2016 Research-status Report
  • [Presentation] KxFe2-yS2の圧力誘起相転移の研究2016

    • Author(s)
      土屋 優 他
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県仙台市)
    • Year and Date
      2016-03-22
    • Related Report
      2015 Research-status Report
  • [Presentation] 核共鳴前方散乱実験による圧力下EuFe2As2の電子状態の研究2016

    • Author(s)
      池田修悟 他
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県仙台市)
    • Year and Date
      2016-03-21
    • Related Report
      2015 Research-status Report
  • [Presentation] YbNiO3の圧力下におけるX線結晶構造解析2016

    • Author(s)
      永澤延元 他
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県仙台市)
    • Year and Date
      2016-03-21
    • Related Report
      2015 Research-status Report
  • [Presentation] 層状Yb化合物の圧力下の物性研究2015

    • Author(s)
      鵜川絵里 他
    • Organizer
      第56回高圧討論会
    • Place of Presentation
      JMSアステールプラザ(広島県広島市)
    • Year and Date
      2015-11-10
    • Related Report
      2015 Research-status Report
  • [Presentation] AFe2As2(A:Sr,Eu)の磁性と超伝導2015

    • Author(s)
      池田修悟 他
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府吹田市)
    • Year and Date
      2015-09-19
    • Related Report
      2015 Research-status Report
  • [Presentation] (Sr,K)Fe2As2の単結晶試料育成と物性2015

    • Author(s)
      中村 歩 他
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府吹田市)
    • Year and Date
      2015-09-19
    • Related Report
      2015 Research-status Report
  • [Presentation] 多重極限環境下におけるb-YbAlB4のX線吸収分光III2015

    • Author(s)
      阪口友唯 他
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府吹田市)
    • Year and Date
      2015-09-18
    • Related Report
      2015 Research-status Report
  • [Presentation] Nuclear resonance scattering on iron-based high-Tc superconductors.2015

    • Author(s)
      H. Kobayashi
    • Organizer
      The 33rd Inter. Conf. on Applications of Mossbauer Effect
    • Place of Presentation
      Hamburg Germany
    • Year and Date
      2015-09-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 57Fe Mossbauer spectroscopic studies of single-crystalline KxFe2-yS2 and KxFe2-ySe22015

    • Author(s)
      Y. Tsuchiya, et al.
    • Organizer
      The 33rd Inter. Conf. on Applications of Mossbauer Effect
    • Place of Presentation
      Hamburg Germany
    • Year and Date
      2015-09-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research

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Published: 2015-04-16   Modified: 2020-05-15  

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