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Liquid cluster ion beam processing of metal films for spintronics devices

Research Project

Project/Area Number 15K06015
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Electron device/Electronic equipment
Research InstitutionKyoto University

Principal Investigator

Ryuto Hiromichi  京都大学, 工学研究科, 講師 (20392178)

Co-Investigator(Kenkyū-buntansha) 竹内 光明  京都大学, 工学研究科, 助教 (10552656)
Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥520,000 (Direct Cost: ¥400,000、Indirect Cost: ¥120,000)
Fiscal Year 2015: ¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Keywordsクラスター / イオンビーム / スピントロニクス / マグネトロン / スパッタリング / 遷移金属 / アルコール / ビーム応用 / 表面加工 / 薄膜 / プロセッシング
Outline of Final Research Achievements

Ethanol cluster ion beams were irradiated on metal surfaces to examine the possibility of applying the liquid cluster ion beam technique to the processing of metal films used in spintronics devices. To perform the processing of metal films using liquid cluster ion beams without exposing the fresh film surfaces just after deposition to the air, a setup combining a liquid cluster ion beam system and magnetron sputtering system was constructed. The sputtering yields of copper, tantalum, and platinum induced by ethanol cluster ions were much larger than those by argon monomer ions at 500 eV. The sputtering yields of metal films kept in vacuum were also larger than those exposed to the air after deposition. The possibility of the liquid cluster ion beam processing of metal films was demonstrated.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (34 results)

All 2017 2016 2015 Other

All Int'l Joint Research (3 results) Journal Article (7 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 7 results,  Open Access: 2 results) Presentation (24 results) (of which Int'l Joint Research: 7 results)

  • [Int'l Joint Research] INFN-LNS/Catania University(イタリア)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] カターニア大学/INFN-LNS(イタリア)

    • Related Report
      2016 Research-status Report
  • [Int'l Joint Research] カターニア大学/INFN-LNS(イタリア)

    • Related Report
      2015 Research-status Report
  • [Journal Article] Effects of ion irradiation on seedlings growth monitored by ultraweak delayed luminescence2016

    • Author(s)
      R. Grasso, T. Abe, G. A. P. Cirrone, G. Cuttone, M. Gulino, F. Musumeci, F. Romano, H. Ryuto, A. Scordino
    • Journal Title

      PLoS ONE

      Volume: 11 Issue: 12 Pages: e0167998-e0167998

    • DOI

      10.1371/journal.pone.0167998

    • NAID

      120005980898

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Crystal Structure and Accelerated Ion-Irradiation Effect of Water Clusters2016

    • Author(s)
      G. H. Takaoka,H. Ryuto, M. Takeuchi, F. Musumeci
    • Journal Title

      e-Journal of Surface Science and Nanotechnology

      Volume: 14 Pages: 144-149

    • NAID

      130005151356

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Characterization by transmission electron microscopy and small-angle X-ray scattering of Au clusters formed in ionic liquids2016

    • Author(s)
      G. H. Takaoka, Y. Matsumoto, M. Takeuchi, H. Ryuto
    • Journal Title

      Surface and interface analysis

      Volume: 48 Issue: 11 Pages: 1148-1152

    • DOI

      10.1002/sia.6132

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Sputtering of silicon and glass substrates with polyatomic molecular ion beams generated from ionic liquids2016

    • Author(s)
      M. Takeuchi, Y. Hoshide, H. Ryuto, G. H. Takaoka
    • Journal Title

      J. Vac. Sci. Technol. A

      Volume: 34 Issue: 2

    • DOI

      10.1116/1.4942996

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Spectroscopic evidences of high temperatures and pressures during the cluster ion beam interaction with solid surfaces2016

    • Author(s)
      F. Musumeci, H. Ryuto, A. Sakata, M. Takeuchi, G. H. Takaoka
    • Journal Title

      Journal of Luminescence

      Volume: 172 Pages: 224-230

    • DOI

      10.1016/j.jlumin.2015.12.018

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Growth behavior of gold nanoparticles synthesized in unsaturated fatty acids by vacuum evaporation methods2016

    • Author(s)
      A. Fujita, Y. Matsumoto, M. Takeuchi, H. Ryuto, G. H. Takaoka
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 18 Issue: 7 Pages: 5464-5470

    • DOI

      10.1039/c5cp07323e

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ion-Beam Deposition/Etching Using EMIM-N(CN)<sub>2</sub> Ionic Liquid Ion Source2015

    • Author(s)
      M. Takeuchi, Y. Hoshide, T. Hamaguchi, H. Ryuto, G. H. Takaoka
    • Journal Title

      Transactions of the Materials Research Society of Japan

      Volume: 40 Issue: 2 Pages: 87-90

    • DOI

      10.14723/tmrsj.40.87

    • NAID

      130005089519

    • ISSN
      1382-3469, 2188-1650
    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] 液体クラスターイオンビームの遷移金属薄膜への照射効果2017

    • Author(s)
      清水友規、清水大貴、竹内光明、龍頭啓充
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川県・横浜市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] クラスターイオンビーム誘起発光を用いた表面分析法の開発2017

    • Author(s)
      山岡昌貴、龍頭啓充、Francesco Musumeci、竹内光明
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川県・横浜市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] 竹炭を用いたイオン液体イオン源の長時間動作特性2017

    • Author(s)
      東浦佑真、西和哉、竹内光明、龍頭啓充
    • Organizer
      第64回応用物理学会春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川県・横浜市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Research-status Report
  • [Presentation] Sputtering and photon emission of metal surface induced by cluster ion collision2017

    • Author(s)
      H. Ryuto, Y. Shimizu, M. Yamaoka, D. Shimizu, D. Yamamoto, M. Takeuchi, F. Musumeci
    • Organizer
      International Union of Material Research Societies-The 15th International Conference on Advanced Materials (IUMRS-ICAM2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Long-life emitter for ionic liquid ion source using open-pore structure of bamboo chacoal2017

    • Author(s)
      M. Takeuchi, Y. Higashiura, K. Nishi, H. Ryuto
    • Organizer
      International Union of Material Research Societies-The 15th International Conference on Advanced Materials (IUMRS-ICAM2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 液体クラスターイオンビームによる遷移金属薄膜の表面加工2017

    • Author(s)
      清水大貴、山本大介、竹内光明、龍頭啓充
    • Organizer
      応用物理学会関西支部平成29年度第2回講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 数十keV電子線照射によるイオン液体中でのCu薄膜の形成2017

    • Author(s)
      東浦佑真、竹内光明、龍頭啓充
    • Organizer
      応用物理学会関西支部平成29年度第2回講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] CuCl含有イオン液体EMIM -DCAへの電子線照射によるCu薄膜の形成2017

    • Author(s)
      東浦佑真、竹内光明、龍頭啓充
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 遷移金属薄膜に対する液体クラスターイオンビームの照射効果2017

    • Author(s)
      清水大貴、山本大介、竹内光明、龍頭啓充
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Etching, oxidation, and photon emission induced by cluster ion collision2017

    • Author(s)
      H. Ryuto, M. Takeuchi
    • Organizer
      International Symposium on Photonics and Electronics Science and Engineering 2017
    • Place of Presentation
      京都大学(京都府・京都市)
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Setup for measuring cluster ion beam induced luminescence2016

    • Author(s)
      山岡昌貴、松井亮祐、Francesco Musumeci、竹内光明、龍頭啓充
    • Organizer
      第17回「イオンビームによる表面・界面解析」特別研究会
    • Place of Presentation
      京都府立大学(京都府・京都市)
    • Year and Date
      2016-12-03
    • Related Report
      2016 Research-status Report
  • [Presentation] Sputtering, oxidation, and photon emission induced by liquid cluster ion collision2016

    • Author(s)
      H. Ryuto, M. Takeuchi, F. Musumeci, G. H. Takaoka
    • Organizer
      Ninth International Meeting on Recent Developments in the Study of Radiation Effects in Matter (REM9)
    • Place of Presentation
      京都市国際交流会館(京都府・京都市)
    • Year and Date
      2016-10-26
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 竹炭エミッタを用いたイオン液体イオン源の開発2016

    • Author(s)
      竹内光明、西和哉、龍頭啓充
    • Organizer
      第77回応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ(新潟県・新潟市)
    • Year and Date
      2016-09-13
    • Related Report
      2016 Research-status Report
  • [Presentation] 固体表面へのクラスターイオンビーム照射による発光スペクトル2016

    • Author(s)
      織田 啓佑、龍頭 啓充、Francesco Musumeci、竹内 光明、高岡義寛
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] イオン液体EMIM-BF4 イオンビームの固体表面照射効果2016

    • Author(s)
      西和哉, 上田弘貴, 藤井志貴, 竹内光明, 龍頭啓充, 高岡義寛
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] イオン液体EMIM-DCAイオンビームの表面処理応用に関する検討2016

    • Author(s)
      竹内光明, 星出優輝, 竹内裕人, 龍頭啓充, 高岡義寛
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] イオン液体EMIM-DCAイオンビーム蒸着によるCN膜の形成2016

    • Author(s)
      竹内光明、西和哉、龍頭啓充
    • Organizer
      応用物理学会関西支部平成28年度第1回講演会
    • Place of Presentation
      産業技術総合研究所(大阪府・池田市)
    • Related Report
      2016 Research-status Report
  • [Presentation] イオン液体EMIM-BF4から生成したBF4イオンによる二次イオン収率評価2016

    • Author(s)
      西和哉、竹内光明、龍頭啓充
    • Organizer
      応用物理学会関西支部平成28年度第1回講演会
    • Place of Presentation
      産業技術総合研究所(大阪府・池田市)
    • Related Report
      2016 Research-status Report
  • [Presentation] 固体試料のクラスターイオンビーム誘起発光スペクトル2016

    • Author(s)
      山岡昌貴、織田啓佑、龍頭啓充、Francesco Musumeci、坂田彬、竹内光明、高岡義寛
    • Organizer
      応用物理学会関西支部平成28年度第1回講演会
    • Place of Presentation
      産業技術総合研究所(大阪府・池田市)
    • Related Report
      2016 Research-status Report
  • [Presentation] イオン液体イオンビームにより形成したC-N薄膜の基板温度依存性2015

    • Author(s)
      星出優輝、竹内光明、龍頭啓充、高岡義寛
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
  • [Presentation] Sputtering of silicon and glass substrates with polyatomic molecular ion beams generated from ionic liquids2015

    • Author(s)
      M. Takeuchi, Y. Hoshide, H. Ryuto, G. H Takaoka
    • Organizer
      Thirteenth International Symposium on Sputtering & Plasma Processes, ISSP 2015
    • Place of Presentation
      京都
    • Year and Date
      2015-07-08
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Oxygen cluster ion beam assisted deposition of aluminum oxide film2015

    • Author(s)
      H. Ryuto, T. Yakushiji, M. Takeuchi, G. H. Takaoka
    • Organizer
      Thirteenth International Symposium on Sputtering & Plasma Processes, ISSP 2015
    • Place of Presentation
      京都
    • Year and Date
      2015-07-08
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Interaction of polyatomic carbon ions with Si surface2015

    • Author(s)
      M. Takeuchi, K. Hayashi, H. Ryuto, G. H Takaoka, T. Nagayama, K. Matsuda
    • Organizer
      Thirteenth International Symposium on Sputtering & Plasma Processes, ISSP 2015
    • Place of Presentation
      京都
    • Year and Date
      2015-07-08
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] アルゴンクラスターイオンビーム照射による発光スペクトル2015

    • Author(s)
      龍頭啓充、Francesco Musumeci、坂田彬、竹内光明、高岡義寛
    • Organizer
      ナノ学会第13回大会
    • Place of Presentation
      仙台
    • Year and Date
      2015-05-11
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2019-03-29  

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