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Magnetocaloric-effect study on quantum-spin-liquid states of organic triangular-lattice systems

Research Project

Project/Area Number 15K05188
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionInstitute of Physical and Chemical Research (2016-2017)
National Institute for Materials Science (2015)

Principal Investigator

Isono Takayuki  国立研究開発法人理化学研究所, 加藤分子物性研究室, 特別研究員 (70625631)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2016: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2015: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywords量子スピン液体 / 三角格子有機磁性体 / 磁気熱量効果
Outline of Final Research Achievements

In order to systematically understand magnetic excitations in quantum spin-liquid states of organic triangular-lattice magnets, we performed torque magnetometry and magnetocaloric-effect study on kappa-(BEDT-TTF)2Cu2(CN)3. We found from the torque magnetometry that the magnetic susceptibility is scaled in the wide temperature and field region, which unveils the zero-field quantum criticality, and the value of the critical exponents. The magnetocaloric-effect measurements revealed that the electron-spin system is decoupled from the lattice bath at low temperature and in magnetic field. This spin-lattice decoupling phenomenon well explains the discrepancy of the low-energy excitation spectrum of kappa-(BEDT-TTF)2Cu2(CN)3. The present results provide the unified understanding to the macroscopic properties of the quantum spin-liquid states in the organic triangular-lattice systems.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (13 results)

All 2018 2017 2016 2015

All Journal Article (8 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 8 results,  Open Access: 2 results) Presentation (5 results) (of which Invited: 2 results)

  • [Journal Article] Spin-lattice decoupling in a triangular-lattice quantum spin liquid2018

    • Author(s)
      Takayuki Isono, Shiori Sugiura, Taichi Terashima, Kazuya Miyagawa, Kazushi Kanoda and Shinya Uji
    • Journal Title

      Nature Communications

      Volume: 9 Issue: 1

    • DOI

      10.1038/s41467-018-04005-1

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Fulde-Ferrell-Larkin-Ovchinnikov superconductivity in the layered organic superconductor b”-(BEDT-TTF)4[(H3O)Ga(C2O4)3]C6H5NO22018

    • Author(s)
      S. Uji, Y. Iida, S. Sugiura, T. Isono, K. Sugii, N. Kikugawa, T. Terashima, S. Yasuzuka, H. Akutsu, Y. Nakazawa, D. Graf, P. Day
    • Journal Title

      Phys. Rev. B

      Volume: 97 Issue: 14 Pages: 144505-144505

    • DOI

      10.1103/physrevb.97.144505

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetocaloric Effect in Layered Organic Conductor lambda-(BETS)2FeCl42018

    • Author(s)
      Shiori Sugiura, Kazuo Shimada, Naoya Tajima, Yutaka Nishio, Taichi Terashima, Takayuki Isono, Reizo Kato, Biao Zhou, Shinya Uji
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 4 Pages: 044601-044601

    • DOI

      10.7566/jpsj.87.044601

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Quantum vortex melting and phase diagram in the layered organic superconductor κ-(BEDT-TTF)2Cu(NCS)22018

    • Author(s)
      S. Uji, Y. Fujii, S. Sugiura, T. Terashima, T. Isono, J. Yamada
    • Journal Title

      Phys. Rev. B

      Volume: 97 Issue: 2

    • DOI

      10.1103/physrevb.97.024505

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic Torque Studies in Two-Dimensional Organic Conductor λ-(BETS)2FeCl42017

    • Author(s)
      S. Sugiura, K. Shimada, N. Tajima, Y. Nishio, T. Terashima, T. Isono, R. Kato, and S. Uji
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 86 Issue: 1 Pages: 014702-014702

    • DOI

      10.7566/jpsj.86.014702

    • NAID

      210000134224

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Quantum criticality in an organic spin-liquid insulator κ-(BEDT-TTF)2(CN)32016

    • Author(s)
      Takayuki Isono, Taichi Terashima, Kazuya Miyagawa, Kazushi Kanoda, and Shinya Uji
    • Journal Title

      Nature Communications

      Volume: 7 Issue: 1 Pages: 13494-13494

    • DOI

      10.1038/ncomms13494

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Charge Transport in Antiferromagnetic Insulating Phase of Two-Dimensional Organic Conductor λ-(BETS)2FeCl42016

    • Author(s)
      S. Sugiura, K. Shimada, N. Tajima, Y. Nishio, T. Terashima, T. Isono, A. Kobayashi, B. Zhou, R. Kato, and S. Uji
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 85 Issue: 6 Pages: 064703-064703

    • DOI

      10.7566/jpsj.85.064703

    • NAID

      210000133965

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] In-Plane Anisotropy of Upper Critical Field and Flux-Flow Resistivity in Layered Organic Superconductor β”-(ET)2SF5CH2CF2SO32015

    • Author(s)
      S. Yasuzuka, S. Uji, T. Terashima, K. Sugii, T. Isono, Y. Iida, and J. A. Schlueter
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 84 Issue: 9 Pages: 094709-094709

    • DOI

      10.7566/jpsj.84.094709

    • NAID

      210000133679

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] スピン液体的振舞を示す三角格子有機磁性体の磁気特性の系統的研究2018

    • Author(s)
      磯野貴之
    • Organizer
      日本物理学会 2018年年次大会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 磁気トルクで見た有機三角格子系X[Pd(dmit)2]2 (X = Me4P, Me4Sb)の反強磁性状態2017

    • Author(s)
      磯野貴之,崔亨波,杉浦栞理,寺嶋太一,宇治進也,加藤礼三
    • Organizer
      日本物理学会 2017年年次大会
    • Place of Presentation
      大阪大学(大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Research-status Report
  • [Presentation] 有機三角格子系物質κ-(BEDT-TTF)2Cu2(CN)3におけるスピン-格子デカップリング2016

    • Author(s)
      磯野貴之,杉浦栞理,寺嶋太一,宮川和也,鹿野田一司,宇治進也
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学(石川県金沢市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 有機三角格子系物質κ-(BEDT-TTF)2Cu2(CN)3における量子臨界現象2016

    • Author(s)
      磯野貴之,寺嶋太一,宮川和也,鹿野田一司,宇治進也
    • Organizer
      日本物理学会 2016年年次大会
    • Place of Presentation
      東北学院大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] 有機三角格子系における量子スピン液体状態の低温磁気トルク2015

    • Author(s)
      磯野貴之
    • Organizer
      日本物理学会 2015年秋季大会
    • Place of Presentation
      関西大学
    • Year and Date
      2015-09-18
    • Related Report
      2015 Research-status Report
    • Invited

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Published: 2015-04-16   Modified: 2020-05-15  

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